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Theoretical considerations are made for the nuclear excitation from the ground state to the 8 eV $^{229m}$Th isomer via near-resonant electron transitions in Sb-like ($q=39+$) thorium ions. The energy of the first excited atomic state…

原子物理 · 物理学 2025-04-17 Karol Kozioł , Jacek Rzadkiewicz

We use advanced computational techniques to study the electronic structure of the Hf$^{12+}$ ion, with the goal of assessing its potential for use in highly accurate atomic optical clocks and search for new physics. Such clocks should…

原子物理 · 物理学 2025-11-04 Saleh O. Allehabi , V. A. Dzuba , V. V. Flambaum

We calculate hyperfine structure of $^{229}$Th and its ions (Th~IV, Th~III, Th~II, Th~I) to reveal the dependence of the nuclear clock frequency on the hyperfine interaction (hfi). We calculate first and second-order hfi shifts and…

原子物理 · 物理学 2023-12-18 V. A. Dzuba , V. V. Flambaum

The $^{229}$Th nucleus has a unique transition at only 8 eV which could be used for a novel nuclear clock. We investigate theoretically the prospects of driving this transition with vortex light beams carrying orbital angular momentum.…

原子物理 · 物理学 2024-04-22 Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy

The 7.6-eV-isomer of Thorium-229 offers the opportunity to perform high resolution laser spectroscopy of a nuclear transition. We give a brief review of the investigations of this isomer. The nuclear resonance connecting ground state and…

光学 · 物理学 2017-08-23 E. Peik , K. Zimmermann , M. Okhapkin , Chr. Tamm

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

核实验 · 物理学 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

We have considered an effect of atomic electrons due to the electronic bridge process on the nuclear $^{229m}$Th -- $^{229g}$Th transition in ^{229}$Th$^{3+}$. Based on a recent experimental result we assumed the energy difference between…

原子物理 · 物理学 2010-04-29 S. G. Porsev , V. V. Flambaum

Iridium ions near $4f$-$5s$ level crossings are the leading candidates for a new type of atomic clocks with a high projected accuracy and a very high sensitivity to the temporal variation of the fine structure constant $\alpha$. To identify…

原子物理 · 物理学 2015-08-12 U. I. Safronova , V. V. Flambaum , M. S. Safronova

We identify Ba$^{4+}$ (Te-like) as a promising candidate for a high-accuracy optical clock. The lowest-lying electronic states are part of a $^3P_J$ fine structure manifold with anomalous energy ordering, being non-monotonic in $J$. We…

原子物理 · 物理学 2020-10-26 Kyle Beloy , Vladimir A. Dzuba , Samuel M. Brewer

The $^{229}\text{Th}$ isotope is a promising candidate for nuclear clocks, with its transition frequency influenced by electron-induced nuclear frequency shifts. This effect is comparatively small and requires high-precision theoretical…

原子物理 · 物理学 2025-05-09 Ran Si , Chaofan Shi , Nan Xue , Xiangjin Kong , Chongyang Chen , Bingsheng Tu , Yu-Gang Ma

Electronic bridge excitation of the 76 eV nuclear isomeric state in $^{235}$U is shown to be strongly enhanced in the U$^{7+}$ ion, potentially enabling laser excitation of this nucleus. This is because the electronic spectrum has a very…

原子物理 · 物理学 2019-01-08 J. C. Berengut

$^{229}$Th, a crucial candidate for nuclear clocks and many other applications, is a typical heavy nucleus with an extremely low-energy isomeric state $^{229m}$Th. A detailed study of the nuclear structure of $^{229}$Th is performed here by…

核理论 · 物理学 2025-08-28 Zi-Rui Chen , Long-Jun Wang , Yuanbin Wu

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

We examine energy level-crossings of fine-structure (FS) levels in the heavier highly charged ions (HCIs) with $d^6$ and $d^8$ configurations. From the analysis, we find that some of these HCIs are tailor-made for atomic clocks with quality…

原子物理 · 物理学 2023-07-28 Yan-mei Yu , B. K. Sahoo

Thorium-229 is a unique case in nuclear physics: it presents a metastable first excited state Th-229m, just a few electronvolts above the nuclear ground state. This so-called isomer is accessible by VUV lasers, which allows transferring the…

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of $^{229}{\mathrm Th}$. Due to the very low transition energy, the $^{229}{\mathrm…

原子物理 · 物理学 2017-03-22 Pavlo V. Bilous , Georgy A. Kazakov , Iain D. Moore , Thorsten Schumm , Adriana Pálffy

The low-energy isomeric transition in Thorium-229 offers a unique interface between nuclear and atomic physics, presenting a resource for quantum technologies that is notably resilient to environmental decoherence. While early experiments…

量子物理 · 物理学 2025-08-15 Jingbo Wang , Haixing Miao , Shiqian Ding , Dong E. Liu

Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider…

原子物理 · 物理学 2015-06-11 V. A. Dzuba , A. Derevianko , V. V. Flambaum

Level crossings in the ground state of ions occur when the nuclear charge Z and ion charge Z_ion are varied along an isoelectronic sequence until the two outermost shells are nearly degenerate. We examine all available level crossings in…

原子物理 · 物理学 2012-09-11 J. C. Berengut , V. A. Dzuba , V. V. Flambaum , A. Ong

There exist in nature a few nuclear isomers with very low (eV) excitation energies, and the combination of low energy and narrow width makes them possible candidates for laser-based investigations. The best candidate is the lowest-energy…

核理论 · 物理学 2008-11-26 A. C. Hayes , J. L. Friar