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相关论文: Dynamics of excitons in CdSe nanoplatelets

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We show how to calculate the optical functions of a nanoplatelet, taking into account the effect of a dielectric confinement on excitonic states. Real density matrix approach is employed to obtain analytical and semi-analytical relations…

We investigated the nonlinear optical properties of CdSe/CdS nanoplatelets in the vicinity of heavy hole and light hole exciton resonances. The two color pump-probe technique was applied. The first intense pulse created non-equilibrium…

We show that the finite lateral sizes of ultrathin CdSe nanoplatelets strongly affect both their photoluminescence and optical absorption spectra. This is in contrast to the situation in quantum wells, in which the large lateral sizes may…

We experimentally investigated for the first time the lowest four band structure of Cd Se nanoplatelets at the r point of Brillouin zone [heavy-hole (hh), light-hole (lh) and two spin-orbital bands] and its modification due to the changing…

We calculate the optical properties of a series of passivated non-stoichiometric CdSe clusters using two first-principles approaches: time-dependent density functional theory within the local density approximation, and by solving the…

材料科学 · 物理学 2007-05-23 Marie Lopez del Puerto , Murilo L. Tiago , James R. Chelikowsky

The optical spectra of CdSe nanocrystals up to 55 A in diameter are analyzed in a wide range of energies from the fine structure of the low-energy excitations to the so-called high-energy transitions. We apply a symmetry-based method in two…

介观与纳米尺度物理 · 物理学 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee

We report on the experimental and theoretical studies of optical alignment and optical orientation effects in an ensemble of core/shell CdSe/CdS colloidal nanoplatelets. The dependences of three Stokes parameters on the magnetic field…

We report excited state emission from p-states at excitation fluences well below ground state saturation in CdSe nanoplatelets. Size dependent exciton ground state-excited state energies and dynamics are determined by three independent…

The picosecond dynamics of excitons in colloidal CdSe nanorods are directly measured via their 1s to 2p-like internal transitions by ultra-broadband terahertz spectroscopy. Broadened absorption peaks from both the longitudinal and…

介观与纳米尺度物理 · 物理学 2015-06-17 David G. Cooke , Peter Uhd Jepsen , Jun Yan Lek , Yeng Ming Lam , Fredrik Sy , Marc M. Dignam

CdSe nanoplatelets show perfectly quantized thicknesses of few monolayers. They present a situation of extreme, yet well defined quantum confinement. Due to large dielectric contrast between the semiconductor and its ligand environment,…

We study the band-edge exciton fine structure and in particular its bright-dark splitting in colloidal semiconductor nanocrystals by four different optical methods based on fluorescence line narrowing and time-resolved measurements at…

Two-dimensional electron-hole gases in colloidal semiconductors have a wide variety of applications. Therefore, a proper physical understanding of these materials is of great importance. In this paper we present a detailed theoretical…

介观与纳米尺度物理 · 物理学 2019-12-18 F. García Flórez , Aditya Kulkarni , Laurens D. A. Siebbeles , H. T. C. Stoof

Luminescent colloidal CdSe nanorings are a new type of semiconductor structure that have attracted interest due to the potential for unique physics arising from their non-trivial toroidal shape. However, the exciton properties and dynamics…

Semiconductor nanoplatelets possess exceptional optical properties that make them promising candidates for next-generation optoelectronic applications. However, unlike quantum dots where absorption spectroscopy alone can determine both size…

Quantum Stark effect in semiconductor nanocrystals is theoretically investigated, using the effective mass formalism within a $4\times 4$ Baldereschi-Lipari Hamiltonian model for the hole states. General expressions are reported for the…

材料科学 · 物理学 2009-11-10 Eduardo Ariel Menendez Proupin , Carlos Trallero Giner

We present the phase diagram of free charges (electrons and holes), excitons, and biexcitons in highly excited CdSe nanoplatelets that predicts a crossover to a biexciton-dominated region at easily attainable low temperatures or high…

介观与纳米尺度物理 · 物理学 2020-09-16 F. García Flórez , Laurens D. A. Siebbeles , H. T. C. Stoof

Theory of electronic and optical properties of exciton and bi-exciton complexes confined in CdSe spherical nanocrystals is presented. The electron and hole states are computed using atomistic $sp^3d^5s^*$ tight binding Hamiltonian including…

介观与纳米尺度物理 · 物理学 2015-05-20 Marek Korkusinski , Oleksandr Voznyy , Pawel Hawrylak

We address spin properties and spin dynamics of carriers and charged excitons in CdSe/CdS colloidal nanoplatelets with thick shells. Magneto-optical studies are performed by time-resolved and polarization-resolved photoluminescence,…

The optoelectronic properties of metal chalcogenide colloidal nanoplatelets are often interpreted in terms of excitonic states. However, recent spectroscopic experiments evidence the presence of trion states, enabled by the slow Auger…

介观与纳米尺度物理 · 物理学 2021-05-06 David F. Macías-Pinilla , Josep Planelles , Iván Mora-Seró , Juan I. Climente

By performing spectroscopic single-particle measurements at cryogenic temperatures over the course of hours we study %By performing spectroscopic longtime single-particle measurements at cryogenic temperatures we study both the spectral…

介观与纳米尺度物理 · 物理学 2017-11-13 Sven-Hendrik Lohmann , Christian Strelow , Alf Mews , Tobias Kipp
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