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We report a single-ion optical clock based on the 4S_1/2-3D_5/2 transition of the 40Ca+ ion, operated in a liquid nitrogen cryogenic environment,achieving a total systematic uncertainty of 4.4E-19. We employ a refined temperature evaluation…

We perform quantum logic spectroscopy with a $^{27}$Al$^{+}$/$^{40}$Ca$^{+}$ mixed ion crystal in a linear Paul trap for a measurement of the $(3s^{2})\,^{1}\mathrm{S}_{0} \leftrightarrow \, (3s3p)\,^{3}\mathrm{P}_{1}, F=7/2$…

We present an experimental investigation of the Rydberg 23 P$_{1/2}$ state of laser-cooled $^{40}$Ca$^+$ ions in a radiofrequency ion trap. Using micromotion sideband spectroscopy on a narrow quadrupole transition, the oscillating electric…

Appraising the projected $10^{-18}$ fractional uncertainty in the optical frequency standards using singly ionized ions, we estimate the black-body radiation (BBR) shifts due to the magnetic dipole (M1) and electric quadrupole (E2)…

原子物理 · 物理学 2015-05-30 Bindiya Arora , D. K. Nandy , B. K. Sahoo

We have measured transition frequencies, isotope shifts and hyperfine structure splittings in the $3 d^{2}\left({ }^{3\!}F\right) 4 s\,{ }^{4} F_J\rightarrow 3 d^{2}\left({ }^{3\!} F\right) 4 p \,^{4} G_{J+1}$ transitions in Ti$^+$ ions for…

High-precision quasi-simultaneous collinear/anticollinear laser spectroscopy was performed to measure the $5s$ $^2S_{1/2}\rightarrow 5p$ $^2P_{1/2}$ (D1), the $5s$ $^2S_{1/2}\rightarrow 5p$ $^2P_{3/2}$ (D2), and the three $4d\rightarrow 5p$…

Extra-laboratory atomic clocks are necessary for a wide array of applications (e.g. satellite-based navigation and communication). Building upon existing vapor cell and laser technologies, we describe an optical atomic clock, designed…

At optical frequencies, interactions of the electric field component of light with matter are dominating, whereas magnetic dipole transitions are inherently weak and challenging to access independently from electric dipole transitions.…

Electrometry is performed using Rydberg states to evaluate the quadratic Stark shift of the $5s^2$ $^1\textrm{S}_0-5s5p$ $^3\textrm{P}_0$ clock transition in strontium. By measuring the Stark shift of the highly excited…

Isotope shifts in dielectronic recombination spectra were studied for Li-like ^{A}Nd^{57+} ions with A=142 and A=150. From the displacement of resonance positions energy shifts \delta E^{142,150}(2s-2p_1/2)= 40.2(3)(6) meV (stat)(sys)) and…

The finite field calculations are performed for two heavy frequency-standard candidates In$^+$ and Sr. The progressive hierarchy of electron correlations is implemented by the relativistic coupled-cluster and configuration interaction…

原子物理 · 物理学 2015-12-09 Yan-mei Yu , Bing-bing Suo , Hui-hui Feng , Heng Fan , Wu-Ming Liu

Vibrational overtones in deeply bound molecules are sensitive probes for variation of the proton-to-electron mass ratio $\mu$. In nonpolar molecules, these overtones may be driven as two-photon transitions. Here, we present procedures for…

原子物理 · 物理学 2019-01-03 Ryan Carollo , Alexander Frenett , David Hanneke

We present the observations of x-rays emitted from the $1s2s^{2}2p_{1/2}2p_{3/2}$ inner shell excited state of B-like W and Bi ions. The relative transition rates are obtained for two dominant radiative transitions to $1s^{2}2s^{2}2p_{1/2}$…

We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

强关联电子 · 物理学 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

Future transportable optical clocks require compact and reliable light sources. Here, broadband, unpolarized repumper and state clearout sources for Sr+ single-ion optical clocks are reported. These turn-key devices require no frequency…

原子物理 · 物理学 2015-04-20 T. Fordell , T. Lindvall , P. Dubé , A. A. Madej , A. E. Wallin , M. Merimaa

We report results regarding the electron transport in vertical quasi-2D layered 1T-TaS2 charge-density-wave devices. The low-frequency noise spectroscopy was used as a tool to study changes in the cross-plane electrical characteristics of…

To support efforts on cooling and trapping of alkaline-earth atoms and designs of atomic clocks, we performed ab initio relativistic many-body calculations of electric-dipole transition amplitudes between low-lying states of Mg, Ca, and Sr.…

原子物理 · 物理学 2009-11-07 S. G. Porsev , M. G. Kozlov , Yu. G. Rakhlina , A. Derevianko

The possibility of using neutral and double ionized erbium for atomic clocks of high precision is investigated. In both cases the narrow electric quadrupole clock transition between the ground and first exited state of the same…

原子物理 · 物理学 2015-06-16 A. Kozlov , V. A. Dzuba , V. V. Flambaum

The recent detections of electric-quadrupole (E2) transitions in water vapor and magnetic-dipole (M1) transitions in carbon dioxide have opened a new field in molecular spectroscopy. While in their present status, the spectroscopic…

化学物理 · 物理学 2022-07-27 Hélène Fleurbaey , Roberto Grilli , Didier Mondelain , Samir Kassi , Alain Campargue

Doppler cooling of calcium ions has been experimentally demonstrated using the S1/2 to D5/2 dipole-forbidden transition. Scattering forces and fluorescence levels a factor of 5 smaller than for usual Doppler cooling on the dipole allowed…

量子物理 · 物理学 2009-11-13 R. J. Hendricks , J. L. Sørensen , C. Champenois , M. Knoop , M. Drewsen