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For over a decade, cold atoms in lattice potentials have been an attractive platform to simulate phenomena known from solid state theory, as the Mott-insulator transition. In contrast, the field of photonics usually deals with…

Polaritonic states arise when a bright optical transition of a molecular ensemble is resonantly matched to an optical cavity mode frequency. Here, we lay the groundwork to study the behavior of polaritons in clean, isolated systems by…

化学物理 · 物理学 2023-10-20 Adam D. Wright , Jane C. Nelson , Marissa L. Weichman

We develop a kinetic theory of microcavity polaritons in presence of both Coulomb and polariton-phonon interaction, obeying particle number conservation. We study the growth of a macroscopic population of condensed particles in the lowest…

其他凝聚态物理 · 物理学 2007-05-23 Davide Sarchi , Vincenzo Savona

Polaritons are compositional light-matter quasiparticles that arise as a result of strong coupling between a vacuum field of a resonant optical cavity and electronic excitations in quantum emitters. Reaching such a regime is often hard, as…

Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…

介观与纳米尺度物理 · 物理学 2024-08-05 Anna M. Grudinina , Nina S. Voronova

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

化学物理 · 物理学 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

We have developed a non-Markovian theory of the polariton luminescence taking the molecular vibrations into account. The calculations were made in the polariton basis. We have shown that the frequency shift and the polariton spectral lines…

介观与纳米尺度物理 · 物理学 2022-04-19 B. D. Fainberg , V. Al. Osipov

A cavity-polariton, formed due to the strong coupling between exciton and cavity mode, is one of the most promising composite bosons for realizing macroscopic spontaneous coherence at high temperature. Up to date, most of polariton quantum…

介观与纳米尺度物理 · 物理学 2010-07-28 Liaoxin Sun , Shulin Sun , Hongxing Dong , Wei Xie , M. Richard , Lei Zhou , L. S. Dang , Xuechu Shen , Zhanghai Chen

Recent years have seen significant developments in the study of strong light-matter coupling including the control of chemical reactions by altering the vibrational normal modes of molecules. In the vibrational strong coupling regime the…

量子物理 · 物理学 2021-08-27 John Bonini , Johannes Flick

Starting from a set of coupled Boltzmann equations, we investigate the thermalization of a two-species cold atomic gas confined either in a box or in an isotropic harmonic trap. We show that the thermalization times, by contrast to the…

其他凝聚态物理 · 物理学 2008-09-15 Marco Anderlini , David Guery-Odelin

We show how to apply the scaling theory in an inhomogeneous system like harmonically trapped Bose condensate at finite temperatures. We calculate the temperature dependence of the critical number of particles by a scaling theory within the…

统计力学 · 物理学 2009-11-18 Shyamal Biswas

Strong coupling between light and matter is possible with a variety of organic materials. In contrast to the simpler inorganic case, organic materials often have a complicated spectrum, with vibrationally dressed electronic transitions.…

介观与纳米尺度物理 · 物理学 2018-02-02 M. Ahsan Zeb , Peter G. Kirton , Jonathan Keeling

Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…

Polaritonic chemistry exploits strong light-matter coupling between molecules and confined electromagnetic field modes to enable new chemical reactivities. In systems displaying this functionality, the choice of the cavity determines both…

光学 · 物理学 2022-08-25 Jacopo Fregoni , Francisco J. García-Vidal , Johannes Feist

We present indications of thermalization and cooling of quasi-particles, a precursor for quantum condensation, in a plasmonic nanoparticle array. We investigate a periodic array of metallic nanorods covered by a polymer layer doped with an…

Bose-condensation of mass-less quasiparticles (photons) can be easily achieved at the room temperature in lasers. On the other hand, condensation of bosons having a non-zero mass requires usually ultra-low temperatures. Recently, it has…

材料科学 · 物理学 2009-11-10 A. V. Kavokin , I. A. Shelykh , M. M. Glazov

Vibrational polaritons, hybrid light-matter states formed between molecular vibrations and infrared (IR) cavity modes, provide a novel approach for modifying chemical reaction pathways and energy transfer processes. For vibrational…

化学物理 · 物理学 2025-05-16 Xinwei Ji , Tao E. Li

Thermalization of radiation by contact to matter is a well-known concept, but the application of thermodynamic methods to complex quantum states of light remains a challenge. Here we observe Bose-Einstein condensation of photons into the…

The polaronic system consisting of an impurity in a dilute Bose-Einstein condensate is considered in the presence of a narrow Feshbach resonance. For this purpose a coupled-channel model is used, which at the mean field level predicts the…

量子气体 · 物理学 2014-07-04 Wim Casteels , Michiel Wouters

Excitons in lead bromide perovskites exhibit high binding energy and high oscillator strength, allowing for a strong light-matter coupling regime in the perovskite-based cavities localizing photons at the nanoscale. This opens up the way…