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Antimony sulfide (Sb2S3) and selenide (Sb2Se3) are emerging earth-abundant absorbers for photovoltaic applications. Solar cell performance depends strongly on charge carrier transport properties but these remain poorly understood in Sb2X3.…

材料科学 · 物理学 2023-02-20 Xinwei Wang , Alex M. Ganose , Seán R. Kavanagh , Aron Walsh

Antimony Selenide (Sb$_2$Se$_3$) is an attractive candidate of photovoltaics with not yet satisfying efficiency. Beside defects, polaron formation originated from lattice distortion was proposed to account for trapping free carriers, and…

材料科学 · 物理学 2024-10-08 Yijie Shi , Xi Wang , Zhong Wang , Zheng Zhang , Fuyong Hua , Chao Chen , Chunlong Hu , Jiang Tang , Wenxi Liang

SnSe is a layered material that currently holds the record for bulk thermoelectric efficiency. The primary determinant of this high efficiency is thought to be the anomalously low thermal conductivity resulting from strong anharmonic…

Excitons consist of electrons and holes held together by their attractive Coulomb interaction. Although excitons are neutral excitations, spatial fluctuations in their charge density couple with the ions of the crystal lattice. This…

材料科学 · 物理学 2024-01-18 Zhenbang Dai , Chao Lian , Jon Lafuente-Bartolome , Feliciano Giustino

Antimonene is a recently discovered two-dimensional semiconductor with exceptional environmental stability, high carrier mobility, and strong spin-orbit interactions. In combination with electric field, the latter provides an additional…

超导电性 · 物理学 2019-03-06 A. V. Lugovskoi , M. I. Katsnelson , A. N. Rudenko

We report a comprehensive THz, infrared and optical study of Nb doped SrTiO3 as well as DC conductivity and Hall effect measurements. Our THz spectra at 7K show the presence of a very narrow (<2 meV) Drude peak, the spectral weight of which…

We investigate the ${\rm H_3S}$ phase of sulphur hydride under high pressure $\simeq$ 200 GPa by means of {\it ab-initio} calculations within the framework of the density-functional theory (DFT) with the PBE0 hybrid exchange-correlation…

超导电性 · 物理学 2015-11-30 Matej Komelj , Henry Krakauer

The phonon-mode decomposition of the electron-phonon coupling in the MgB2-like system Li_{1-x}BC is explored using first principles calculations. It is found that the high temperature superconductivity of such systems results from extremely…

超导电性 · 物理学 2009-11-07 J. M. An , S. Y. Savrasov , H. Rosner , W. E. Pickett

Evidence for strong electron-phonon coupling in high-Tc cuprates is reviewed, with emphasis on the electron and phonon spectral functions. Effects due to the interplay between the Coulomb and electron-phonon interactions are studied. For…

强关联电子 · 物理学 2008-01-17 O. Gunnarsson , O. Rösch

Magnetic measurements have been carried out in the superconducting and normal states of the optimally doped nonmagnetic bismuthate superconductor Ba0.63K0.37BiO3. The magnetic data along with previous muSR, resistivity, and tunneling data…

超导电性 · 物理学 2014-10-16 N. Derimow , J. Labry , A. Khodagulyan , J. Wang , Guo-meng Zhao

Anisotropic electron-phonon interaction is shown to lead to the anisotropic polaron effect. The resulting anisotropy of the polaron band is an exponential function of the electron-phonon coupling and might be as big as $10^3$. This also…

强关联电子 · 物理学 2009-10-31 P E Kornilovitch

Exciton dynamics can be strongly affected by lattice vibrations through electron-phonon coupling. This is rarely explored in two-dimensional magnetic semiconductors. Focusing on bilayer CrI3, we first show the presence of strong…

The polaron binding energy E_{p} in undoped parent cuprates has been determined to be about 1.0 eV from the unconventional oxygen-isotope effect on the antiferromagnetic ordering temperature. The deduced value of E_{p} is in quantitative…

超导电性 · 物理学 2009-11-10 Guo-meng Zhao

When the electron-phonon coupling is quadratic in the phonon coordinates, electrons can pair to form bipolarons due to phonon zero-point fluctuations, a purely quantum effect. We study superconductivity originating from this pairing…

超导电性 · 物理学 2024-09-18 Zhaoyu Han , Steven A. Kivelson , Pavel A. Volkov

Linear response methods are applied to identify the increase in electron-phonon coupling in elemental yttrium that is responsible for its high superconducting critical temperature Tc, which reaches nearly 20 K at 115 GPa. While the…

超导电性 · 物理学 2007-05-23 Z. P. Yin , S. Y. Savrasov , W. E. Pickett

Layered superatomic semiconductors, whose buildings blocks are atomically precise molecular clusters, exhibit interesting electronic and vibrational properties. In recent work [Science 382, 438 (2023)], transient reflection microscopy…

材料科学 · 物理学 2024-01-26 Petra Shih , Timothy C. Berkelbach

Recent studies demonstrate that novel 2D triphosphides semiconductors possess high carrier mobility and promising thermoelectric performance, while the carrier transport behaviors in 2D semimetal triphosphides have never been elucidated…

材料科学 · 物理学 2023-08-09 Yongchao Rao , C. Y. Zhao , Lei Shen , Shenghong Ju

In conventional superconductors, the electron-phonon coupling plays a dominant role in pairing the electrons and generating superconductivity. In high temperature cuprate superconductors, the existence of the electron coupling with phonons…

We perform a high-throughput screening on phonon-mediated superconductivity in ternary metal diboride structure with alkali, alkaline earth, and transition metals. We find 17 ground states and 78 low-energy metastable phases. From fast…

We report on the fabrication and optimization of semi-transparent antimony sulfide (Sb$_2$S$_3$) thin-film solar cells in a superstrate configuration, using RF magnetron sputtering of metallic antimony followed by post-deposition…

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