相关论文: Observation and dynamic control of a new pathway o…
The formation of Li$_2^+$ and subsequently Li$^+$ ions, during the excitation of $^7$Li atoms to the $3S_{1/2}$ state in a $^7$Li magneto optical trap (MOT), is probed in an ion-atom hybrid trap. Associative ionization occurs during the…
Direct D-H exchange in radicals is investigated in a quasi-uniform flow employing chirped pulse mm-wave spectroscopy. Inspired by the H-atom catalyzed isomerization of C3H2 reported in our previous study, D atom reactions with the propargyl…
The formation of $^{40}$Ca$_2^+$ molecular ions is observed in a hybrid $^{40}$Ca magneto-optical and ion trap system. The molecular ion formation process is determined to be two-photon photo-associative ionization of ultracold $^{40}$Ca…
Ultracold atoms coupled to optical cavities offer a powerful platform for studying strongly correlated many-body physics. Here, we propose an experimental scheme for creating biatomic molecules via cavity-enhanced photoassociation from an…
H2 formation in metal-free gas occurs via the intermediate H- or H2+ ions. Destruction of these ions by photodissociation therefore serves to suppress H2 formation. In this paper, I highlight the fact that several processes that occur in…
We examine the detection of the intermediate-mass Higgs boson (IMH) at LHC through the associate production channel pp-->t+(anti-t)+H+X-->l+photon+ photon+X'. It is shown that by applying kinematic cuts or b-tagging on the final state jets,…
The formation of silicon monosulfide (SiS) in space appears to be a difficult process, but the present work is showing that a previously excluded pathway may contribute to its astronomical abundance. Reaction of the radicals SH + SiH…
Femtosecond structural dynamics of diiodomethane ($\mathrm{CH_2I_2}$) triggered by ultraviolet (UV) photoabsorption at 290 nm and 330 nm are studied using time-resolved coincident Coulomb explosion imaging driven by a near-infrared probe…
The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…
Molecular hydrogen (H$_2$) plays a critical role in astrophysical processes from galaxy evolution to the formation of planets. While the dominant formation channel in the interstellar medium is considered as dust-catalyzed H$_2$ formation,…
The first detection of the molecular ion H3+ in an extragalactic object has been made toward the highly obscured ultraluminous galaxy, IRAS 08572+3915. Two absorption features near 3.9 microns in its spectrum are identified as the…
We discuss theoretically ion-atom collisions at low energy and predict the possibility of formation of cold molecular ion by photoassociation. We present results on radiative homo- and hetero-nuclear atom-ion cold collisions that reveal…
Water is the main component of interstellar ice mantles, is abundant in the solar system and is a crucial ingredient for life. The formation of this molecule in the interstellar medium cannot be explained by gas-phase chemistry only and its…
Forty years ago it was proposed that gas phase organic chemistry in the interstellar medium was initiated by the methyl cation CH3+, but hitherto it has not been observed outside the Solar System. Alternative routes involving processes on…
We present a path-integral Monte Carlo study of dissociation in dense hydrogen ($1.75 \leq r_s \leq 2.2$, with $r_s$ the Wigner sphere radius). As temperature is lowered from $10^5$ to 5000 K, a molecular hydrogen gas forms spontaneously…
We present a study on ion-atom-atom reaction A+A+B$^+$ in a wide range of systems and collision energies ranging from 100$~\mu$K to 10$^5~$K, analyzing the two possible products: molecules and molecular ions. The dynamics is performed via a…
We investigate the formation of molecular hydrogen (H_2) in a primordial H+He gas cloud irradiated by a power-law UV flux. We find that at high densities (>1 cm^{-3}) and low temperatures (<10^4 K), the background radiation enhances the…
Methanol (CH3OH) is thought to form on interstellar ice dust via successive hydrogenation reactions. The reaction between CH3 and OH radicals could also conceivably generate methanol at temperatures above approximately 20 K, at which…
With the presence of evermore complex S-bearing molecules being detected lately, studies on their chemical formation routes need to keep up the pace to rationalize observations, suggest new candidates for detection, and provide input for…
Context. Recent Monte Carlo simulations and laboratory studies of interstellar ices have proposed an alternative pathway involving the radical-molecule H-atom abstraction reaction in the overall mechanism of methanol (CH3OH) formation in…