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The functioning and efficiency of natural photosynthetic complexes is strongly influenced by their embedding in a noisy protein environment, which can even serve to enhance the transport efficiency. Interactions with the environment induce…

生物物理 · 物理学 2015-06-03 Sebastiaan M. Vlaming , Robert J. Silbey

A numerical method of calculating the non-Markovian evolution of a driven atom radiating into a structured continuum is developed. The formal solution for the atomic reduced density matrix is written as a Markovian algorithm by introducing…

量子物理 · 物理学 2009-11-06 M. W. Jack , J. J. Hope

Excitation of molecules by incident incoherent electromagnetic radiation, such as sunlight, is described in detail and contrasted with the effect of coherent (e.g. laser) light. The nature of the quantum coherences induced by the former,…

量子物理 · 物理学 2022-02-23 Amro Dodin , Paul Brumer

We have developed a non-Markovian theory of the polariton luminescence taking the molecular vibrations into account. The calculations were made in the polariton basis. We have shown that the frequency shift and the polariton spectral lines…

介观与纳米尺度物理 · 物理学 2022-04-19 B. D. Fainberg , V. Al. Osipov

The photosystem II reaction centre is the photosynthetic complex responsible for oxygen production on Earth. Its water splitting function is particularly favoured by the formation of a stable charge separated state via a pathway that starts…

Photosynthesis powers life on our planet. The basic photosynthetic architecture comprises antenna complexes to harvest solar energy and reaction centers to convert the energy into a stable charge separated state. In oxygenic photosynthesis,…

生物物理 · 物理学 2013-10-07 Franklin D. Fuller , Jie Pan , S. Seckin Senlik , Daniel E. Wilcox , Jennifer P. Ogilvie

In this paper, we investigate the non-Markovian dynamics of a model to mimic the excitation energy transfer (EET) between chromophores in photosynthesis systems. The numerical path integral method is used. This method includes the…

化学物理 · 物理学 2015-05-14 Xian-Ting Liang

Quantum thermal transistors have been widely studied in the context of three-qubit systems, where each qubit interacts separately with a Markovian harmonic bath. Markovianity is an assumption that is imposed on a system if the environment…

量子物理 · 物理学 2025-10-31 Deepika Bhargava , Paranjoy Chaki , Aparajita Bhattacharyya , Ujjwal Sen

A remarkable amount of theoretical research has been carried out to elucidate the physical origins of the recently observed long-lived quantum coherence in the electronic energy transfer process in biological photosynthetic systems.…

量子物理 · 物理学 2015-03-19 Sangwoo Shim , Patrick Rebentrost , Stéphanie Valleau , Alan Aspuru-Guzik

We explore energy transfer in a generic three-level system, which is coupled to three non-equilibrium baths. Built on the concept of quantum heat engine, our three-level model describes non-equilibrium quantum processes including…

量子物理 · 物理学 2016-02-17 Dazhi Xu , Chen Wang , Yang Zhao , Jianshu Cao

Most of our current understanding of mechanisms of photosynthesis comes from spectroscopy. However, classical definition of radio-antenna can be extended to optical regime to discuss the function of light-harvesting antennae. Further to our…

生物物理 · 物理学 2019-04-09 Julian Juhi-Lian Ting

Non-Markovianity, as an important feature of general open quantum systems, is usually difficult to quantify with limited knowledge of how the plant that we are interested in interacts with its environment-the bath. It often happens that the…

量子物理 · 物理学 2011-11-28 Huan Yang , Haixing Miao , Yanbei Chen

A fundamental issue that limits the efficiency of many photoelectrochemical systems is that the photon absorption length is typically much longer than the electron diffusion length. Various photon management schemes have been developed to…

The way a principle system and its environment interact characterizes the non-Markovianity of the dynamics. Herein, we investigate the non-Markovian dynamics of photon polarization in a birefringent crystal. We consider the so-called…

量子物理 · 物理学 2018-10-31 Kai-Hung Wang , Shih-Hsuan Chen , Yu-Cheng Lin , Che-Ming Li

Various engine types are thermodynamically equivalent in the quantum limit of small 'engine action'. Our previous derivation of the equivalence is restricted to Markovian heat baths and to implicit classical work repository (e.g., laser…

量子物理 · 物理学 2016-05-04 Raam Uzdin , Amikam Levy , Ronnie Kosloff

A theoretical investigation on slow light propagation based on eletromagnetically induced transparency in a three-level quantum-dot system is performed including non-Markovian effects and correlated dephasing reservoirs. It is…

量子物理 · 物理学 2016-01-08 D. Mogilevtsev , E. Reyes-Gomez , S. B. Cavalcanti , L. E. Oliveira

Semiconductor quantum dots (QDs) have been demonstrated to be versatile candidates to study the fundamentals of light-matter interaction [1-3]. In contrast with atom optics, dissipative processes are induced by the inherent coupling to the…

介观与纳米尺度物理 · 物理学 2013-10-25 Alexander Carmele , Andreas Knorr , Frank Milde

We study how much the efficiency of a solar cell as a quantum heat engine could be enhanced by quantum coherence. In contrast to the conventional approach that a quantum heat engine is in thermal equilibrium with both hot and cold…

量子物理 · 物理学 2020-05-28 Sangchul Oh

We present the experimental control of Non-Markovian dynamics of open quantum systems simulated with photonic entities. The polarization of light is used as the system, whereas the surrounding environment is represented by light's spatial…

Photosynthetic antenna complexes are responsible for absorbing energy from sunlight and transmitting it to remote locations where it can be stored. Recent experiments have found that this process involves long-lived quantum coherence…

原子物理 · 物理学 2011-08-29 Zachary B. Walters