相关论文: Quasi-classical simulations of resonance Raman spe…
Classical simulation of quantum computation has often been viewed as the method to determine where the horizon of quantum supremacy is located---that is, where quantum computation can no longer be simulated by classical methods. As of now,…
Understanding the interaction of charge carriers with lattice vibrations in the quasi-equilibrium regime is crucial for semiconductor functionality. However, the structural signatures of these interactions are often too subtle for…
We present a self-consistent quantum optics approach to calculating the surface enhanced Raman spectrum of molecules coupled to arbitrarily shaped plasmonic systems. Our treatment is intuitive to use and provides fresh analytical insight…
These lectures are intended as an introduction to the technique of path integrals and their applications in physics. The audience is mainly first-year graduate students, and it is assumed that the reader has a good foundation in quantum…
A numerical algorithm for studying strongly correlated electron systems is proposed. The groundstate wavefunction is projected out after numerical renormalization procedure in the path integral formalism. The wavefunction is expressed from…
Transient absorption and Raman scattering measurements on noble metal nanoparticles offer complimentary information on their vibrational modes and mechanical interactions with their surroundings. We have developed a comprehensive modeling…
Highly excited vibrational states of an isolated molecule encode the vibrational energy flow pathways in the molecule. Recent studies have had spectacular success in understanding the nature of the excited states mainly due to the extensive…
A detailed derivation of the semiclassical propagator in the generalized coherent-state representation is performed by applying the saddle-point method to a path integral over the classical phase space. With the purpose of providing greater…
We present detailed numerical simulations of semiclassical and quantum spectra of a cavity quantum electrodynamics system consisting of a single three-level atom in $\Lambda$-configuration with one of its transitions strongly interacting…
We present a methodology for computing vibrationally and time-resolved pump-probe spectra, which takes into account all vibrational degrees of freedom and is based on the combination of the thawed Gaussian approximation with on-the-fly ab…
The recently introduced acoustic ray-tracing semiclassical (RTS) method is validated for a set of practically relevant boundary conditions. RTS is a frequency domain geometrical method which directly reproduces the acoustic Green's…
In this paper we have presented a generalized treatment of a photon scattering by a harmonic oscillator initially at ground state. We have predicted the scattering cross-section of the oscillator and showed how the treatment invariably…
We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…
We present a quantum-classical hybrid algorithm that simulates electronic structures of periodic systems such as ground states and quasiparticle band structures. By extending the unitary coupled cluster (UCC) theory to describe crystals in…
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes…
To date, two types of coupling between electromagnetic radiation and a crystal lattice have been identified experimentally. One is direct, for infrared (IR)-active vibrations that carry an electric dipole. The second is indirect, it occurs…
We calculate the resonance fluorescence signal of a two-level system coupled to a quantized phonon mode. By treating the phonons in the independent boson model and not performing any approximations in their description, we also have access…
We present a quantum-classical hybrid random power method that approximates a ground state of a Hamiltonian. The quantum part of our method computes a fixed number of elements of a Hamiltonian-matrix polynomial via quantum polynomial…
We introduce coherent-state propagation, a computational framework for simulating bosonic systems. We focus on bosonic circuits composed of displaced linear optics augmented by Kerr nonlinearities, a universal model of bosonic quantum…
Raman spectroscopy stands as a cornerstone technique for probing collective excitations and emergent quantum phases in solids. While polarization-resolved Raman scattering has been widely used to extract symmetry information of eigenmodes,…