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Two-photon ionization of an alkali-metal atom in the presence of a uniform electric field is investigated using a standardized form of local frame transformation and generalized quantum defect theory. The relevant long-range quantum defect…

量子物理 · 物理学 2015-06-11 P. Giannakeas , F. Robicheaux , Chris H. Greene

Transition matrix elements between electronic states where one electron can be in the continuum are required for a wide range of applications of the molecular R-matrix method. These include photoionization, photorecombination and…

化学物理 · 物理学 2014-01-03 Alex G. Harvey , Danilo S. Brambila , Felipe Morales , Olga Smirnova

The time-dependent surface flux (t-SURFF) method is introduced for computing of strong-field infrared photo-ionization spectra of atoms by numerically solving the time-dependent Schr\"odinger equation on minimal simulation volumes. The…

计算物理 · 物理学 2015-05-30 Liang Tao , Armin Scrinzi

The feasibility of complete photoionization experiments, in which the full set of photoionization matrix elements are determined, using multiphoton ionization schemes with polarization-shaped pulses has recently been demonstrated [Hockett…

原子物理 · 物理学 2015-07-22 P. Hockett , M. Wollenhaupt , C. Lux , T. Baumert

We present an {\it ab initio} and non-perturbative time-dependent approach to the problem of double ionization of a general atom driven by intense XUV laser pulses. After using a highly flexible $B$-Spline $R$-matrix method to generate…

原子物理 · 物理学 2016-11-17 Xiaoxu Guan , O Zatsarinny , C J Noble , K Bartschat , B I Schneider

Two-photon free-free transitions in elastic laser-assisted electron-hydrogen collisions are studied in the domain of high scattering energies and low or moderate field intensities, in the third order of perturbation theory, taking into…

原子物理 · 物理学 2013-03-07 Aurelia Cionga , Gabriela Buica

We give examples showing that two well-known versions of the S-matrix theory, which describes a nonresonant multiphoton ionization of atoms and ions in intense laser fields, lead to qualitatively different results. The latter refer not only…

原子物理 · 物理学 2015-05-28 J. H. Bauer

Electron-impact cross sections for the dissociation process of vibrationally excited He2+ molecular ion, as a function of the incident electron energy are calculated for the dissociative transition X2\Sigma+u \to A2\Sigma+g by using the…

等离子体物理 · 物理学 2015-06-29 R. Celiberto , K. L. Baluja , R. K. Janev , V. Laporta

We use the recently introduced independent-atom-model pixel counting method to calculate proton-impact net ionization cross sections for a large class of biologically relevant systems including pyrimidines, purines, amino acids, and…

原子与分子团簇 · 物理学 2019-10-02 Hans Jürgen Lüdde , Marko Horbatsch , Tom Kirchner

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

原子物理 · 物理学 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

原子物理 · 物理学 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

Stimulated by a recent measurement of coherent control in photoionization of atomic barium, we have calculated one- and two-photon ionization cross sections of the aligned 6s6p^1P_1 state of barium in the energy range between the 5d_{3/2}…

X-ray photoabsorption cross sections have been computed for all magnesium ions using the $R$-matrix method. A comparison with the other available data for Mg II-Mg X shows good qualitative agreement in the resultant resonance shapes.…

原子物理 · 物理学 2015-06-15 M. F. Hasoglu , Sh. A. Abdel-Naby , E. Gatuzz , J. Garcia , T. R. Kallman , C. Mendoza , T. W. Gorczyca

K-shell photoabsorption cross sections for the isonuclear C I - C IV ions have been computed using the R-matrix method. Above the K-shell threshold, the present results are in good agreement with the independent-particle results of Reilman…

原子物理 · 物理学 2015-05-18 M. F. Hasoglu , Sh. A. Abdel-Naby , T. W. Gorczyca , J. J. Drake , B. M. McLaughlin

We outline a formalism and develop a computational procedure to treat the process of multiphoton ionization (MPI) of atomic targets in strong laser fields. We treat the MPI process nonperturbatively as a decay phenomenon by solving a…

原子物理 · 物理学 2026-03-03 I. A. Ivanov , A. S. Kheifets

A new approach is laid out to investigate the two photon atomic transitions. It is based on application of the finite basis solutions constructed from the Bernstein Polynomial (B-Polynomial) sets. We show that such an approach provides a…

数学物理 · 物理学 2015-05-28 P. Amaro , A. Surzhykov , F. Parente , P. Indelicato , J. P. Santos

The photon-ion merged-beams technique was used at a synchrotron light source for measuring absolute cross sections of double and triple photodetachment of O$^{-}$ ions. The experimental photon energy range of 524-543 eV comprised the…

原子物理 · 物理学 2016-10-07 S. Schippers , R. Beerwerth , L. Abrok , S. Bari , T. Buhr , M. Martins , S. Ricz , J. Viefhaus , S. Fritzsche , A. Müller

We apply relativistic many-body methods to compute static differential polarizabilities for transitions inside the ground-state hyperfine manifolds of monovalent atoms and ions. Knowing this transition polarizability is required in a number…

原子物理 · 物理学 2011-07-13 V. A. Dzuba , V. V. Flambaum , K. Beloy , A. Derevianko

X-ray photoelectron spectra provide a wealth of information on the electronic structure. The extraction of molecular details requires adequate theoretical methods, which in case of transition metal complexes has to account for effects due…

A possible route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal and nanometer spatial resolution is to employ recolliding electrons as `probes'. The recollision process in molecules is, however,…