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BiFeO3 is a model multiferroic in which the ferroelectric polarization is coupled to ferroelastic lattice distortions, yet deterministic control of its domain structure remains limited by high switching fields and competing polarization…

In a solid, the electronic subsystem can exhibit incipient order with lower point group symmetry than the crystal lattice. External fields that couple to electronic order parameters have rarely been investigated, however, despite their…

强关联电子 · 物理学 2024-01-11 Xinshu Zhang , Tyler Carbin , Adrian B. Culver , Kai Du , Kefeng Wang , Sang-Wook Cheong , Rahul Roy , Anshul Kogar

The crystal structure of BiFeO3/BaxSr1-xTiO3 (BFO/BST) heterostructures with x = 0.2, 0.6 and 0.8, grown on single-crystal MgO (001) substrate was investigated by x-ray diffraction and Raman spectroscopy in order to determine the influence…

While BiFeO3-based solid solutions show great promise for applications in energy conversion and storage, realizing this promise necessitates understanding the structure-property relationship in particular pertaining to the relaxor-like…

Multiferroic oxides, such as BiFeO3, have garnered significant attention due to their coupled ferroelectric, magnetic, and elastic properties, offering exciting opportunities for multifunctional device applications. Controlling phase…

材料科学 · 物理学 2025-02-19 Fei Sun , Chao Chen , Deyang Chen , Minghui Qin , Xubing Lu , Xingsen Gao , Christopher T Nelson , Jun-Ming Liu

Nonvolatile bipolar resistive switching has been observed in an Au/BiFeO3/Pt structure, where a Schottky contact and a quasi-Ohmic contact were formed at the Au/BiFeO3 and BiFeO3/Pt interface, respectively. By changing the polarity of the…

材料科学 · 物理学 2011-06-30 Yao Shuai , Shengqiang Zhou , Danilo Bürger , Manfred Helm , Heidemarie Schmidt

Heterostructures based on two dimensional (2D) materials offer the possibility to achieve synergistic functionalities which otherwise remain secluded by their individual counterparts. Herein ferroelectric polarization switching in…

Utilizing ultrafast light-matter interaction to manipulate electronic states of quantum materials is an emerging area of research in condensed matter physics. It has significant implications for the development of future ultrafast…

The structural and polar properties of BiFeO3 at finite temperature are investigated using an atomistic shell model fitted to first-principles calculations. Molecular Dynamics simulations show a direct transition from the low-temperature…

材料科学 · 物理学 2015-06-23 M. Graf , M. Sepliarsky , S. Tinte , M. G. Stachiotti

Electric-field (E-field) control of magnetism enabled by multiferroics has the potential to revolutionize the landscape of present memory devices plagued with high energy dissipation. To date, this E-field controlled multiferroic scheme at…

Intrinsic magnetoelectric coupling describes the interaction between magnetic and electric polarization through an inherent microscopic mechanism in a single phase material. This phenomenon has the potential to control the magnetic state of…

The interplay between crystal symmetry and its optical responses is at the heart of tremendous recent advances in light-matter interactions and applications. Nonlinear optical processes that produce electric currents, for example bulk…

材料科学 · 物理学 2021-10-27 Yongliang Shi , Jian Zhou

Bismuth ferrite is one of the most widely studied multiferroic materials because of its large ferroelectric polarisation coexisting with magnetic order at room temperature. Using density functional theory (DFT), we identify several…

材料科学 · 物理学 2021-05-12 Bastien F. Grosso , Nicola A. Spaldin

Given the paucity of single phase multiferroic materials (with large ferromagnetic moment), composite systems seem an attractive solution in the quest to realize magnetoelectric cou-pling between ferromagnetic and ferroelectric order…

介观与纳米尺度物理 · 物理学 2014-09-15 P. Jain , Q. Wang , M. Roldan , A. Glavic , V. Lauter , C. Urban , Z. Bi , T. Ahmed , J. Zhu , M. Varela , Q. Jia , M. R. Fitzsimmons

We study the electrical behavior of multiferroic BiFeO$_3$ by means of first-principles calculations. We do so by constraining a specific component of the electric displacement field along a variety of structural paths, and by monitoring…

材料科学 · 物理学 2016-01-20 Massimiliano Stengel , Jorge Íñiguez

The kinetics and thermodynamics of first order transitions is universally controlled by defects that act as nucleation sites and pinning centers. Here we demonstrate that defect-domain interactions during polarization reversal processes in…

材料科学 · 物理学 2009-11-13 S. V. Kalinin , S. Jesse , B. J. Rodriguez , Y. H. Chu , R. Ramesh , E. A. Eliseev , A. N. Morozovska

The highly mobile electrons at the interface of SrTiO3 with other oxide insulators, such as LaAlO3 or AlOx, are of great current interest. A vertical gate voltage allows controlling a metal/superconductor-to-insulator transition, as well as…

Under a sufficiently high applied electric field, a non-polar antiferroelectric material, such as \ce{PbZrO3}, can undergo a rapid transformation to a polar ferroelectric phase. While this behavior is promising for energy storage and…

A comparative study of the non-equilibrium magnetic phenomena (magnetic blocking, memory, exchange bias and aging effect) has been presented for ferrimagnetic Co$_{1.75}$Fe$_{1.25}$O$_4$ (CFO) and its composite with non-magnetic BaTiO$_3$…

材料科学 · 物理学 2021-05-19 R. N. Bhowmik , R. Ranganathan

Multiferroic BiFeO$_3$ (BFO) possesses a rich phase diagram that allows strain tuning of its properties in thin-film form. In particular, at large compressive strain, a supertetragonal (T) phase with giant polarization is stabilized over…

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