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We present a direct comparison between resonant terahertz (THz) and nonresonant impulsive stimulated Raman scattering (ISRS) excitation of phonon-polaritons in ferroelectric lithium niobate. THz excitation offers advantages of selectively…

材料科学 · 物理学 2017-02-01 Blake S. Dastrup , Jacob R. Hall , Jeremy A. Johnson

We report on the observation of terahertz radiation in a non-centrosymmetric insulating oxide, paratellurite ($\alpha$-TeO$_2$) by irradiation of a femtosecond laser pulse at room temperature. In the power spectrum of the terahertz…

材料科学 · 物理学 2015-06-22 M. Sotome , N. Kida , R. Takeda , H. Okamoto

We study the generation of narrowband terahertz (THz) pulses by stimulated Raman scattering and molecular modulation in hydrogen-filled hybrid hollow-core fibers. Using a judicious combination of materials and transverse structures, this…

光学 · 物理学 2024-07-08 Sebastien Loranger , Foroogh Jafari , Joseba Zubia , David Novoa

We demonstrate dynamic control of the lattice by THz light by exploiting the coupling of phonon modes. The low-energy sliding phonon modes in the spin-ladder system, Sr$_{14}$Cu$_{24}$O$_{41}$, are excited using THz radiation with high…

Direct manipulation of the atomic lattice using intense long-wavelength laser pulses has become a viable approach to create new states of matter in complex materials. Conventionally, a high frequency vibrational mode is driven resonantly by…

Intense, single-cycle terahertz (THz) pulses offer a promising approach for understanding and controlling the properties of a material on an ultrafast time scale. In particular, resonantly exciting phonons leads to a better understanding of…

Time-resolved spectroscopies using intense THz pulses appear as a promising tool to address collective electronic excitations in condensed matter. In particular recent experiments showed the possibility to selectively excite collective…

强关联电子 · 物理学 2019-11-18 Mattia Udina , Tommaso Cea , Lara Benfatto

Laser-driven coherent phonons can act as modulated strain fields and modify the adiabatic ground state topology of quantum materials. Here we use time-dependent first-principles and effective model calculations to simulate the effect of the…

It is found that single-cycle THz electromagnetic fields efficiently excite a GHz spin resonance mode in ferrimagnetic Tm$_3$Fe$_5$O$_{12}$, despite the near absence of GHz spectral components in the exciting THz pulse. By analyzing how the…

External electric fields are highly attractive for dynamical manipulation of excitons in two-dimensional materials. Here, we theoretically study the ionization of excitons in monolayer transition metal dichalcogenides (TMDs) by intense…

材料科学 · 物理学 2022-01-05 Høgni C. Kamban , Thomas G. Pedersen

Tailored light excitation and nonlinear control of lattice vibrations have emerged as powerful strategies to manipulate the properties of quantum materials out of equilibrium. Generalizing the use of coherent phonon-phonon interactions to…

We observe a terahertz radiation from a hydrogen-bonded organic molecular ferroelectric 5,6-dichloro-2-methylbenzimidazole excited by a femtosecond laser pulse at room temperature. The emitted terahertz wave consists of three oscillatory…

材料科学 · 物理学 2018-08-01 M. Sotome , N. Kida , S. Horiuchi , H. Okamoto

We have applied femtosecond pump-probe technique with variable pump wavelength to study coherent lattice dynamics in Bi single crystal. Comparison of the coherent amplitude as a function of pump photon energy for two different in symmetry…

材料科学 · 物理学 2015-05-20 A. A. Melnikov , O. V. Misochko , S. V. Chekalin

Ionic conduction in solids that exceeds 1 mS/cm is predicted to involve coupled phonon-ion interactions in the crystal lattice. Here, we use theory and experiment to measure the possible contribution of coupled phonon-ion hopping modes…

Here, we investigate phonon mode- and electron band-selective electron-phonon couplings in centrosymmetric 1T$'$-MoTe$_2$ using time- and angle-resolved photoemission spectroscopy combined with frequency-domain analysis. Femtosecond…

材料科学 · 物理学 2026-02-24 Carl E. Jensen , Christoph Emeis , Stephan Jauernik , Petra Hein , Fabio Caruso , Michael Bauer

The capability of magnons to hybridize and strongly couple with diverse excitations offers a promising avenue for realizing and controlling emergent properties that hold significant potential for applications in devices, circuits, and…

材料科学 · 物理学 2024-02-22 D. -Q. To , A. Rai , J. M. O. Zide , S. Law , J. Q. Xiao , M. B. Jungfleisch , M. F. Doty

A coherent THz optical lattice mode is triggered by femtosecond laser pulses in the antiferromagnetic van der Waals semiconductor FePS$_3$. The 380 nm thick exfoliated flake was placed on a substrate and laser-driven lattice and spin…

Electrically injected terahertz (THz) radiation sources are extremely appealing given their versatility and miniaturization potential, opening the venue for integrated-circuit THz technology. In this work, we show that coherent THz…

介观与纳米尺度物理 · 物理学 2021-01-27 Pedro Cosme , Hugo Terças

Among its many outstanding properties, graphene supports terahertz surface plasma waves -- sub-wavelength charge density oscillations connected with electromagnetic fields that are tightly localized near the surface[1,2]. When these waves…

A Terahertz (THz) laser with strong strength could excite more than one phonons and induce a transient lattice distortion termed as nonlinear phononics. This process allows dynamic control of various physical properties, including…

材料科学 · 物理学 2024-12-02 Hongyu Chen , Xi Wu , Jiali Yang , Peizhe Tang , Jia Li