相关论文: Nanocavities for Molecular Optomechanics: their fu…
In many experiments isolated atoms and ions have been inserted into high-finesse optical resonators for the study of fundamental quantum optics and quantum information. Here, we introduce another application of such a system, as the…
In this work we identify coherent electron-vibron interactions between near-resonant and non-resonant electronic levels that contribute beyond standard optomechanical models for off-resonant or resonance SERS. By developing an open-system…
In a canonical optomechanical system, mechanical vibrations are dynamically encoded on an optical probe field which reciprocally exerts a backaction force. Due to the weak single photon coupling strength achieved with macroscopic…
In this study, we apply the monitoring master equation describing decoherence of internal states to an optically active molecule prepared in a coherent superposition of nondegenerate internal states interacting with thermal photons at low…
The interaction of organic molecules and molecular aggregates with electromagnetic fields that are strongly confined inside optical cavities within nanoscale volumes, has allowed the observation of exotic quantum regimes of light-matter…
Observation of quantum phenomena in cryogenic, optically cooled mechanical resonators has been recently achieved by a few experiments based on cavity optomechanics. A well-established experimental platform is based on a thin film…
Herein we report experimental evidence of directional SERS from molecules situated inside a single nanowire-nanoparticle junction cavity. The emission was confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In…
Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered…
Optically measuring in the photon counting regime is a recurrent challenge in modern physics and a guarantee to develop weakly invasive probes. Here we investigate this idea on a hybrid nano-optomechanical system composed of a nanowire…
Cavity optomechanics explores the coupling between the optical field and the mechanical oscillation to induce cooling and regenerative oscillation in a mechanical oscillator. So far, optomechanics relies on the detuning between the cavity…
Frequency upconversion is a cornerstone of electromagnetic signal processing, analysis and detection. It is used to transfer energy and information from one frequency domain to another where transmission, modulation or detection is…
We show a break down of the conventional partition of optical states into its radiative and non-radiative parts. Large divergence of experimental observations from current theory in the case of emitters interacting with fully absorbing…
We investigate how proximity to a metal nanostructure, particularly to a flat mirror or a cavity confined between two mirrors, affects the vibronic structure of Raman scattering signals. We find that such proximity, particularly for the…
Molecular self-assembly, the function of biomembranes, and the performance of organic solar cells rely on molecular interactions on the nanoscale. The understanding and design of such intrinsic or engineered heterogeneous functional soft…
We investigate the optomechanical photon-phonon coupling of a single light mode propagating through an array of vibrating mechanical elements. As recently shown for the particular case of a periodic array of membranes embedded in a…
We propose and analyze a nanomechanical architecture where light is used to perform linear quantum operations on a set of many vibrational modes. Suitable amplitude modulation of a single laser beam is shown to generate squeezing,…
In an optomechanical setup, the coupling between cavity and resonator can be increased by tuning them to the same frequency. We study this interaction between a carbon nanotube resonator and a radio-frequency circuit. In this resonant…
In the field of cavity nano-optomechanics, the nanoresonator-in-the-middle approach consists in inserting a sub-wavelength sized deformable resonator, here a nanowire, in the small mode volume of a fiber microcavity. Internal resonances in…
Plasmonic molecular nanojunctions exhibit opto-mechanical coupling at the nanoscale, enabling intertwined optical, vibrational and electronic phenomena. Here, we demonstrate plasmon-mediated phonon pumping, driven by inelastic electron…
In the past decade, advances in nanotechnology have led to the development of plasmonic nanocavities which facilitate light-matter strong coupling in ambient conditions. The most robust example is the nanoparticle-on-mirror (NPoM) structure…