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X-ray photoelectron spectroscopy (XPS) is a widely used technique for chemical analysis of solid surfaces, sensitive to the chemical environments of atoms via core-level binding energy shifts. While modern instruments allow experimental…

材料科学 · 物理学 2026-05-12 Jan Čechal

Photon emission correlation spectroscopy is an indispensable tool for the study of atoms, molecules, and, more recently, solid-state quantum defects. In solid-state systems, its most common use is as an indicator of single-photon emission,…

量子物理 · 物理学 2023-11-28 Rebecca E. K. Fishman , Raj N. Patel , David A. Hopper , Tzu-Yung Huang , Lee C. Bassett

Realistic simulations of experiments at large scale photon facilities, such as optical laser laboratories, synchrotrons, and free electron lasers, are of vital importance for the successful preparation, execution, and analysis of these…

Device architectures and dimensions are now at an unimaginable level not thought possible even 10 years ago. The continued downscaling, following the so-called Moore's law, has motivated the development and use of extreme ultraviolet (EUV)…

Characterization of the electronic band structure of solid state materials is routinely performed using photoemission spectroscopy. Recent advancements in short-wavelength light sources and electron detectors give rise to multidimensional…

Optical spectroscopy is an important and widely used technique, for instance, to characterize new materials and to identify unknown compounds. Spectra are typically reported as a function of the wavelength of light, yet the information…

光学 · 物理学 2026-05-06 Erik F. Woering , Richard Hildner

Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

光学 · 物理学 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

In this short communication, we revise and refine our previous articles on this topic to simplify the modifications to the angle-resolved photoemission spectroscopy (ARPES) spectrometers required to finally implement our idea, with minimal…

仪器与探测器 · 物理学 2026-04-07 Swapnil Patil

Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes the electron optics allows imaging of the image plane, momentum plane, or…

Photon-based spectroscopies have had a significant impact on both fundamental science and applications by providing an efficient approach to investigate the microscopic physics of materials. Together with the development of synchrotron…

We present a simplified web-based application for simulating x-ray and photoelectron spectra of transition metals, built around the notion that web-based applications lower the bar for novice users. The application provides a simple…

强关联电子 · 物理学 2021-09-14 T. P. Devereaux , B. Moritz , C. Jia , J. J. Kas , J. J. Rehr

Photoemission electron microscopy was used to image the electrons photoemitted from specially tailored Ag nanoparticles deposited on a Si substrate (with its native oxide SiO$_{x}$). Photoemission was induced by illumination with a Hg…

Progress in performing angle-resolved photoemission spectroscopy (ARPES) with high spatial resolution in the order of 1~$\mu$m or less (nanoARPES) has opened the possibility to map the spectral function of solids on this tiny scale and…

强关联电子 · 物理学 2021-05-24 Philip Hofmann

Exploring the interaction of light and matter at the ultimate limit of single photons and single emitters is of great interest both from a fundamental point of view and for emerging applications in quantum engineering. However, the…

量子物理 · 物理学 2015-05-30 Y. L. A. Rezus , S. G. Walt , R. Lettow , A. Renn , G. Zumofen , S. Goetzinger , V. Sandoghdar

The issue of surface sensitivity, and its relationship with interpretation of spectral features observed in angle-resolved photoemission spectroscopy experiments is investigated. Rather than attempt to make an explicit connection to bulk…

强关联电子 · 物理学 2023-07-19 Ryan P. Day , Ilya S. Elfimov , Andrea Damascelli

At photoelectrosynthetic interfaces, an electrochemical reaction is driven by excited charge-carriers from a semiconducting photoabsorber. Structure and composition of this interface determine both the electronic and electrochemical…

化学物理 · 物理学 2022-05-30 Matthias M. May , Wolfram Jaegermann

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

In this review, we aim to introduce the reader to the technique of electrical impedance spectroscopy (EIS) with a focus on its biological and medical applications. We explain the theoretical and experimental aspects of the EIS with the…

The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…

量子物理 · 物理学 2015-06-22 Allan S. Johnson , Joel Yuen-Zhou , Alán Aspuru-Guzik , Jacob J. Krich

Following the lifespan of optical excitations from their creation to decay into photons is crucial in understanding materials optical properties. Macroscopically, techniques such as the photoluminescence excitation spectroscopy provide…

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