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Exciton mobility in two-dimensional semiconductors is a key ingredient in materials-based design of optoelectronic functionalities. Monolayer transition metal dichalcogenides (TMDs) set a good test case, with tightly bound excitons and…

材料科学 · 物理学 2026-02-17 Amir Kleiner , Sivan Refaely-Abramson

The optical dielectric function of ZnGeN$_2$ is calculated from the interband transitions using the energy bands calculated in the quasiparticle self-consistent (QS)$G\hat W$ method using two different levels of approximation: the…

材料科学 · 物理学 2024-03-22 Ozan Dernek , Walter R. L. Lambrecht

The non-equilibrium semiconductors physics is based on the paradigm that different degrees of freedom interact on different timescales. In this context the photo-excitation is often treated as an impulsive injection of electronic energy…

We theoretically investigate the energy of the ground state exciton confined to two-dimensional (2D) monolayers with circular shape. Within an effective mass approach employing a nonlocal screening effect on the Coulomb potential energy, we…

介观与纳米尺度物理 · 物理学 2018-08-15 Shota Ono , Tomohiro Ogura

The quasiparticle (QP) band structures of both strainless and strained monolayer MoS$_{2}$ are investigated using more accurate many body perturbation \emph{GW} theory and maximally localized Wannier functions (MLWFs) approach. By solving…

材料科学 · 物理学 2013-04-10 Hongliang Shi , Hui Pan , Yong-Wei Zhang , Boris I. Yakobson

Exciton optical transitions in transition-metal dichalcogenides offer unique opportunities to study rich many-body physics. Recent experiments in monolayer WSe$_2$ and WS$_2$ have shown that while the low-temperature photoluminescence from…

材料科学 · 物理学 2016-08-23 Hanan Dery

We present a systematic theory of Coulomb interaction effects in the nonlinear optical processes in semiconductors using a perturbation series in the exciting laser field. The third-order dynamical response consists of phase-space filling…

凝聚态物理 · 物理学 2009-10-31 Th. Oestreich , K. Schoenhammer , L. J. Sham

A quantum-kinetic approach to the ultrafast dynamics of carrier multiplication in semiconductor quantum dots is presented. We investigate the underlying dynamics in the electronic subband occupations and the time-resolved optical emission…

其他凝聚态物理 · 物理学 2015-05-28 Franz Schulze , Mario Schoth , Ulrike Woggon , Carsten Weber , Andreas Knorr

Engineering and probing excitonic properties at the nanoscale remains a central challenge in quantum photonics and optoelectronics. While exciton confinement via electrical control and strain engineering has been demonstrated in 2D…

介观与纳米尺度物理 · 物理学 2025-09-03 Yueh-Chun Wu , Bogdan Dryzhakov , Huan Zhao , Ivan Vlassiouk , Kyle Kelley , Takashi Taniguchi , Kenji Watanabe , Jun Yan , Benjamin Lawrie

The optical response of quasi-one-dimensional systems is often dominated by tightly bound excitons, that significantly influence their basic electronic properties. Despite their importance for device performance, accurately predicting their…

介观与纳米尺度物理 · 物理学 2024-03-26 Cesar E. P. Villegas , Alexandre R. Rocha

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and…

Excitons are vital in the photophysics of materials, especially in low-dimensional systems. The conceptual and quantitative understanding of excitonic effects in nonlinear optical (NLO) processes is more challenging compared to linear ones.…

材料科学 · 物理学 2026-02-26 Jiawei Ruan , Y. -H. Chan , Steven G. Louie

Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…

Wigner crystals, lattices made purely of electrons, are a quintessential paradigm of studying correlation-driven quantum phase transitions. Despite decades of research, the internal dynamics of Wigner crystals has remained extremely…

In this paper we consider dynamics of a molecular system subjected to external pumping by a light source. Within a completely quantum mechanical treatment, we derive a general formula, which enables to asses effects of different light…

生物物理 · 物理学 2012-01-30 Tomas Mancal , Leonas Valkunas

In strongly correlated systems the strength of Coulomb interactions between electrons, relative to their kinetic energy, plays a central role in determining their emergent quantum mechanical phases. We perform resonant x-ray scattering on…

One of the most striking features of novel 2D semiconductors (e.g., transition metal dichalcogenide monolayers or phosphorene) is a strong Coulomb interaction between charge carriers resulting in large excitonic effects. In particular, this…

介观与纳米尺度物理 · 物理学 2015-11-18 Kirill A. Velizhanin , Avadh Saxena

Electron-phonon coupling is central to many condensed matter phenomena. Harnessing these effects for novel material functionality in materials always involves non-equilibrium electronic states, which in turn alter quasi-free-carrier density…

Excitonic quasi-particles, excitons/trions/bi-excitons, and their coupling with phonons and charge carriers play a crucial role in controlling the optical properties of atomically thin semiconducting 2D materials. In this work, we…

材料科学 · 物理学 2021-10-01 Deepu Kumar , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

A key feature of monolayer semiconductors, such as transition-metal dichalcogenides, is the poorly screened Coulomb potential, which leads to large exciton binding energy (Eb) and strong renormalization of the quasiparticle bandgap (Eg) by…

强关联电子 · 物理学 2019-06-26 Fang Liu , Mark Ziffer , Kameron R. Hansen , Jue Wang , Xiaoyang Zhu