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In stimulated Raman scattering, two incident optical waves induce a force oscillating at the difference of the two light frequencies. This process has enabled important applications such as the excitation and coherent control of phonons and…

材料科学 · 物理学 2017-09-27 Sebastian Maehrlein , Alexander Paarmann , Martin Wolf , Tobias Kampfrath

Achieving parametric excitation in an oscillating physical system involves periodically adjusting one of its parameters to modulate the oscillator's natural frequency. This phenomenon has been observed in numerous systems within physics and…

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

We investigate the out-of-equilibrium lattice dynamics in the spin-ladder system $\alpha'$-NaV$_2$O$_5$ using intense terahertz (THz) pump and near-infrared (NIR) probe spectroscopy. When quasi-single-cycle THz pulses interact with…

Coherent phonons describe the collective, ultrafast motion of atoms and play a central role in light-induced structural dynamics. Here, we employ terahertz scanning tunneling microscopy (THz-STM) to excite and detect coherent phonons in…

Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…

介观与纳米尺度物理 · 物理学 2021-11-29 Ziqi Li , Bo Peng , Miao-Ling Lin , Yu-Chen Leng , Bin Zhang , Chi Pang , Ping-Heng Tan , Bartomeu Monserrat , Feng Chen

Ultrafast atomic vibrations mediate heat transport, serve as fingerprints for chemical bonds and drive phase transitions in condensed matter systems. Light pulses shorter than the atomic oscillation period can not only probe, but even…

光学 · 物理学 2021-04-06 Alexandra Voelkel , Georg Herink

The interaction of a single-cycle THz electric field with the topological insulator $\mathrm{MnBi}_2\mathrm{Te}_4$ triggers strongly anharmonic lattice dynamics, promoting fully coherent energy transfer between the otherwise non-interacting…

Density Functional Theory (DFT) calculations not only allow to predict the vibrational and optical properties of solids but also to understand and disentangle the mechanisms playing a key role in the generation of coherent optical phonons.…

材料科学 · 物理学 2025-10-09 A. Levchuk , R. Busselez , G. Vaudel , P. Ruello , V. Juvé , B. Arnaud

Selective excitation of coherent high-amplitude vibrations of atoms in a solid can induce exotic nonequilibrium states, in which the character of interactions between electronic, magnetic and lattice degrees of freedom is considerably…

材料科学 · 物理学 2020-12-08 A. A. Melnikov , Yu. G. Selivanov , S. V. Chekalin

We propose an experimental technique to generate large amplitude coherent phonons with irradiation of THz-rate pump pulses and to study the dynamics of phase transition in GeTe ferroelectrics. When a single pump pulse irradiates the sample…

材料科学 · 物理学 2011-02-01 Muneaki Hase , Masahiro Kitajima , Shin-ichi Nakashima , Kohji Mizoguchi

Excitation of coherent high-frequency magnons (quanta of spin waves) is critical to the development of high-speed magnonic devices. Here we computationally demonstrate the excitation of coherent sub-terahertz (THz) magnons in ferromagnetic…

应用物理 · 物理学 2022-06-22 Shihao Zhuang , Jia-Mian Hu

Advanced magnetic recording paradigms typically use large temperature changes to drive switching which is detrimental to device longevity, hence finding non-thermal routes is crucial for future applications. By employing atomistic…

We report an observation of coherent phonons of $E_g^1$, $E_u^1$, $A_{1g}^1$, and $E_g^2$ symmetry generated in a single-crystal film of $Bi_2Se_3$ by an intense single-cycle THz pulse. The atomic vibrations reveal themselves through…

The advent of high-intensity ultrafast laser pulses has opened new opportunities for controlling and designing quantum materials. In particular, terahertz (THz) pulses can resonantly drive optical phonon modes, enabling dynamic manipulation…

量子物理 · 物理学 2025-12-22 Yulong Qiao , Richard. Matthias Geilhufe

Coherent manipulation of magnetism through the lattice provides unprecedented opportunities for controlling spintronic functionalities on the ultrafast timescale. Such nonthermal control conventionally involves nonlinear excitation of…

Terahertz (THz) spin waves or their quanta, magnons, can be efficiently excited by acoustic phonons because these excitations have similar wavevectors in the THz regime. THz acoustic phonons can be produced using photoacoustic phenomena but…

介观与纳米尺度物理 · 物理学 2024-08-07 Shihao Zhuang , Xufeng Zhang , Yujie Zhu , Nian X. Sun , Chang-Beom Eom , Paul G. Evans , Jia-Mian Hu

We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…

超导电性 · 物理学 2015-05-25 R. Mankowsky , M. Först , T. Loew , J. Porras , B. Keimer , A. Cavalleri

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective…

Nonlinear responses to intense terahertz (THz) fields provide unique insights into complex dynamics of contemporary material systems. However, the interpretation of the obtained data, in particular, distinguishing genuine ionic oscillations…

材料科学 · 物理学 2025-06-13 Chao Shen , Maximilian Frenzel , Sebastian F. Maehrlein , Zhanybek Alpichshev
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