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High bias electrical transport characteristics of freely suspended metallic single-walled carbon nanotubes (SWNTs) are investigated at 250-400K in vacuum and various gases. Self-heating is exploited to examine the temperature dependence of…

介观与纳米尺度物理 · 物理学 2007-05-23 David Mann , Eric Pop , Jien Cao , Qian Wang , Kenneth Goodson , Hongjie Dai

Two-photon absorption in indirect gap semiconductors is an frequently encountered, but not well-understood phenomenon. To address this, the Real Density Matrix Approach is applied to describe two-photon absorption in silicon through the…

The recent discovery of semiconducting two-dimensional materials has led to the prediction of a revolution in the field of optoelectronics, driven by the introduction of a series of new components that are just a few atoms thick. Key…

We developed the model of the internal phonon bottleneck to describe the energy exchange between the acoustically soft ultrathin metal film and acoustically rigid substrate. Discriminating phonons in the film into two groups, escaping and…

仪器与探测器 · 物理学 2018-07-24 M. Sidorova , A. Kozorezov , A. Semenov , A. Korneev , G. Chulkova , Yu. Korneeva , M. Mikhailov , A. Devizenko , G. Goltsman

Light emission in atomically thin heterostructures is known to depend on the type of materials, number and stacking sequence of the constituent layers. Here we show that the thickness of a two-dimensional substrate can be crucial in…

Light emission from higher-order correlated excitonic states has been recently reported in hBN-encapsulated monolayer WSe2 and WS2 upon optical excitation. These exciton complexes are found to be bound states of excitons residing in…

介观与纳米尺度物理 · 物理学 2019-04-19 Matthias Paur , Aday J. Molina-Mendoza , Rudolf Bratschitsch , Kenji Watanabe , Takashi Taniguchi , Thomas Mueller

Uniformity in the excitonic spectrum is a key requirement for accessing intrinsic excitonic physics in two-dimensional semiconductors; however, in transition-metal dichalcogenide (TMD) monolayers supported on substrates, exciton energies…

We report a comprehensive study of the two-phonon inter-valley (2D) Raman mode in graphene monolayers, motivated by recent reports of asymmetric 2D-mode lineshapes in freestanding graphene. For photon energies in the range $1.53 \rm eV -…

介观与纳米尺度物理 · 物理学 2014-06-26 Stéphane Berciaud , Xianglong Li , Han Htoon , Louis E. Brus , Stephen K. Doorn , Tony F. Heinz

Monolayer transition metal dichalcogenides (TMDs) support robust excitons in the visible to near-infrared spectral range. Their reduced dielectric screening results in large binding energies, and combined with a direct bandgap in monolayer…

We propose and design photonic crystal cavities (PCCs) in hexagonal boron nitride (hBN) for diverse photonic and quantum applications. Two dimensional (2D) hBN flakes contain quantum emitters which are ultra-bright and photostable at room…

应用物理 · 物理学 2017-09-12 Sejeong Kim , Milos Toth , Igor Aharonovich

Transition metal dichalcogenide monolayers and heterostructures are highly tunable material systems that provide excellent models for physical phenomena at the two-dimensional (2D) limit. While most studies to date have focused on electrons…

Optical absorption is one of fundamental light-matter interactions. In most materials, optical absorption is a weak perturbation to the light. In this regime, absorption and emission are irreversible, incoherent processes due to strong…

Recently, holey graphene (HG) has successfully synthesized at atomic precision of hole size and shape. This shows interesting physical and chemical properties for energy and environmental applications. Shaping of the pores also transforms…

介观与纳米尺度物理 · 物理学 2020-09-02 Deobrat Singh , Vivekanand Shukla , Rajeev Ahuja

We have developed a contact-less technique for the real time measurement of a-thermal (Cooper-pair breaking) phonons in an absorber held at sub-Kelvin temperatures. In particular, a thin-film aluminum superconducting resonator was realized…

Due to potential applications in nano- and opto-electronics, two-dimensional (2D) materials have attracted tremendous interest. Their thermal transport properties are closely related to the performance of 2D materials-based devices. Here,…

材料科学 · 物理学 2019-02-20 San-Dong Guo

Optically active defects in hexagonal boron nitride (hBN) have become amongst the most attractive single-photon emitters in the solid state, owing to their high-quality photophysical properties, combined with the unlimited possibilities of…

Understanding the limits of phononic heat dissipation from a two-dimensional layered material (2DLM) to its hexagonal boron nitride (h-BN) substrate and how it varies with the structure of the 2DLM is important for the design and thermal…

介观与纳米尺度物理 · 物理学 2021-04-19 Zhun-Yong Ong , Gang Zhang , Yong-Wei Zhang

The strong light-matter interaction in monolayer transition metal dichalcogenides (TMDs) is promising for nanoscale optoelectronics with their direct band gap nature and the ultra-fast radiative decay of the strongly bound excitons these…

Based on the Bethe-Salpeter equation eigenstates, we present a first-principles many-body formalism for calculating the two-photon absorption (TPA) coefficient of semiconductors. We apply this formalism to calculate the TPA spectra of MoS2…

材料科学 · 物理学 2020-06-02 You-Zhao Lan , Xiao-Hu Bao

Excitons in atomically-thin semiconductors interact very strongly with electromagnetic radiation and are necessarily close to a surface. Here, we exploit the deep-subwavelength confinement of surface plasmon polaritons (SPPs) at the edge of…