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We show that the photoelectron angular distributions produced by elliptical and cross-polarized two-color laser fields interacting with randomly oriented chiral molecules decompose into four irreducible representations of the $D_{2h}$ point…

Magneto optic measurements are a very powerful tool for investigating the polarization of a conduction band as a function of temperature and are used here to study the polarization of the mobile electrons in 50nm LSMO (x=0.3) strained thin…

强关联电子 · 物理学 2009-11-13 T. K. Nath , J. R. Neal , G. A. Gehring

The high brightness, broad spectral coverage and pulsed characteristics of infrared synchrotron radiation enable time-resolved spectroscopy under throughput-limited optical systems, as can occur with the high-field magnet cryostat systems…

The practical applications of chiral discrimination are usually limited by the weak chiral response of enantiomers and the high complexity of detection methods. Here, we propose to use the C lines (i.e., lines of polarization singularities)…

光学 · 物理学 2022-03-22 Shiqi Jia , Jie Peng , Yuqiong Cheng , Shubo Wang

We propose a predictive building-up of tetrahedral molecules, based on a previously derived chirality index, which characterizes a tetrahedral molecule, with n chiral centers, as achiral, diastereoisomer, or enantiomer as a function of the…

化学物理 · 物理学 2008-11-26 S. Capozziello , A. Lattanzi

Polarization-dependent photon spectroscopy (dichroism) of the second-harmonic generation (SHG) response is shown to reveal chiral and magnetic properties of a sample. Two dichroic signals are allowed with electric-dipole (E1) and…

强关联电子 · 物理学 2019-12-11 S. W. Lovesey , G. van der Laan

A new application of a fast CCD drift scanning technique that allows us to perform speckle imaging of binary stars is presented. For each observation, an arbitrary number of speckle frames is periodically stored on a computer disk, each…

天体物理学 · 物理学 2007-05-23 O. Fors , E. P. Horch , J. Nunez

We theoretically investigate light matter interactions for chiral molecules in the presence of non-chiral nanoantennas. Isotropic nanostructures supporting optical-frequency electric or magnetic dipoles are sufficient to locally enhance the…

介观与纳米尺度物理 · 物理学 2013-06-14 Aitzol Garcia-Etxarri , Jennifer A. Dionne

We describe an optical near shot-noise limited time-resolved circular dichroism (TRCD) pump-probe spectrometer capable of reliably measuring {\mu}deg circular dichroism signal with nanosecond time resolution. Such sensitivity is achieved…

仪器与探测器 · 物理学 2018-04-04 Valentyn Stadnytskyi , Gregory S. Orf , Robert E. Blankenship , Sergei Savikhin

Magnetic circular dichroism (MCD) in the x-ray absorption spectroscopy (XAS) at the L2,3 edges for almost entire series of rare-earth (RE) elements in RE2Fe14B, is studied experimentally and theoretically. By a quantitative comparison of…

强关联电子 · 物理学 2009-10-31 K. Fukui , H. Ogasawara , A. Kotani , I. Harada , H. Maruyama , N. Kawamura , K. Kobayashi , J. Chaboy , A. Marcelli

Recent experiments have probed the chiral properties of semiconductor nanocrystal (NC) quantum dots (QDs), but understanding the circular dichroism lineshape, excitonic features, and ligand induction mechanism remains a challenge. We…

材料科学 · 物理学 2024-04-18 Daniel Chabeda , Stephen Gee , Eran Rabani

Recently, two related three wave mixing experiments have been demonstrated that use allowed rotational transitions to produce a free induction decay signal with an amplitude linearly proportional to the enantiomeric excess of a chiral…

化学物理 · 物理学 2015-01-22 Kevin K. Lehmann

It is very interesting to bring plasmonic circular dichroism spectroscopy to the mid-infrared spectral interval, and there are two reasons for this. This spectral interval is very important for thermal bio-imaging and, simultaneously, this…

材料科学 · 物理学 2017-09-08 Xiang-Tian Kong , Runbo Zhao , Zhiming Wang , Alexander O. Govorov

Utilizing the line-group symmetry of single-wall nanotubes, we have assigned their electron-energy bands by the symmetry-based quantum numbers. The selection rules for optical absorption are presented in terms of these quantum numbers.…

软凝聚态物质 · 物理学 2009-10-31 I. Bozovic , N. Bozovic , M. Damnjanovic

Polariton states with high levels of chiral dissymmetry offer exciting prospects for quantum information, sensing, and lasing applications. Such dissymmetry must emanate from either the involved optical resonators or the quantum emitters.…

化学物理 · 物理学 2022-09-28 Andrew H. Salij , Randall H. Goldsmith , Roel Tempelaar

This study aims to develop a novel Cycle-guided Denoising Diffusion Probability Model (CG-DDPM) for cross-modality MRI synthesis. The CG-DDPM deploys two DDPMs that condition each other to generate synthetic images from two different MRI…

图像与视频处理 · 电气工程与系统科学 2023-05-02 Shaoyan Pan , Chih-Wei Chang , Junbo Peng , Jiahan Zhang , Richard L. J. Qiu , Tonghe Wang , Justin Roper , Tian Liu , Hui Mao , Xiaofeng Yang

Circular dichroism is the differential rate of absorption of right- and left-handed circularly polarized light by chiral particles. Optical vortices which convey orbital angular momentum (OAM) possess a chirality associated with the…

光学 · 物理学 2021-05-26 Kayn A. Forbes , Garth A. Jones

Enantiomers are chiral molecules that exist in right-handed and left-handed conformations. Optical techniques of enantiomers detection are widely employed to discriminate between left- and right-handed molecules. However, identical spectra…

量子物理 · 物理学 2023-05-10 Mohsen Izadyari , M. Tahir Naseem , Özgür E. Müstecaplıouglu

Molecular chirality has traditionally been viewed as a binary property where a molecule is classified as either chiral or achiral, yet in the recent decades mathematical methods for quantifying chirality have been explored. Here we use toy…

化学物理 · 物理学 2024-11-28 Ethan Abraham , Abraham Nitzan

The development of efficient techniques to distinguish mirror images of chiral molecules (enantiomers) is very important in both chemistry and physics. Enantiomers share most molecular properties except, for instance, the absorption of…

化学物理 · 物理学 2023-07-11 Rosario R. Riso , Laura Grazioli , Enrico Ronca , Tommaso Giovannini , Henrik Koch