相关论文: Persistent spin dynamics in magnetically ordered h…
Motivated by the possible triple-$\bf Q$ classical order in the Kitaev candidate material Na$_2$Co$_2$TeO$_6$, we investigate microscopic models that may stabilize the triple-$\bf Q$ order by studying an extended Kitaev honeycomb model with…
There have been constant efforts to find exotic quantum spin-liquid (QSL) materials. Some of the transition metal insulators dominated by the direction dependent anisotropic exchange interaction (Kitaev model for honeycomb network of…
Finding new materials with antiferromagnetic (AFM) Kitaev interaction is an urgent issue to broaden and enrich the quantum magnetism research significantly. By carrying out inelastic neutron scattering experiments and subsequent analysis,…
We report terahertz spectroscopic measurements of quantum spin dynamics in the spin-1/2 honeycomb magnet Na$_2$Co$_2$TeO$_6$ as a function of applied magnetic field with different terahertz polarizations. Distinct field dependencies of the…
Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…
Competition and cooperation between electron correlation and relativistic spin-orbit coupling give rise to diverse exotic quantum phenomena in solids. An illustrative example is spin-orbit entangled quantum liquids, which exhibit remarkable…
Na$_2$IrO$_3$, a honeycomb 5$d^5$ oxide, has been recently identified as a potential realization of the Kitaev spin lattice. The basic feature of this spin model is that for each of the three metal-metal links emerging out of a metal site,…
Spin-orbital generalization of Kitaev model provides a robust extension to the original Kitaev model. However, real materials often exhibit competing interactions that break exact solvability which can give rise to new phases. Motivated by…
Kitaev iridates have been proposed as candidates for realizing an elusive quantum spin liquid (QSL) state, in which strong spin-orbit coupling and bond-directional exchange generate a highly frustrated and entangled ground state. However,…
We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…
We report the synthesis and properties of (H,Li)$_{6}$Ru$_{2}$O$_{6}$, which is shown to be a $J_{\text{eff}}=\frac{1}{2}$ system made out of Ru$^{3+}$ moments in a honeycomb geometry. Bulk magnetization, heat capacity, nuclear magnetic…
The Kitaev spin liquid, stabilized as the ground state of the Kitaev honeycomb model, is a paradigmatic example of a topological $\mathbb{Z}_2$ quantum spin liquid. The fate of the Kitaev spin liquid in presence of an external magnetic…
Co-based honeycomb magnets have been actively studied recently for the potential realization of emergent quantum magnetism therein such as the Kitaev spin liquid. Here we employ density functional and dynamical mean-field theory methods to…
We propose a theoretical model for a gapless spin liquid phase that may have been observed in a recent experiment on $\mathrm{H_3Li Ir_2 O_6}$. Despite the insulating and non-magnetic nature of the material, the specific heat coefficient…
Recently, realizations of Kitaev physics have been sought in the A2IrO3 family of honeycomb iridates, originating from oxygen-mediated exchange through edge-shared octahedra. However, for the j = 1/2 Mott insulator in these materials…
The honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has recently been proposed as a candidate material for hosting field-induced quantum spin liquid (QSL) behavior. Here, we present a comprehensive thermodynamic study of its low-temperature,…
The layered honeycomb magnet $\alpha$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a…
We have investigated the magnetic properties and mapped out the phase diagram of the honeycomb magnet Na2Co2TeO6 with Co 3d7 in out-of-plane magnetic fields. This material has previously been proposed to show nearest-neighbor Kitaev…
Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…
A prominent feature of quantum spin liquids is fractionalization of the spin degree of freedom. Fractionalized excitations have their own dynamics in different energy scales, and hence, affect finite-temperature ($T$) properties in a…