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The inelastic nature of 3-phonon processes is investigated within the framework of perturbation theory and linearized Boltzmann Transport Equation. By considering the energy conservation rule governing this type of interactions in a…

材料科学 · 物理学 2017-09-07 Ahmed Hamed , Anter El-Azab

Nanostructured superlattices have been the focus of many researchers due to their physical and manipulatable properties. They aim to find promising materials for new electronic and thermoelectric devices. In the present study, we…

材料科学 · 物理学 2021-07-29 Leila Razzaghi , Farhad Khoeini , Ali Rajabpour , Maryam Khalkhali

Peierls-Boltzmann transport equation, coupled with third-order anharmonic lattice dynamics calculations, has been widely used to model lattice thermal conductivity ($\kappa_{l}$) in bulk crystals. However, its application to materials with…

材料科学 · 物理学 2018-11-08 Yi Xia , Maria K. Y. Chan

Group-VI transition metal dichalcogenides (TMDs), MoS$_2$ and MoSe$_2$, have emerged as prototypical low-dimensional systems with distinctive phononic and electronic properties, making them attractive for applications in nanoelectronics,…

材料科学 · 物理学 2025-09-18 Tugbey Kocabas , Murat Keceli , Tanju Gurel , Milorad Milosevic , Cem Sevik

Lattice thermal conductivities of two SiO$_2$ polymorphs, i.e., $\alpha$-quartz (low) and $\alpha$-cristobalite (low), were studied using first-principles anharmonic phonon calculation and linearized phonon Boltzmann transport equation.…

材料科学 · 物理学 2018-06-20 Keiyu Mizokami , Atsushi Togo , Isao Tanaka

Ternary pnictides semiconductors with II-IV-V2 stoichiometry hold potential as cost effective thermoelectric materials with suitable electronic transport properties, but their lattice thermal conductivities ($\kappa$) are typically too…

We compute the thermal conductivity of monolayer beryllene using the linearized phonon Boltzmann transport equation with interatomic force constants obtained from \textit{ab-initio} calculations. Monolayer beryllene exhibits an impressive…

材料科学 · 物理学 2024-09-10 Sapta Sindhu Paul Chowdhury , Santosh Mogurampelly

We calculate the phonon thermal conductivity of various moir\'e bilayer systems using a continuum approach and the semiclassical transport theory. When the twist angle is close to 0, we observe a significant reduction of thermal…

介观与纳米尺度物理 · 物理学 2025-03-11 Lukas P. A. Krisna , Takuto Kawakami , Mikito Koshino

The layered semiconductor SnSe is one of the highest-performing thermoelectric materials known. We demonstrate, through a first-principles lattice-dynamics study, that the high-temperature Cmcm phase is a dynamic average over lower-symmetry…

We carry out a systematic study of the thermal conductivity of four single-layer transition metal dichalcogenides, MX$_2$ (M = Mo, W; X = S, Se) from first-principles by solving the Boltzmann Transport Equation (BTE). We compare three…

材料科学 · 物理学 2019-03-29 Pol Torres , Francesc Xavier Alvarez , Xavier Cartoixà , Riccardo Rurali

The proximity to structural phase transitions in IV-VI thermoelectric materials is one of the main reasons for their large phonon anharmonicity and intrinsically low lattice thermal conductivity $\kappa$. However, the $\kappa$ of GeTe…

材料科学 · 物理学 2021-02-23 Đorđe Dangić , Olle Hellman , Stephen Fahy , Ivana Savić

Lead and tin chalcogenides have been studied widely due to their promising thermoelectric (TE) properties. Further enhancement in their TE efficiency has been reported upon the reduction of the dimension, which is an important feature in…

材料科学 · 物理学 2020-10-14 Abhiyan Pandit , Bothina Hamad

Transition metal dichalcogenides are investigated for various applications at the nanoscale thanks to their unique combination of properties and dimensionality. For many of the anticipated applications, heat conduction plays an important…

The phonon thermal conductivity of a multilayer is calculated for transport perpendicular to the layers. There is a cross over between particle transport for thick layers to wave transport for thin layers. The calculations shows that the…

材料科学 · 物理学 2009-10-31 M. V. Simkin , G. D. Mahan

We design a hybrid graphene/hexagonal boron nitride superlattice monolayer and investigate its thermoelectric properties using density functional theory and Boltzmann transport equations with the relaxation time accurately treated by…

材料科学 · 物理学 2019-05-31 Zizhen Zhou , Huijun Liu , Dengdong Fan , Guohua Cao

The lattice thermal conductivity ($\kappa_{\rm L}$) of PbTiO$_3$ (PTO) is estimated using a combination of {\em ab initio} calculations and semiclassical Boltzmann transport equation. The computed $\kappa_{\rm L}$ is remarkably low, nearly…

材料科学 · 物理学 2016-03-23 Anindya Roy

Lattice thermal conductivities (LTCs) of \alpha-, \beta-, and \gamma-Si$_3$N$_4$ single crystals are investigated from ab initio anharmonic lattice dynamics, within the single-mode relaxation-time approximation of the linearized phonon…

材料科学 · 物理学 2016-12-28 Kazuyoshi Tatsumi , Atsushi Togo , Isao Tanaka

Elemental 2D materials exhibit intriguing heat transport and phononic properties. Here we have investigated the lattice thermal conductivity of newly proposed arsenene, the 2D honeycomb structure of arsenic, using {\it ab initio}…

材料科学 · 物理学 2016-02-24 M. Zeraati , S. M. Vaez Allaei , I. Abdolhosseini Sarsari , M. Pourfath , D. Donadio

We calculate the thermal conductivity (\k{appa}) of both bulk crystalline and single-chain polyethylene (PE) using the first-principles-based anharmonic lattice dynamics. Despite its low \k{appa} in amorphous state, the predicted bulk…

介观与纳米尺度物理 · 物理学 2017-01-11 Xinjiang Wang , Massoud Kaviany , Baoling Huang

We systematically investigated the phonon and electron transport properties of monolayer InSe and its Janus derivatives including monolayer In2SSe and In2SeTe by first-principles calculations. The breaking of mirror symmetry produce a…

材料科学 · 物理学 2019-08-05 Wenhui Wan , Shan Zhao , Yanfeng Ge , Yong Liu