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Cryogenic temperatures are the prerequisite for many advanced scientific applications and technologies. The accurate determination of temperature in this range and at the submicrometer scale is, however, nontrivial. This is due to the fact…

Transition metal dichalcogenides hold promise for applications in novel optoelectronic devices. There is therefore a need for materials that can be obtained in large quantities and with well understood optical properties. In this report, we…

介观与纳米尺度物理 · 物理学 2018-01-04 Ł. Kłopotowski , C. Backes , A. A. Mitioglu , V. Vega-Mayoral , D. Hanlon , J. N. Coleman , V. Y. Ivanov , D. K. Maude , P. Plochocka

Lead-halide perovskite nanocrystals such as CsPbBr$_3$, exhibit efficient photoluminescence (PL) up-conversion, also referred to as anti-Stokes photoluminescence (ASPL). This is a phenomenon where irradiating nanocrystals up to 100 meV…

介观与纳米尺度物理 · 物理学 2024-02-29 Zhuoming Zhang , Sushrut Ghonge , Yang Ding , Shubin Zhang , Mona Berciu , Richard D. Schaller , Boldizsár Jankó , Masaru Kuno

Two-dimensional monolayer transition metal dichalcogenides (TMDs) have unique optical and electronic properties for applications pertaining to field effect transistors, light emitting diodes, photodetectors, and solar cells. Vertical…

Colloidal Cadmium Selenide (CdSe) nanoplatelets (NPLs) are a recently developed class of efficient luminescent nanomaterial suitable for optoelectronic device applications. A change in temperature greatly affects their electronic…

介观与纳米尺度物理 · 物理学 2017-10-26 Sumanta Bose , Sushant Shendre , Zhigang Song , Vijay Kumar Sharma , Dao Hua Zhang , Cuong Dang , Weijun Fan , Hilmi Volkan Demir

Nanoscale thermometry is paramount to study primary processes of heat transfer in solids and is a subject of hot debate in cell biology. Here we report ultrafast temperature sensing using all-optical thermometry exploiting synthetic…

应用物理 · 物理学 2019-04-24 Sumin Choi , Viatcheslav N. Agafonov , Valery A. Davydov , Taras Plakhotnik

Anti-Stokes photoluminescence of metal nanoparticles, in which emitted photons have a higher energy than the incident photons, is an indicator of the temperature prevalent within a nanoparticle. Previous work has shown how to extract the…

光学 · 物理学 2020-08-21 Thomas Jollans , Martín Caldarola , Yonatan Sivan , Michel Orrit

Near-field optical microscopy can be used as a viable route to understand the nanoscale material properties below the diffraction limit. On the other hand, atomically thin two-dimensional (2D) transition metal dichalcogenides (TMDs) are the…

Two-dimensional (2D) transition metal dichalcogenides (TMDs) with tantalizing layer-dependent electronic and optical properties have emerged as a new paradigm for integrated flat opto-electronic devices. However, daunting challenges remain…

光学 · 物理学 2021-02-23 Dejiao Hu , Hao Li , Yupeng Zhu , Yuqiu Lei , Jiajin Zheng , Yaoyu Cao , Bai-Ou Guan , Lei Bi , Xiangping Li

Transition metal dichalcogenides (TMDs) is a promising platform for new generation optoelectronics and nanophotonics due to their unique optical properties. However, in contrast to direct bandgap TMDs monolayers, bulk samples have an…

Hyperspectral photoluminescence (HSPL) imaging provides spatially resolved spectral information for monolayer transition-metal dichalcogenides (TMDs), enabling the detection of subtle variations in excitonic features that are not accessible…

材料科学 · 物理学 2026-04-03 Adam Alfrey , Cole Tait , Takashi Taniguchi , Kenji Watanabe , Steven T. Cundiff

Two-dimensional materials, including transition metal dichalcogenides, are attractive for a variety of applications in electronics as well as photonics and have recently been envisioned as an appealing platform for phonon polaritonics.…

Monolayer transition metal dichalcogenides (TMDs) show an optimal surface-to-volume ratio and are thus promising candidates for novel molecule sensor devices. It was recently predicted that a certain class of molecules exhibiting a large…

Lanthanide-doped upconversion nanoparticles emerged recently as an attractive material platform underpinning a broad range of innovative applications such as optical cryptography, luminescent probes, and lasing. However, the intricate…

光学 · 物理学 2023-05-17 Ziwei Feng , Tan Shi , Guangzhou Geng , Junjie Li , Zi-Lan Deng , Yuri Kivshar , Xiangping Li

Individual monolayers of metal dichalcogenides are atomically thin two-dimensional crystals with attractive physical properties different from their bulk layered counterpart. Here we describe the direct synthesis of WS2 monolayers with…

Monolayers of Transition Metal Dichalcogenides (TMDs) are atomically thin two-dimensional crystals with attractive optoelectronic properties, which are promising for emerging applications in nanophotonics. Here, we report on the…

材料科学 · 物理学 2016-06-27 I. Paradisanos , N. Pliatsikas , P. Patsalas , C. Fotakis , E. Kymakis , G. Kioseoglou , E. Stratakis

Nanoplasmonic systems combined with optically-active two-dimensional materials provide intriguing opportunities to explore and control light-matter interactions at extreme sub-wavelength lengthscales approaching the exciton Bohr radius.…

Anti-Stokes photoluminescence (PL) is light emission at a higher photon energy than the excitation, with applications in optical cooling, bioimaging, lasing, and quantum optics. Here, we show how plasmonic nano-cavities activate anti-Stokes…

Developments in optoelectronics and spin-optronics based on transition metal dichalcogenide monolayers (MLs) need materials with efficient optical emission and well-defined transition energies. In as-exfoliated MoS2 MLs the…

Strongly quantum-confined 2D colloidal PbS nanoplatelets (NPLs) are highly interesting materials for near-infrared optoelectronic applications. Here, we use ultrafast transient optical absorption spectroscopy to study the characteristics…

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