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Modeling charge transport in DNA is essential to understand and control the electrical properties and develop DNA-based nanoelectronics. DNA is a fluctuating molecule that exists in a solvent environment, which makes the electron…

生物物理 · 物理学 2023-10-05 Hashem Mohammad , M. P. Anantram

Charge transfer can take place along double helical DNA over distances as long as 30 nanometers. However, given the active role of the thermal environment surrounding charge carriers in DNA, physical mechanisms driving the transfer process…

介观与纳米尺度物理 · 物理学 2020-12-04 Roman Korol , Dvira Segal

Charge migration along DNA molecules has attracted scientific interest for over half a century. Reports on possible high rates of charge transfer between donor and acceptor through the DNA, obtained in the last decade from solution…

材料科学 · 物理学 2009-11-10 Danny Porath , Gianaurelio Cuniberti , Rosa Di Felice

Motivated by the wide ranging experimental results on the conductivity of DNA, we have investigated extraordinary configurations and chemical environments in which DNA might become a true molecular wire, perticularly from enhanced…

软凝聚态物质 · 物理学 2009-09-29 R. G. Endres , D. L. Cox , R. R. P. Singh

Measurements of electron transfer rates as well as of charge transport characteristics in DNA produced a number of seemingly contradictory results, ranging from insulating behaviour to the suggestion that DNA is an efficient medium for…

软凝聚态物质 · 物理学 2007-05-23 R. Bulla , R. Gutierrez , G. Cuniberti

Strong influence of water molecules on the transport and magnetic properties of DNA, observed in this study, opens up real opportunities for application of DNA in molecular electronics. Interaction of the nucleobases with water molecules…

化学物理 · 物理学 2010-08-13 Julia Berashevich , Tapash Chakraborty

We study the electronic properties of DNA by way of a tight-binding model applied to four particular DNA sequences. The charge transfer properties are presented in terms of localisation lengths, crudely speaking the length over which…

基因组学 · 定量生物学 2007-05-23 Daphne Klotsa , Rudolf A. Roemer , Matthew S. Turner

The rapid progress in the field of molecular electronics has led to an increasing interest on DNA oligomers as possible components of electronic circuits at the nanoscale. For this, however, an understanding of charge transfer and transport…

软凝聚态物质 · 物理学 2007-05-23 R. Gutierrez , G. Cuniberti

The question of whether DNA conducts electric charges is intriguing to physicists and biologists alike. The suggestion that electron transfer/transport in DNA might be biologically important has triggered a series of experimental and…

无序系统与神经网络 · 物理学 2020-05-04 H. Wang , R. Marsh , J. P. Lewis , R. A. Roemer

Microscopic mechanisms of positive charge transfer in DNA remain unclear. A quantum state of electron hole in DNA is determined by the competition of a pi-stacking interaction $b$ smearing a charge between different base pairs and…

软凝聚态物质 · 物理学 2008-03-15 D. B. Uskov , A. L. Burin

In this work we report the study of conformation dependent electronic transport properties of DNA double-helix within tight-binding framework including its helical symmetry. We have studied the changes in localization properties of DNA as…

介观与纳米尺度物理 · 物理学 2022-06-20 Sourav Kundu , S. N. Karmakar

Microscopic mechanisms of positive charge transfer in DNA remain unclear. A quantum state of electron hole in DNA is determined by the competition of the pi-stacking interaction $b$ sharing a charge between different base pairs and the…

软凝聚态物质 · 物理学 2008-06-06 Dmitry B. Uskov , Alexander L. Burin

Long range charge transfer experiments in DNA oligomers and the subsequently measured -- and very diverse -- transport response of DNA wires in solid state experiments exemplifies the need for a thorough theoretical understanding of charge…

基因组学 · 定量生物学 2015-05-13 G. Cuniberti , E. Macia , A. Rodriguez , R. A. Römer

We studied the electrical conductivity of DNA molecules with conducting atomic force microscopy as a function of the chemical nature of the substrate surfaces, the nature of the electrical contact, and the number of DNA molecules (from a…

材料科学 · 物理学 2009-11-10 Thomas Heim , Dominique Deresmes , Dominique Vuillaume

Electronic properties of DNA are believed to play a crucial role in many phenomena in living organisms, for example the location of DNA lesions by base excision repair (BER) glycosylases and the regulation of tumor-suppressor genes such as…

其他定量生物学 · 定量生物学 2012-02-21 Chi-Tin Shih , Stephen A. Wells , Ching-Ling Hsu , Yun-Yin Cheng , Rudolf A. Römer

The complex mechanisms governing charge migration in DNA oligomers reflect the rich structural and electronic properties of the molecule of life. Controlling the mechanical stability of DNA nanowires in charge transport experiments is a…

介观与纳米尺度物理 · 物理学 2015-05-13 Bo Song , Marcus Elstner , Gianaurelio Cuniberti

Charge transport through a short DNA oligomer (Dickerson dodecamer) in presence of structural fluctuations is investigated using a hybrid computational methodology based on a combination of quantum mechanical electronic structure…

软凝聚态物质 · 物理学 2015-05-14 R. Gutierrez , R. Caetano , P. B. Woiczikowski , T. Kubar , M. Elstner , G. Cuniberti

Quantum transport for DNA conduction has widely studied with interest in application as a candidate in making nanowires as well as interest in the scientific mechanism. In this paper, we review recent works with concerning the electronic…

无序系统与神经网络 · 物理学 2015-03-13 Hiroaki Yamada , Kazumoto Iguchi

Fast, reliable and inexpensive DNA sequencing is an important pursuit in healthcare, especially in personalized medicine with possible deep societal impacts. Despite significant progress of various nanopore-based sequencing configurations,…

The interaction between metal atoms and nucleobases has been a topic of high interest due to the wide scientific and technological implications. Combining density functional theory simulations with a literature overview, we achieved an…

材料科学 · 物理学 2020-02-10 Leonardo Andres Espinosa Leal , Olga Lopez-Acevedo
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