相关论文: Optical-cavity manipulation strategies of singlet …
We present a new ab initio approach to study molecules containing heavy atoms strongly interacting with quantum fields in optical devices. The theory has been derived from the relativistic quantum electrodynamics (QED) introducing the…
Singlet fission may boost photovoltaic efficiency [by transforming a singlet exciton into two triplet excitons and thereby doubling the number of excited charge carriers. The primary step of singlet fission is the ultrafast creation of the…
The exact time-dependent potential energy surface driving the nuclear dynamics was recently shown to be a useful tool to understand and interpret the coupling of nuclei, electrons, and photons, in cavity settings. Here we provide a detailed…
In this paper, using a quasi-classical statistical approach based on the Langevin equation, we simulate the fission dynamics of selected even-even $\rm U$, $\rm Pu$, $\rm Cm$, $\rm Cf$ and $\rm Fm$ actinide nuclei. As a preparatory part of…
We consider the superradiant transition of a generalized Tavis-Cummings model, where a number of two-level qubits are coupled to a dissipative cavity. The cavity is coherently driven through a parametric medium, and all-to-all interactions…
Radiation pressure forces in cavity optomechanics allow for efficient cooling of vibrational modes of macroscopic mechanical resonators, the manipulation of their quantum states, as well as generation of optomechanical entanglement. The…
We present a comparison of methods for treating the electrostatic interactions of finite, isolated systems within periodic boundary conditions (PBCs), within Density Functional Theory (DFT), with particular emphasis on linear-scaling (LS)…
Ultracold atoms with cavity-mediated long-range interactions offer a promising platform for investing novel quantum phenomena. Exploiting recent experimental advancements, we propose an experimental scheme to create self-ordered supersolid…
In this work we study singlet fission in tetracene para-dimers, covalently linked by a phenyl group. In contrast to most previous works, we account for the full quantum dynamics of the combined excitonic and vibrational system. For our…
Collision refers to a striking nonlinear interaction in dissipative systems, revealing the particle-like properties of solitons. In dual-wavelength mode-locked fiber lasers, collisions are inherent and periodic. However, how collisions…
Polaritonic chemistry exploits strong light-matter coupling between molecules and confined electromagnetic field modes to enable new chemical reactivities. In systems displaying this functionality, the choice of the cavity determines both…
The Froissart (\F) asymptotic behavior of high energy cross-sections, if considered in a parton picture, is usually represented as a kind of behavior that occurs in the process of a collision of two almost black disks, filled with partons,…
We develop a powerful tree tensor network states method that is capable of simulating exciton-phonon quantum dynamics of larger molecular complexes and open quantum systems with multiple bosonic environments. We interface this method with…
Despite recent numerical evidence, one of the fundamental theoretical mysteries of polaritonic chemistry is how and if collective strong coupling can induce local changes of the electronic structure to modify chemical properties. Here we…
Polycrystalline hcp metals - an important class of engineering materials - typically exhibit complex plasticity because of a limited number of slip systems. Among these metals, deformation is even more complicated in cobalt as it commonly…
Singlet fission (SF) is a multi-exciton generation process that could be harnessed to improve the efficiency of photovoltaic devices. Experimentally, systems derived from the pentacene molecule have been shown to exhibit ultrafast SF with…
A pertinent question in cavity optomechanics is whether reaching the regime of large single-photon cooperativity, where the single-photon coupling rate exceeds the geometric mean of the cavity and mechanical decay rates, can enable any new…
We present a framework for simulating relaxation dynamics through a conical intersection of an open quantum system that combines methods to approximate the motion of degrees of freedom with disparate time and energy scales. In the vicinity…
The fermionic Hubbard model (FHM)[1], despite its simple form, captures essential features of strongly correlated electron physics. Ultracold fermions in optical lattices[2, 3] provide a clean and well-controlled platform for simulating…
With a help of the selfconsistent Hartree-Fock-Bogoliubov (HFB) approach with the D1S effective Gogny interaction and the Generator Coordinate Method (GCM) we incorporate the transverse collective vibrations to the one-dimensional model of…