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Efficient energy transport is highly desirable for organic semiconductor (OSC) devices such as photovoltaics, photodetectors, and photocatalytic systems. However, photo-generated excitons in OSC films mostly occupy highly localized states…

The bound electron-hole pairs known as excitons govern the optical properties of insulating solids. While their behavior in equilibrium is well-understood theoretically, the nonequilibrium regime at high excitation densities-where phenomena…

介观与纳米尺度物理 · 物理学 2025-10-31 Pushpendra Yadav

The potential for low-threshold optical nonlinearity has received significant attention in the fields of photonics and conceptual optical neuron networks. Excitons in two-dimensional (2D) semiconductors are particularly promising in this…

Excitons -- two-particle correlated electron-hole pairs -- are the dominant low-energy optical excitation in the broad class of semiconductor materials, which range from classical silicon to perovskites, and from two-dimensional to organic…

材料科学 · 物理学 2025-11-25 Marcel Reutzel , G. S. Matthijs Jansen , Stefan Mathias

Two-dimensional stacking fault defects embedded in a bulk crystal can provide a homogeneous trapping potential for carriers and excitons. Here we utilize state-of-the-art structural imaging coupled with density functional and effective-mass…

Exciton dissociation plays a crucial role in the performance of optoelectronic devices based on two-dimensional (2D) transition metal dichalcogenides (TMDs). In this work, we investigate the effect of an in-plane electric field on the…

材料科学 · 物理学 2024-10-11 Tao Zhu , Chenhang Zheng , Lei Xu , Ming Yang

We theoretically investigate the binding energy and electron-hole (e-h) overlap of excitonic states confined at the interface between two-dimensional materials with type-II band alignment, i.e., with lowest conduction and highest valence…

介观与纳米尺度物理 · 物理学 2025-11-20 Igor L. C. Lima , M. V. Milošević , F. M. Peeters , Andrey Chaves

Due to a strong Coulomb interaction, excitons dominate the excitation kinetics in 2D materials. While Coulomb-scattering between electrons has been well studied, the interaction of excitons is more challenging and remains to be explored. As…

材料科学 · 物理学 2021-01-27 Daniel Erkensten , Samuel Brem , Ermin Malic

The ultrathin transition metal dichalcogenides (TMDs) have emerged as promising materials for various applications using two dimensional (2D) semiconductors. They have attracted increasing attention due to their unique optical properties…

介观与纳米尺度物理 · 物理学 2016-09-20 Aïda Hichri , Imen Ben Amara , Sabrine Ayari , Sihem Jaziri

We study the zero-temperature phase diagram of a symmetric electron-hole bilayer system by comparing the ground state energies of two distinct limiting cases, characterized by an electron-hole plasma or an exciton gas, respectively. For the…

介观与纳米尺度物理 · 物理学 2024-04-23 Yi-Ting Tu , Seth M. Davis , Sankar Das Sarma

Transition metal dichalcogenides layered nano-crystals are emerging as promising candidates for next-generation optoelectronic and quantum devices. In such systems, the interaction between excitonic states and atomic vibrations is crucial…

介观与纳米尺度物理 · 物理学 2023-12-29 Jianbo Hu , Yang Xiang , Beatrice Matilde Ferrari , Emilio Scalise , Giovanni Maria Vanacore

In superlattices of twisted semiconductor monolayers, tunable moir\'e potentials emerge, trapping excitons into periodic arrays. In particular, spatially separated interlayer excitons are subject to a deep potential landscape and they…

介观与纳米尺度物理 · 物理学 2023-06-02 Samuel Brem , Ermin Malic

Excitons in atomically-thin semiconductors necessarily lie close to a surface, and therefore their properties are expected to be strongly influenced by the surrounding dielectric environment. However, systematic studies exploring this role…

介观与纳米尺度物理 · 物理学 2016-12-06 Andreas V. Stier , Nathan P. Wilson , Genevieve Clark , Xiaodong Xu , Scott A. Crooker

When electron-hole pairs are excited in a semiconductor, it is a priori not clear if they form a fermionic plasma of unbound particles or a bosonic exciton gas. Usually, the exciton phase is associated with low temperatures. In atomically…

The concept of \textit{optical} exciton - a photo-excited bound electron-hole pair within a crystal - is routinely used to interpret and model a wealth of excited-state phenomena in semiconductors. Beside originating sub-band gap signatures…

材料科学 · 物理学 2022-09-21 Fulvio Paleari , Andrea Marini

In two-dimensional transition metal dichalcogenide structures, the optical excitation of a bright exciton may be followed by the formation of a plethora of lower energy dark states. In these formation and relaxation processes between…

Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

介观与纳米尺度物理 · 物理学 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

We study theoretically the exciton Bose-Einstein condensation and exciton vortices in a two-dimensional (2D) perovskite (PEA)2PbI4 monolayer. Combining the first-principles calculations and the Keldysh model, the exciton binding energy of…

介观与纳米尺度物理 · 物理学 2020-11-06 Yingda Chen , Dong Zhang , Kai Chang

We present a theoretical study of the exciton binding energy for anisotropic two-dimensional crystals. We obtain analytical expressions from variational wave functions in different limits of the screening length to exciton size ratio and…

介观与纳米尺度物理 · 物理学 2016-03-15 Elsa Prada , J. V. Alvarez , K. L. Narasimha-Acharya , F. J. Bailen , J. J. Palacios