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Long-range correlations, which are partially responsible for the observed fragmentation and depletion of low-lying single-particle strength, are studied in the Green's function formalism. The self-energy is expanded up to second order in…

核理论 · 物理学 2009-10-30 Y. Dewulf , D. Van Neck , L. Van Daele , M. Waroquier

The subject of this study is the exchange-correlation-energy functional of reduced density matrix functional theory. Approximations of this functional are tested by applying them to the homogeneous electron gas. We find that two…

材料科学 · 物理学 2011-01-14 N. N. Lathiotakis , N. Helbig , E. K. U. Gross

We present an overview of electronic device modeling using non-equilibrium Green function techniques. The basic approach developed in the early 1970s has become increasingly popular during the last 10 years. The rise in popularity was…

介观与纳米尺度物理 · 物理学 2007-05-23 Roger K. Lake , Rajeev R. Pandey

In this paper, we propose a new Green's function embedding method called PEXSI-$\Sigma$ for describing complex systems within the Kohn-Sham density functional theory (KSDFT) framework, after revisiting the physics literature of Green's…

计算物理 · 物理学 2016-10-20 Xiantao Li , Lin Lin , Jianfeng Lu

For the computational prediction of core electron binding energies in solids, two distinct kinds of modelling strategies have been pursued: the $\Delta$-Self-Consistent-Field method based on density functional theory (DFT), and the GW…

材料科学 · 物理学 2023-06-12 Juhan Matthias Kahk , Johannes Lischner

Disorder is a key factor influencing the behavior of condensed states of matter, however the true extent of its impact is generally difficult to determine due to the prominent roles played by quantum interference, entanglement between spin…

介观与纳米尺度物理 · 物理学 2022-09-27 Simão M. João , J. M. Viana Parente Lopes , Aires Ferreira

We study within the many-body Green's function GW and Bethe-Salpeter formalisms the excitation energies of a paradigmatic model dipeptide, focusing on the four lowest-lying local and charge-transfer excitations. Our GW calculations are…

材料科学 · 物理学 2015-06-17 Carina Faber , Paul Boulanger , Ivan Duchemin , Claudio Attaccalite , Xavier Blase

The Anderson model for a single impurity coupled to two leads is studied using the $GW$ approximation in the strong electron-electron interaction regime as a function of the alignment of the impurity level relative to the chemical…

强关联电子 · 物理学 2015-05-13 Catalin D. Spataru , Mark S. Hybertsen , Steven G. Louie , Andrew J. Millis

The energy gap of correlated Hubbard clusters is well studied for one-dimensional systems using analytical methods and density-matrix-renormalization-group (DMRG) simulations. Beyond 1D, however, exact results are available only for small…

强关联电子 · 物理学 2021-03-09 J. -P. Joost , N. Schlünzen , S. Hese , M. Bonitz , C. Verdozzi , P. Schmitteckert , M. Hopjan

We develop a Green's function approach to quasiparticle excitations of open-shell systems within the GW approximation. It is shown that accurate calculations of the characteristic multiplet structure require a precise knowledge of the self…

材料科学 · 物理学 2014-09-11 Johannes Lischner , Jack Deslippe , Manish Jain , Steven G. Louie

We present a nontrivial model system of interacting electrons that can be solved analytically in the GW approximation. We obtain the particle number from the GW Green's function strictly analytically, and prove that there is a genuine…

材料科学 · 物理学 2008-02-03 Arno Schindlmayr

We present a rigorous framework that combines single-particle Green's function theory with density functional theory based on a separation of electron-electron interactions into short-range and long-range components. Short-range…

化学物理 · 物理学 2018-06-07 Alexei A. Kananenka , Dominika Zgid

The fully self-consistent GW approximation is an established method for electronic structure calculations. Its most serious deficiency is known to be an incorrect prediction of the dielectric response. In this work we examine the GW…

强关联电子 · 物理学 2017-05-24 Kris Van Houcke , Igor S. Tupitsyn , Andrey S. Mishchenko , Nikolay V. Prokof'ev

In this study, we introduce a novel approach to coupled-cluster Green's function (CCGF) embedding by seamlessly integrating conventional CCGF theory with the state-of-the-art sub-system embedding sub-algebras coupled cluster (SES-CC)…

量子物理 · 物理学 2023-12-21 Bo Peng , Karol Kowalski

We demonstrate an efficient nonequilibrium Green's function transport calculation procedure based on the real-space finite-difference method. The direct inversion of matrices for obtaining the self-energy terms of electrodes is…

材料科学 · 物理学 2024-01-09 Tomoya Ono , Yoshiyuki Egami , Kikuji Hirose

Similar to other electron correlation methods, many-body perturbation theory methods based on Green functions, such as the so-called $GW$ approximation, suffer from the usual slow convergence of energetic properties with respect to the size…

In this work we present a three step procedure for generating a closed form expression of the Green's function on both closed and open finite quantum graphs with general self-adjoint matching conditions. We first generalize and simplify the…

量子物理 · 物理学 2023-09-21 Tristan Lawrie , Sven Gnutzmann , Gregor Tanner

The fundamental gap of an interacting many-electron system is given by the sum of the single-particle Kohn-Sham gap and the derivative discontinuity. The latter can be generated by advanced approximations to the exchange-correlation (XC)…

强关联电子 · 物理学 2018-07-16 Maria Hellgren

The algorithm to calculate the generating function for the number of ``skeleton'' diagrams for the irreducible self-energy and vertex parts is derived for the problems with Gaussian random fields. We find an exact recurrence relation…

无序系统与神经网络 · 物理学 2009-10-30 E. Z. Kuchinskii , M. V. Sadovskii

In the last decades, dynamical mean-field theory (DMFT) and its diagrammatic extensions have been successfully applied to describe local and nonlocal correlation effects in correlated electron systems. Unfortunately, except for the exact…

强关联电子 · 物理学 2022-11-02 Julian Stobbe , Georg Rohringer