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Molecular matter-wave interferometry enables novel strategies for manipulating the internal mechanical motion of complex molecules. Here, we show how chiral molecules can be prepared in a quantum superposition of two enantiomers by…

量子物理 · 物理学 2021-09-22 Benjamin A. Stickler , Mira Diekmann , Robert Berger , Daqing Wang

Molecular chirality detection and enantiomer discrimination are very important issues for many areas of science and technology, prompting intensive investigations via optical methods. However, these methods are hindered by the intrinsically…

Two molecules are enantiomers if they are non-superimposable mirror images of each other. Electric dipole-allowed cyclic transitions $|1\rangle\to|2\rangle\to|3\rangle\to|1\rangle$ obey the symmetry relation…

量子物理 · 物理学 2022-03-08 Kai Schwennicke , Joel Yuen-Zhou

We introduce a microscopy technique that facilitates the prediction of spatial features of chirality of nanoscale samples by exploiting photo-induced optical force exerted on an achiral tip in the vicinity of the test specimen. The…

Chirality is probably the most mysterious among all symmetry transformations. Very readily broken in biological systems, it is practically absent in naturally occurring inorganic materials and is very challenging to create artificially.…

A novel optical method for distinguishing chiral molecules is proposed and validated within a quantum simulator employing a trapped-ion qudit. This approach correlates the sign disparity of the dipole moment of chiral molecules with…

量子物理 · 物理学 2024-03-11 Teng Liu , Fa Zhao , Pengfei Lu , Qifeng Lao , Min Ding , Ji Bian , Feng Zhu , Le Luo

Preferential selection of a given enantiomer over its chiral counterpart becomes increasingly relevant in the advent of the next era of medical drug design. In parallel, cavity quantum electrodynamics has grown into a solid framework to…

量子物理 · 物理学 2023-04-14 Christian Schäfer , Denis G. Baranov

Circular Dichroism (CD) can distinguish the handedness of chiral molecules. However, it is typically very weak due to vanishing absorption at low molecular concentrations. Here, we suggest Thermal Circular Dichroism (TCD) for chiral…

光学 · 物理学 2024-07-19 Ershad Mohammadi , Giulia Tagliabue

Enantioselective interactions of chiral molecules include distinct absorptions to opposite-handed circularly polarized light, known as chiral absorption. Traditionally, chiral absorption has been primarily attributed to electric dipole and…

光学 · 物理学 2024-06-03 Hanwei Wang , Yang Zhao

The recent research of topological photonics has not only proposed and realized novel topological phenomena such as one-way broadband propagation and robust transport of light, but also designed and fabricated photonic devices with…

Time photonic crystals are media in which their electromagnetic parameters are modulated periodically in time, showing promising applications in non-resonant lasers and particle accelerators, among others. Traditionally utilized to study…

The integration of chirality into functional materials enables control of light-matter interactions beyond binary illumination (on/off). Conventional photoactuators rely on binary modulation, limiting them to unidirectional motion. In…

材料科学 · 物理学 2025-12-11 Wookjin Jung , Dongkyu Lee , Yonghee Lee , Ki Hyun Park , Jihyeon Yeom

Chiral edge modes in photonic topological insulators host great potential to realize slow-light waveguides with topological protection. Increasing the winding of the chiral edge mode around the Brillouin zone can lead to broadband…

应用物理 · 物理学 2021-03-31 Letian Yu , Haoran Xue , Baile Zhang

Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…

It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…

光学 · 物理学 2020-04-14 David Ayuso , Andres Ordonez , Piero Decleva , Misha Ivanov , Olga Smirnova

Geometrical chirality is a universal property encountered on very different length scales ranging from geometrical shapes of living organisms to protein and DNA molecules. Interaction of chiral matter with chiral light - that is,…

光学 · 物理学 2022-01-25 Kirill Voronin , Alexey Taradin , Maxim V. Gorkunov , Denis G. Baranov

We examine spin-resolved photoionization of randomly oriented chiral molecules via circularly polarized light, and revisit earlier predictions of Cherepkov (J. Phys. B: Atom. Mol. Phys. 16, 1543, 1983). We will show that the dynamical…

Photonic modes exhibiting a polarization winding akin to a vortex possess an integer topological charge. Lasing with topological charge 1 or 2 can be realized in periodic lattices of up to six-fold rotational symmetry. Higher order charges…

Non-Hermitian topological systems simultaneously posses two antagonistic features: ultra sensitivity due to exceptional points and robustness of topological zero energy modes, and it is unclear which one prevails under different…

光学 · 物理学 2022-03-08 I. Komis , D. Kaltsas , S. Xia , H. Buljan , Z. Chen , K. G. Makris

Topological photonics provides an important platform for the development of photonic devices with robust disorder-immune light transport and controllable helicity. Mixing photons with excitons (or polaritons) gives rise to nontrivial…