相关论文: Rational pulse design for enantiomer-selective mic…
Polar molecules are an emerging platform for quantum technologies based on their long-range electric dipole-dipole interactions, which open new possibilities for quantum information processing and the quantum simulation of strongly…
We present the first quantum mechanical study of hyperfine effects in the rotational cluster states of a symmetric triatomic molecule H$_2$S. Rotational clusters arise from spontaneous symmetry breaking induced by high-angular-momentum…
In quantum computation, information is processed by gates that must coherently couple separate qubits. In many systems the qubits are naturally coupled, but such an always-on interaction limits the algorithms that may be implemented.…
We experimentally demonstrate stimulated four-wave mixing in two linearly uncoupled integrated Si$_3$N$_4$ micro-resonators. In our structure the resonance combs of each resonator can be tuned independently, with the energy transfer from…
The rotational echo response of molecules is found to strongly depend on the delay between the two ultrashort laser pulses, as opposed to two-level systems. We study this dependence experimentally and theoretically and show that by…
On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…
This work proposes the use of orbital angular momentum (OAM) waves to improve the performance of a computational imaging (CI) system. Specifically, in contrast to a solely frequency-diverse operation, leveraging multiple OAM waves leads to…
The behavior of the generation efficiency and radiation spectrum of a three-cavity axial vircator versus the radius of the injected electron beam, its impedance and energy homogeneity is studied. This paper establishes that for each…
Irradiating intercalated nanorings by optical vortices ignites a charge flow that emits coherent trains of high harmonic bursts with frequencies and time structures that are controllable by the topological charge of the driving vortex beam.…
We show that the chirality of artificial media, made of a planar periodic arrangement of three-dimensional metallic meta-atoms, can be tailored. The meta-atoms support localized plasmon polaritons and exhibit a chirality exceeding that of…
Chiral molecules with broken parity symmetries can be modeled as quantum systems with cyclic-transition structures. By using these novel properties, we design two-step laser pulses to distinguish left- and right-handed molecules from the…
In this work we investigate the theory for three different uni-directional population transfer schemes in trapped multilevel systems which can be utilized to cool molecular ions. The approach we use exploits the laser-induced coupling…
We propose a general technique to produce cold spin-polarized molecules, in which rotationally excited states are first populated by coherent microwave excitation, and then allowed to spin-flip and relax via collisional quenching, which…
In this paper we experimentally demonstrated a broadband microwave scheme suitable for the multiresonator quan- tum memory-interface. The microwave scheme consists of the system of composed mini-resonators strongly inter- acting with a…
Coherent control of ensembles of light emitters by means of multi-wave mixing processes is key for the realization of high capacity optical quantum memories and information processing devices. In this context, semiconductor quantum dots…
Inclusion of time-odd components into the wave function is important for reliable description of rotational motion by the angular-momentum-projection method; the cranking procedure with infinitesimal rotational frequency is an efficient way…
In the previous paper on this topic it was shown how, for a pulse of arbitrary shape and duration, the drive frequency can be analytically optimized to maximize the amplitude of the population oscillations between the selected two levels in…
Performing computational tasks with wave-based devices is becoming a groundbreaking paradigm that can open new opportunities for the next generation of efficient analogue and digital computing systems. Decision-making processes for…
The controlled preparation of the excited state in a quantum emitter is a prerequisite for its usage as single-photon sources - a key building block for quantum technologies. In this paper we propose a coherent excitation scheme using…
We analyze two simple model planar molecules: an ionic molecule with D3 symmetry and a covalent molecule with D6 symmetry. Both symmetries allow the existence of chiral molecular orbitals and normal modes that are coupled to each other in a…