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Various noncollinear spin textures and magnetic phases have been predicted in twisted two-dimensional CrI$_3$ due to competing ferromagnetic (FM) and antiferromagnetic (AFM) interlayer exchange from moir\'e stacking - with potential…

Diverse interlayer tunability of physical properties of two-dimensional layers mostly lies in the covalent-like quasi-bonding that is significant in electronic structures but rather weak for energetics. Such characteristics result in…

材料科学 · 物理学 2019-04-03 Peiheng Jiang , Cong Wang , Dachuan Chen , Zhicheng Zhong , Zhe Yuan , Zhong-Yi Lu , Wei Ji

A monolayer of CrI$_3$ is a two-dimensional crystal that in its equilibrium configuration is a ferromagnetic semiconductor, however, two coupled layers can be ferromagnetic or antiferromagnetic depending on the stacking. We study the…

介观与纳米尺度物理 · 物理学 2020-04-07 Andrea Leon , J. W. González , J. Mejía-López , F. Crasto de Lima , E. Suárez Morell

Bilayer CrI$_3$ attracted much attention owing to peculiar switching between the layered ferromagnetic and antiferromagnetic order upon stacking alternation. This finding pointed out the importance of the apparently small interlayer…

材料科学 · 物理学 2024-06-19 Srdjan Stavrić , Paolo Barone , Silvia Picozzi

We address the interplay between stacking and interlayer exchange for ferromagnetically ordered CrI$_3$, both for bilayers and bulk. Whereas bulk CrI$_3$ is ferromagnetic, both magneto-optical and transport experiments show that interlayer…

介观与纳米尺度物理 · 物理学 2019-08-29 D. Soriano , C. Cardoso , J. Fernández-Rossier

The interlayer magnetic interaction in bilayer CrI$_3$ plays a crucial role for its device applications. In this work, we studied the interlayer magnetic interaction in $\pi/3$-twisted bilayer CrI$_3$ using first-principles calculations.…

材料科学 · 物理学 2022-01-11 Haodong Yu , Jize Zhao , Fawei Zheng

We present a comprehensive theory of the magnetic phases in twisted bilayer Cr-trihalides through a combination of first-principles calculations and atomistic simulations. We show that the stacking-dependent interlayer exchange leads to an…

强关联电子 · 物理学 2021-08-13 Muhammad Akram , Harrison LaBollita , Dibyendu Dey , Jesse Kapeghian , Onur Erten , Antia S. Botana

The emergence of two-dimensional (2D) magnetic crystals and moir\'e engineering has opened the door for devising new magnetic ground states via competing interactions in moir\'e superlattices. Although a suite of interesting phenomena,…

Magnetic anisotropy is crucially important for the stabilization of two-dimensional (2D) magnetism, which is rare in nature but highly desirable in spintronics and for advancing fundamental knowledge. Recent works on CrI$_3$ and CrGeTe$_3$…

材料科学 · 物理学 2018-11-14 Changsong Xu , Junsheng Feng , Hongjun Xiang , L. Bellaiche

We report the connection between the stacking order and magnetic properties of bilayer CrI$_3$ using first-principles calculations. We show that the stacking order defines the magnetic ground state. By changing the interlayer stacking order…

材料科学 · 物理学 2018-11-19 Nikhil Sivadas , Satoshi Okamoto , Xiaodong Xu , Craig. J. Fennie , Di Xiao

Changes in the spin configuration of atomically-thin, magnetic van-der-Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information…

介观与纳米尺度物理 · 物理学 2020-05-28 Zhe Wang , Marco Gibertini , Dumitru Dumcenco , Takashi Taniguchi , Kenji Watanabe , Enrico Giannini , Alberto F. Morpurgo

Long-range magnetic orders in atomically thin ferromagnetic CrI3 give rise to new fascinating physics and application perspectives. The physical properties of two-dimensional (2D) ferromagnetism CrI3 are significantly influenced by…

Atomically thin films of layered chromium triiodide (CrI$_3$) have recently been regarded as suitable candidates to a wide spectrum of technologically relevant applications, mainly owing to the opportunity they offer to achieve a reversible…

强关联电子 · 物理学 2020-05-01 Michele Pizzochero , Oleg V. Yazyev

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

介观与纳米尺度物理 · 物理学 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

Recent observation of intrinsic ferromagnetism in two-dimensional (2D) CrI$_3$ is associated with the large magnetic anisotropy due to strong spin-orbit coupling (SOC) of I. Magnetic anisotropy energy (MAE) defines the stability of…

介观与纳米尺度物理 · 物理学 2018-10-10 Lucas Webster , Jia-An Yan

We use a first-principles calculations approach to reveal the electronic and magnetic properties of chromium diiodide (CrI$_2$) bilayers and establish a hierarchy of magnetic interactions across stable registries. The monolayer presents a…

材料科学 · 物理学 2025-12-23 B. Valdés-Toro , I. Ferreira-Araya , R. A. Gallardo , J. W. González

We performed the detailed microscopic analysis of the inter-layer magnetic couplings for bilayer CrI$_3$. As the first step toward understanding the recent experimental observations and utilizing them for device applications, we estimated…

材料科学 · 物理学 2019-04-10 Seung Woo Jang , Min Yong Jeong , Hongkee Yoon , Siheon Ryee , Myung Joon Han

The marked interplay between the crystalline, electronic, and magnetic structure of atomically thin magnets has been regarded as the key feature for designing next-generation magneto-optoelectronic devices. In this respect, a detailed…

强关联电子 · 物理学 2020-05-25 Michele Pizzochero , Ravi Yadav , Oleg V. Yazyev

Following the recent isolation of monolayer CrI3, there has been a surge of new two-dimensional van der Waals magnetic materials, whose incorporation in van der Waals heterostructures offers a new platform for spintronics, proximity…

The recent discovery of ferromagnetic single-layer CrI3 creates ample opportunities for studying fundamental properties of atomically-thin magnets. By using first-principles calculations and model analysis, we show that a lateral strain…

介观与纳米尺度物理 · 物理学 2017-09-19 Fawei Zheng , Jize Zhao , Zheng Liu , Menglei Li , Mei Zhou , Shengbai Zhang , Ping Zhang
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