相关论文: Nanocavities for Molecular Optomechanics: their fu…
Cavity optomechanics allows the characterization of a vibration mode, its cooling and quantum manipulation using electromagnetic fields. Regarding nanomechanical as well as electronic properties, single wall carbon nanotubes are a…
Confining a laser field between two high reflectivity mirrors of a high-finesse cavity can increase the probability of a given cavity photon to be scattered by an atom traversing the confined photon mode. This enhanced coupling between…
A theoretical model of resonant hyper-Raman scattering by an ensemble of spherical semiconductor quantum dots has been developed. The electronic intermediate states are described as Wannier-Mott excitons in the framework of the envelope…
Bulk glass formation occurs over a very small part of phase space, and "good" glasses (which form even at low quench rates ~ 10K/sec) select an even smaller part of that accessible phase space. An axiomatic theory provides the physical…
We report on the experimental observation of beaming elastic and surface enhanced Raman scattering (SERS) emission from a bent-nanowire on a mirror (B-NWoM) cavity. The system was probed with polarization resolved Fourier plane and…
In the last few decades, the development of miniature biological sensors that can detect and measure different phenomena at the nanoscale has led to transformative disease diagnosis and treatment techniques. Among others, biofunctional…
Raman-gain-enhanced near-field optomechanical transduction between a movable optical cavity and SiN-membrane resonator is demonstrated. The Raman gain compensates for the intrinsic loss of the cavity and amplifies the optomechanical…
Molecular cavity optomechanical systems, featuring ultrahigh vibrational frequencies and strong light-matter interactions, hold significant promise for advancing applications in quantum science and technology. Specifically, by introducing…
Molecular cavity optomechanics (COM), characterized by remarkably efficient optomechanical coupling enabled by a highly localized light field and ultra-small effective mode volume, holds significant promise for advancing applications in…
Strong coupling between cavity photons and molecular vibrations can lead to the formation of vibron-polaritons. In a recent experiment with PVAc molecules in a metal-metal microcavity [A.Shalabney et al., Ang.Chem.Int.Ed. 54 7971 (2015)],…
Cavity optomechanical systems have become a popular playground for studies of controllable nonlinear interactions between light and motion. Owing to the large speed of light, realizing cavity optomechanics in the microwave frequency range…
We study an optomechanical system in which the mechanical motion of a single trapped ion is coupled to a cavity field for the realization of a strongly quantum correlated two-mode system. We show that for large pump intensities the steady…
We propose a molecular optomechanical platform to generate robust entanglement among bosonic modes-photons, phonons, and plasmons-under ambient conditions. The system integrates an ultrahigh-Q whispering-gallery-mode (WGM) optical resonator…
The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…
Light scattering is one of the most established wave phenomena in optics, lying at the heart of light-matter interactions and of crucial importance for nanophotonic applications. Passivity, causality and energy conservation imply strict…
The optomechanical character of molecules was discovered by Raman about one century ago. Today, molecules are promising contenders for high-performance quantum optomechanical platforms because their small size and large energy-level…
Molecules are the most demanding quantum systems to be simulated by quantum computers because of their complexity and the emergent role of quantum nature. The recent theoretical proposal of Huh et al. (Nature Photon., 9, 615 (2015)) showed…
The strong spatial confinement of a nanocavity plasmonic field has made it possible to visualize the inner structure of a single molecule and even to distinguish its vibrational modes in real space. With such ever-improved spatial…
Metallic nanoparticle-on-a-mirror (NPoM) cavities enable extreme field confinement in sub-nm gaps, leading to unrivaled performance for nonlinear processes such as surface-enhanced Raman scattering (SERS). So far, prevailing experimental…
Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…