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The recent discovery of superconductivity in Sr-doped NdNiO$_2$, with a critical temperature of $10-15$ K suggests the possibility of a new family of nickel-based high-temperature superconductors (HTS). NdNiO$_{2}$ is the $n=\infty$ member…

强关联电子 · 物理学 2021-09-15 Harrison LaBollita , Antia S. Botana

It has been recently shown that under pressure trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ (LNO) becomes superconducting below a critical temperature $\sim$20 K, in addition to the infinite-layer and bilayer systems. Motivated…

强关联电子 · 物理学 2024-06-12 I. V. Leonov

Charge order is a central feature of the physics of cuprate superconductors and is known to arise from a modulation of holes with primarily oxygen character. Low-valence nickelate superconductors also host charge order, but the electronic…

Research on nickel-based superconductors has progressed from infinite-layer LaNiO$_2$ to finite-layer La$_{6}$Ni$_{5}$O$_{12}$, and most recently to the Ruddlesden-Popper phase La$_3$Ni$_2$O$_7$, which was found to exhibits onset of…

Flat electronic bands are expected to show proportionally enhanced electron correlations, which may generate a plethora of novel quantum phases and unusual low-energy excitations. They are increasingly being pursued in $d$-electron-based…

强关联电子 · 物理学 2024-06-21 Lei Chen , Fang Xie , Shouvik Sur , Haoyu Hu , Silke Paschen , Jennifer Cano , Qimiao Si

Using DFT+DMFT we study the normal-state electronic structure and magnetic correlations of the recently discovered alternating single-layer bilayer Raddlesden-Popper nickelate La$_5$Ni$_3$O$_{11}$ (1212-LNO). Our results exhibit qualitative…

强关联电子 · 物理学 2026-04-30 I. V. Leonov

The relationship between the long-range antiferromagnetic order in cuprates and the high-temperature superconductivity in these compounds represents unresolved, nearly four-decades long scientific problem. Because recently discovered…

超导电性 · 物理学 2023-09-21 E. F. Talantsev

The interplay among orbital-selective Mott physics, Hund's coupling, tunable structural motifs, and Kondo-like scattering establishes a compelling paradigm for understanding and engineering correlated multi-orbital systems, as vividly…

Since the discovery of cuprate, the origin of high-T$_c$ superconductivity has been an outstanding puzzle. Recently, high-T$_c$ superconductivity was observed in a bilayer nickelate La$_3$Ni$_2$O$_7$ under pressure, whose structure hosts…

超导电性 · 物理学 2025-05-09 Yuhao Gu , Congcong Le , Zhesen Yang , Xianxin Wu , Jiangping Hu

The discovery of superconductivity at 80 K under high pressure in La$_3$Ni$_2$O$_7$ presents the groundbreaking confirmation that high-$T_c$ superconductivity is a property of strongly correlated materials beyond cuprates. We use density…

超导电性 · 物理学 2024-07-30 Zhen Fan , Jian-Feng Zhang , Bo Zhan , Dingshun Lv , Xing-Yu Jiang , Bruce Normand , Tao Xiang

Since the discovery of high-temperature superconductivity in the copper oxide materials, there have been sustained efforts to both understand the origins of this phase and discover new cuprate-like superconducting materials. One prime…

Recently, signatures of superconductivity with critical temperature from 20 to 30 K have been reported in pressured trilayer nickelate La$_4$Ni$_3$O$_{10}$ through a pressure-induced structure transition. Here we explore the evolution of…

强关联电子 · 物理学 2024-06-18 Peng-Fei Tian , Hao-Tian Ma , Xing Ming , Xiao-Jun Zheng , Huan Li

Significant magnetic exchange interactions have been observed in infinite-layer nickelates RNiO2 (R = La, Pr, Nd), which exhibit unconventional superconductivity upon hole doping. Despite their structural and Fermi surface similarities to…

超导电性 · 物理学 2025-05-15 Yanbing Zhou , Dan Zhao , Boyun Zeng , Chengliang Xia , Yu Wang , Hanghui Chen , Tao Wu , Xianhui Chen

Conflicting theoretical scenarios for infinite-layer nickelate superconductors have been hotly debated, particularly regarding whether {only} a single Ni-3$d_{x^2-y^2}$ band is relevant at low energies besides electron pockets or whether…

Superconductivity is one of the most intriguing properties of matter described by an attractive interaction that bounds electrons into Cooper pairs. To date, the highest critical temperature at ambient conditions is achieved in copper…

We report on optical studies of the Ruddlesden-Popper nickelates La$_{n+1}$Ni$_{n}$O$_{3n+1}$ with $n = 2$ (La$_{3}$Ni$_{2}$O$_{7}$), $n = 3$ (La$_{4}$Ni$_{3}$O$_{10}$) and $n = \infty$ (LaNiO$_{3}$). As the number of the NiO$_{6}$…

超导电性 · 物理学 2024-11-14 Zhe Liu , Jie Li , Mengwu Huo , Bingke Ji , Jiahao Hao , Yaomin Dai , Mengjun Ou , Qing Li , Hualei Sun , Bing Xu , Yi Lu , Meng Wang , Hai-Hu Wen

Ruddlesden-Popper nickelates exhibit superconductivity under pressure in bulk crystals and under epitaxial constraint in thin films, while remaining highly sensitive to sample quality, oxygen content, defects, and stress conditions. We…

超导电性 · 物理学 2026-05-15 Liling Sun , Shu Cai , Jinyu Zhao , Qi Wu , Yang Ding , Tao Xiang , Ho-kwang Mao

We report a $^{139}$La-NMR study of polycrystalline samples of multi($n$)-layered nickelates, La$_3$Ni$_2$O$_{7-\delta}$ ($n=2$) and La$_4$Ni$_3$O$_{10-\delta}$ ($n=3$), at ambient pressure. Measurements of the nuclear magnetic resonance…

Weak-coupling approaches to the pairing problem in the iron pnictide superconductors have predicted a wide variety of superconducting ground states. We argue here that this is due both to the inadequacy of certain approximations to the…

超导电性 · 物理学 2009-03-02 S. Graser , T. A. Maier , P. J. Hirschfeld , D. J. Scalapino

Dimensionality and electronic correlations are crucial elements of many quantum material properties. An example is the change of the electronic structure accompanied by the loss of quasiparticles when a metal is reduced from three…