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We explore the outcomes of detailed microscopic models by calculating second- and third-harmonic generation from thin film surfaces with discontinuous free-electron densities. These circumstances can occur in structures consisting of a…

Many metallic transition-metal oxides turn insulating when grown as films that are only a few unit-cells thick. The microscopic origins of these thickness induced metal-to-insulator transitions however remain under dispute. Here, we…

强关联电子 · 物理学 2022-01-19 Matthias Pickem , Josef Kaufmann , Karsten Held , Jan M. Tomczak

Due to its wide band gap and high carrier mobility, ZnO is an attractive material for light-harvesting and optoelectronic applications. Its functional efficiency, however, is strongly affected by defect-related in-gap states that open up…

The interplay of electric charge, spin, and orbital polarizations, coherently driven by picosecond long oscillations of light fields in spin-orbit coupled systems, is the foundation of emerging terahertz spintronics and orbitronics. The…

Superconducting cavity electro-optics (EO) presents a promising route to coherently convert microwave and optical photons and distribute quantum entanglement between superconducting circuits over long-distance through an optical network.…

Near-zero-refractive index materials display unique optical properties such as perfect transmission through distorted waveguides, cloaking, and inhibited diffraction. Compared to conventional media, they can fundamentally behave differently…

光学 · 物理学 2025-11-06 Ben Johns , Hannes Kempf , Lakshmi Das , Aitor De Andrés , Nicolò Maccaferri

Epsilon-near-zero (ENZ) materials, including artificial metamaterials, have been advanced to mold laser beams and antenna-mediated radiated waves. Here we propose an efficient method to control Ohmic losses inherent to natural ENZ materials…

光学 · 物理学 2017-09-13 Mahin Naserpour , Carlos J. Zapata-Rodriguez , Mahdieh Hashemi

We investigate second harmonic generation, low-threshold multistability, all-optical switching, and inherently nonlocal effects due to the free-electron gas pressure in an epsilon-near-zero (ENZ) metamaterial slab made of cylindrical,…

A methodology is proposed for finding structures that are, optically speaking, locally optimal : a physical analysis of much simpler structures is used to constrain the optimization process. The obtained designs are based on a flat…

光学 · 物理学 2012-05-02 Antoine Moreau , Rafik Smaali , Emmanuel Centeno , Christian Seassal

In this paper, we demonstrate NiCo$_2$O$_4$ (NCO) as an efficient new nonlinear optical material with straightforward potential applications in optical limiting devices. We obtain nonlinear absorption coefficient ($\beta$) and nonlinear…

Inversion symmetry breaking is a ubiquitous concept in condensed-matter science. On the one hand, it is a prerequisite for many technologically relevant effects such as piezoelectricity, photovoltaic and nonlinear optical properties and…

材料科学 · 物理学 2021-04-28 J. Nordlander , M. D. Rossell , M. Campanini , M. Fiebig , M. Trassin

In this work, we propose epsilon-near-zero (ENZ) nanoparticles formed of metal and dielectric bilayers and employ the effective medium approach for multilayered nanospheres to study their optical response. We obtained a passive tunable ENZ…

Bacterial infections are a common problem in daily life that can affect human health. Researchers are looking for valuable materials that can help prevent such infections and environmental pollutants. Thin films are a well-known application…

材料科学 · 物理学 2023-12-18 Mehmet Eymen Sumer , Bengu Ozugur Uysal

The development of nanoscale nonlinear elements in photonic integrated circuits is hindered by the physical limits to the nonlinear optical response of dielectrics, which requires that the interacting waves propagate in transparent volumes…

Titanium dioxide is one of the most widely used wide bandgap materials. However, the TiO2 deposited on a substrate is not always transparent leading to a loss in efficiency of the device, especially, the photo response. Herein, we show that…

We present a multifunctional on-chip optical device utilizing epsilon-near-zero (ENZ) metamaterials, allowing precise beam control through phase modulation. This design acts as both an all-optical switch and a tunable beam splitter,…

光学 · 物理学 2025-01-17 Yu Peng

The unique electronic properties of amorphous indium gallium zinc oxide (a-IGZO) thin films are closely associated with the complex charge dynamics of the materials. Conventional studies of charge transport in a-IGZO usually involve…

材料科学 · 物理学 2024-11-19 Jia Yu , Yuchen Zhou , Xiao Wang , Xuejian Ma , Ananth Dodabalapur , Keji Lai

Epsilon-near-zero (ENZ) metamaterial slabs at visible frequencies based on metal-dielectric multilayers are experimentally realized. Transmission, reflection and absorption spectra are measured and used to determine the complex refractive…

The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…

材料科学 · 物理学 2018-12-27 J. L. Cheng , J. E. Sipe , S. W. Wu , Chunlei Guo

Light in the mid-infrared (mid-IR) spans wavelengths from 3-8 $\mu$m and is important to many applications such as gas sensing and thermal imaging. Due to materials challenges, there is currently a lack of mid-IR reconfigurable optical…

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