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Pumping n-type GaAs and InSb with ultrafast THz pulses having intensities higher than 150 MW/cm2 shows strong free carrier absorption saturation at temperatures of 300 K and 200 K respectively. If the energy imparted to the carriers exceeds…

材料科学 · 物理学 2009-06-17 Matthias C. Hoffmann , Janos Hebling , Harold Y. Hwang , Ka-Lo Yeh , Keith A. Nelson

Black phosphorus is a very promising material for telecommunication due to its direct bandgap and strong resonant absorption in near-infrared wavelength range. However, ultrafast nonlinear photonic applications relying on the ultrafast…

Ultrafast coherent control of electric dipoles using strong terahertz (THz) pulses provides a means to discover hidden phases of materials and potentially leads to applications in high-speed electro-optic devices. The effectiveness of this…

材料科学 · 物理学 2025-04-25 Wei Li , Sixu Wang , Pai Peng , Haojie Han , Xinbo Wang , Jing Ma , Jianlin Luo , Jun-Ming Liu , Jing-Feng Li , Ce-Wen Nan , Qian Li

The terahertz (THz) spectral domain offers a myriad of applications spanning chemical spectroscopy, medicine, security and imaging[1]. It has also recently become a playground for fundamental studies of light-matter interactions [2-6]. THz…

We investigate the role of polarization-photon coupling (specifically, polarization-oscillation-induced radiation electric field) in the excitation of ferroelectric thin films by an ultrafast terahertz (THz) electric-field pulse. Analytical…

应用物理 · 物理学 2022-07-21 Shihao Zhuang , Jia-Mian Hu

Black phosphorus (BP) has recently emerged as an alternative 2D semiconductor owing to its fascinating electronic properties such as tunable bandgap and high charge carrier mobility. The structural investigation of few-layer BP, such as…

介观与纳米尺度物理 · 物理学 2017-02-01 Yangjin Lee , Jun-Yeong Yoon , Declan Scullion , Jeongsu Jang , Elton J G Santos , Hu Young Jeong , Kwanpyo Kim

Topological phase transitions occur when the electronic bands change their topological properties, typically featuring the closing of the bandgap. While the influence of topological phase transitions on electronic and optical properties has…

材料科学 · 物理学 2021-01-04 Shengying Yue , Bowen Deng , Yanming Liu , Yujie Quan , Runqing Yang , Bolin Liao

Owing to its outstanding electronic properties, black phosphorus (BP) is considered as a promising material for next-generation optoelectronic devices. In this work, devices based on BP/MXene (Zrn+1CnT2, T = O, F, OH, n = 1, 2) van der…

材料科学 · 物理学 2018-02-13 Hao Yuan , Zhenyu Li

We study the environmental instability of mechanically exfoliated few-layer black phosphorus (BP). From continuous measurements of flake topography over several days, we observe an increase of over 200% in volume due to the condensation of…

Liquid crystal based technologies have found considerably diversified uses and areas of application over the last few decades, proving to be excellent materials for tunable optical elements from visible to near-infrared frequencies.…

化学物理 · 物理学 2023-10-25 Patrick Friebel , Daria Ruth Galimberti , Matteo Savoini , Laura Cattaneo

Through infrared spectroscopy, we systematically study the pressure effect on electronic structures of few-layer black phosphorus (BP) with layer number ranging from 2 to 13. We reveal that the pressure-induced shift of optical transitions…

In time-resolved pump-probe vibrational spectroscopy the internal stretch mode of polar molecules is utilized as a key observable to characterize the ultrafast dynamics of adsorbates on surfaces. The adsorbates non-adiabatic intermode…

材料科学 · 物理学 2023-03-13 Raúl Bombín , Alberto S. Muzas , Dino Novko , J. Iñaki Juaristi , Maite Alducin

Ultrafast atomic vibrations mediate heat transport, serve as fingerprints for chemical bonds and drive phase transitions in condensed matter systems. Light pulses shorter than the atomic oscillation period can not only probe, but even…

光学 · 物理学 2021-04-06 Alexandra Voelkel , Georg Herink

Trilayer graphene in both ABA (Bernal) and ABC (rhombohedral) stacking sequences is shown to exhibit intense infrared absorption from in-plane optical phonons. The feature, lying at ~1580 cm-1, changes strongly with electrostatic gating.…

介观与纳米尺度物理 · 物理学 2013-05-03 Chun Hung Lui , Emmanuele Cappelluti , Zhiqiang Li , Tony F. Heinz

The unique optoelectronic properties of single layer graphene (SLG) are ideal for the development of photonic devices across a broad range of frequencies, from X-rays to microwaves. In the terahertz (THz) range (0.1-10 THz frequency) this…

A promising route for the development of opto-elelctronic technology is to use terahertz radiation to modulate the optical properties of semiconductors. Here we demonstrate the dynamical control of photoluminescence (PL) emission in…

High absorption in a wide frequency band has attracted considerable interest since their potential applications in frequency spectrum imaging systems and anti-radar cloaking. In this paper, a polarization-independent, ultra-broadband and…

光学 · 物理学 2014-09-23 Cheng Shi , XiaoFei Zang , XueBin Ji , Lin Chen , Bin Cai , YiMing Zhu

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~…

强关联电子 · 物理学 2015-05-28 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , G. Karapetrov , R. Hott , R. Heid , K. -P. Bohnen , A. Alatas

Terahertz (THz) fields are widely applied for sensing, communication and quality control. In future applications, they could be efficiently confined, enhanced and manipulated - well below the classical diffraction limit - through the…

Terahertz scanning near-field optical microscope (THz-SNOM) is employed to measure ultrafast evolution of THz conductivity spectra after photoexcitation of GaAs and InP wafers using ultrashort laser pulses. Unlike in GaAs, the THz…

介观与纳米尺度物理 · 物理学 2025-01-22 Tinkara Troha , Arvind Singh , Petr Kužel , Hynek Němec