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We demonstrate computationally the existence of magnetoelectric multipoles, arising from the second order term in the multipole expansion of a magnetization density in a magnetic field, in noncentrosymmetric magnetic metals. While…

材料科学 · 物理学 2021-03-09 Florian Thöle , Nicola A. Spaldin

We show by means of ab-initio calculations that the organic molecular crystal TTF-CA is multiferroic: it has an instability to develop spontaneously both ferroelectric and magnetic ordering. Ferroelectricity is driven by a Peierls…

Multiferroic materials exhibit the coexistence of magnetic and electric order. They are at the forefront of modern condensed matter physics due to their potential applications in next-generation technologies such as data storage, sensors,…

强关联电子 · 物理学 2025-09-15 Daniel C. Cabra , Gerardo L. Rossini

Topological defects in ordered states with spontaneously broken symmetry often have unusual physical properties, such as fractional electric charge or a quantised magnetic field-flux, originating from their non-trivial topology. Coupled…

强关联电子 · 物理学 2025-06-10 Sergey Artyukhin , Kris T. Delaney , Nicola A. Spaldin , Maxim Mostovoy

Four types of atomic-scale multipoles, electric, magnetic, magnetic toroidal, and electric toroidal multipoles, give a complete set to describe arbitrary degrees of freedom for coupled charge, spin, and orbital of electrons. We here present…

强关联电子 · 物理学 2018-10-24 Satoru Hayami , Megumi Yatsushiro , Yuki Yanagi , Hiroaki Kusunose

In this paper we study magnetoelectric effects in two-dimensional magnetic bilayers and introduce the notion of a layer dipole magnetoelectric polarizability. This magnetoelectric polarizability describes the magnetization response to an…

强关联电子 · 物理学 2025-12-08 H. Radhakrishnan , C. Ortix , J. W. F. Venderbos

Ferroelectric Ising chain magnet Ca$_3$Co$_{2-x}$Mn$_x$O$_6$ ($x\simeq$0.96) was studied in magnetic fields up to 33 T. Magnetization and neutron scattering measurements reveal successive metamagnetic transitions from the zero-field…

强关联电子 · 物理学 2009-11-13 Y. J. Jo , Seongsu Lee , E. S. Choi , H. T. Yi , W. Ratcliff , Y. J. Choi , V. Kiryukhin , S. W. Cheong , L. Balicas

Multiferroic particulate composites have been fabricated by taking the morphotropic phase boundary composition of ferroelectric phase Bi(Ni1/2Ti1/2)O3-PbTiO3 and magnetic phase (Ni,Zn)Fe2O4. The ferroelectric phase has coexisting monoclinic…

材料科学 · 物理学 2018-08-06 Rishikesh Pandey , Uma Shankar , Sher Singh Meena , Akhilesh Kumar Singh

We present a simple two-dimensional model in which the lattice degrees of freedom mediate the interactions between magnetic moments and electric dipoles. This model reproduces basic features, such as a sudden electric polarization…

强关联电子 · 物理学 2022-04-06 L. Pili , R. A. Borzi , D. C. Cabra , S. A. Grigera

Magneto-electric multiferroics exemplified by TbMnO3 possess both magnetic and ferroelectric long-range order. The magnetic order is mostly understood, whereas the nature of the ferroelectricity has remained more elusive. Competing models…

First-principles calculations, in combination with the four-state energy mapping method, are performed to extract the magnetic interaction parameters of multiferroic BiFeO$_3$. Such parameters include the symmetric exchange (SE) couplings…

材料科学 · 物理学 2019-03-20 Changsong Xu , Bin Xu , Bertrand Dupé , L. Bellaiche

Competing interactions and geometric frustration provide favourable conditions for exotic states of matter. Such competition often causes multiple phase transitions as a function of temperature and can lead to magnetic structures that break…

Single crystals of Cu$_3$Bi(SeO$_3$)$_2$O$_2$Cl were investigated using high-resolution capacitance dilatometry in magnetic fields up to 15 T. Pronounced magnetoelastic coupling is found upon evolution of long-range antiferromagnetic order…

强关联电子 · 物理学 2022-05-10 S. Spachmann , P. Berdonosov , M. Markina , A. Vasiliev , R. Klingeler

Multiferroics with coexistent ferroelectric and magnetic orders can provide an interesting laboratory to test unprecedented magnetoelectric responses and their possible applications. One such example is the dynamical and/or resonant…

强关联电子 · 物理学 2015-05-27 Y. Tokura , N. Kida

Ferroic magnetic quadrupole order exhibiting macroscopic magnetoelectric activity is discovered in the novel compound $A$(TiO)Cu$_4$(PO$_4$)$_4$ with $A$ = Pb, which is in contrast with antiferroic quadrupole order observed in the…

材料科学 · 物理学 2018-04-19 K. Kimura , M. Toyoda , P. Babkevich , K. Yamauchi , M. Sera , V. Nassif , H. M. Rønnow , T. Kimura

The ferroelectricity of multiferroics induced by spin order is commonly explained by considering either purely electronic or ion-displacement contribution. However, there is no general model which includes both effects simultaneously. Here,…

强关联电子 · 物理学 2014-10-01 H. J. Xiang , P. S. Wang , M. -H. Whangbo , X. G. Gong

Recent data reported on the magneto-electric coupling,{\alpha}, of hexaferrite materials is very high, and they have the potential to impact future technologies in a major way. The fundamental question addressed in this paper is what does…

材料科学 · 物理学 2014-04-23 Carmine Vittoriaa , Somu Sivasubramanianb , Allan Widomc

We use the microscopic weak coupling theory to predict the pairing state in superconductors of cubic, hexagonal, or tetragonal symmetry, where the order parameter is multicomponent, i.e., transforms according to either a 2-dimensional or a…

超导电性 · 物理学 2009-11-11 V Kuznetsova , V. Barzykin

Type-II multiferroics, in which the magnetic order breaks inversion symmetry, are appealing for both fundamental and applied research due their intrinsic coupling between magnetic and electrical orders. Using first-principles calculations…

材料科学 · 物理学 2023-11-20 Urmimala Dey , Mark S. Senn , Nicholas C. Bristowe

The phenomenological theory of ferroelectricity in spiral magnets presented in [M. Mostovoy, Phys. Rev. Lett. 96, 067601 (2006)] is generalized to describe consistently states with both uniform and modulated-in-space ferroelectric…

材料科学 · 物理学 2009-11-13 A. Cano , E. I. Kats