相关论文: Inner-shell excitation in the YbF molecule and its…
We report the complete characterization of various cooling grade Tm-doped crystals including the first demonstration of optical refrigeration in Tm:YLF crystals. Room temperature laser cooling efficiencies of 1% and 2% (mol) Tm:YLF, and 1%…
We generate 555.8nm light with sub-MHz linewidth through the use of laser injection-locking of a semiconductor diode at 1111.6nm, followed by frequency doubling in a resonant cavity. The integrity of the injection lock is investigated by…
We have investigated the structural dynamics in photoexcited 1,2-diiodotetrafluoroethane molecules (C2F4I2) in the gas phase experimentally using ultrafast electron diffraction and theoretically using FOMO-CASCI excited state dynamics…
YbInCu$_4$ undergoes a first order structural phase transition near $T_v$=40 K associated with an abrupt change of Yb valence state. We perform ultrafast pump-probe measurement on YbInCu$_4$ and find that the expected heavy fermion…
We have measured the Stark shift of the $A^2\Pi_{1/2} - X^2\Sigma^+$ transition in YbF. We use a molecular beam triple resonance method, with two laser transitions acting as pump and probe, assisted by an rf transition that tags a single…
We have studied the effects of loading $^{87}$Rb into a far off resonant trap (FORT) in the presence of an ultracold cloud of $^{85}$Rb. The presence of the $^{85}$Rb resulted in a marked decrease of the $^{87}$Rb load rate. This decrease…
An accurate determination of the effective electric field (Eeff) in YbF is important, as it can be combined with the results of future experiments to give an improved new limit for the electric dipole moment of the electron. We report a…
The term `laser cooling' is applied to the use of optical means to cool the motional energies of either atoms and molecules, or micromirrors. In the literature, these two strands are kept largely separate; both, however suffer from severe…
Analysis of the electronic state of the CuO2 planes of high-Tc materials has been performed with special regard to the influence of the Coulomb interactions separated after moments. Different symmetry breaking effects were revealed. A…
Photoionization cross sections and partial ion yields of Xe and XeF$_2$ from Xe 3d$_{5/2}$, Xe 3d$_{3/2}$, and F 1s subshells in the 660--740 eV range are compared to explore effects of the F ligands. The Xe 3d - $\epsilon$f continuum shape…
We report ab initio correlated relativistic calculations of the effective electric field W_d acting on the electron in two excited electronic states of PbO, required for extracting the electric dipole moment of the electron from an ongoing…
We propose a scheme for laser cooling of negatively charged molecules. We briefly summarise the requirements for such laser cooling and we identify a number of potential candidates. A detailed computation study with C$\_2^-$, the most…
Doppler cooling with lasers is essential to ions' trapping and also a preliminary step towards achievement of ultracold ions. Due to lack of effective tools, experimentally monitoring the ions' temperature and the laser-ion coupling is…
The direct laser cooling of neutral diatomic molecules in molecular beams suggests that trapped molecular ions can also be laser cooled. The long storage time and spatial localization of trapped molecular ions provides the opportunity for…
Fast and efficient state preparation of molecules can be accomplished by optical pumping. Molecular structure that most obviously facilitates cycling involves a strong electronic transition, with favorable vibrational branching (diagonal…
We consider ground state of electron-hole graphene bilayer composed of two independently doped graphene layers when a condensate of spatially separated electron-hole pairs is formed. In the weak coupling regime the pairing affects only…
We prepare mixtures of ultracold CaF molecules and Rb atoms in a magnetic trap and study their inelastic collisions. When the atoms are prepared in the spin-stretched state and the molecules in the spin-stretched component of the first…
We describe a spin interferometer using ultracold YbF molecules and develop the complete set of techniques needed to measure the electron's electric dipole moment, $d_e$, with this apparatus. The molecules are cooled in an optical molasses…
Controlling the internal degrees of freedom is a key challenge for applications of cold and ultracold molecules. Here, we demonstrate rotational-state cooling of trapped methyl fluoride molecules (CH3F) by optically pumping the population…
We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…