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Adsorption of organic molecules on well-oriented single crystal coinage metal surfaces fundamentally affects the energy distribution curve of ultra-violet photoelectron spectroscopy spectra. New features not present in the spectrum of the…

Accurately described excitonic properties of transition metal dichalcogenide heterobilayers (HBLs) are crucial to comprehend the optical response and the charge carrier dynamics of them. Excitons in multilayer systems posses inter or…

材料科学 · 物理学 2018-08-01 E. Torun , A. Molina-Sánchez , H. P. C. Miranda , L. Wirtz

Cooperative effects allow for fascinating characteristics in light-matter interacting systems. Here, we study naturally occurring superradiant coupling in a class of quasi-two-dimensional, layered semiconductor systems. We perform optical…

介观与纳米尺度物理 · 物理学 2018-06-08 C. E. Stevens , T. Stroucken , A. V. Stier , J. Paul , H. Zhang , P. Dey , S. A. Crooker , S. W. Koch , D. Karaiskaj

Hybrid interfaces formed by inorganic semiconductors and organic molecules are intriguing materials for opto-electronics. Interfacial charge transfer is primarily responsible for their peculiar electronic structure and optical response.…

The unusual transport properties of graphene are the direct consequence of a peculiar bandstructure near the Dirac point. We determine the shape of the pi bands and their characteristic splitting, and the transition from a pure 2D to…

材料科学 · 物理学 2007-05-23 Taisuke Ohta , Aaron Bostwick , J. L. McChesney , Thomas Seyller , Karsten Horn , Eli Rotenberg

Twisted van der Waals heterostructures and the corresponding superlattices, moire superlattices, are remarkable new material platforms, in which electron interactions and excited-state properties can be engineered. Particularly, the band…

介观与纳米尺度物理 · 物理学 2019-11-13 Xiaobo Lu , Xiaoqin Li , Li Yang

Hybrid inorganic-organic semiconductor interfaces are of interest for new photovoltaic devices operating above the Shockley-Queisser limit. Predicting energy band alignment at the interfaces is crucial for their design, but represents a…

材料科学 · 物理学 2023-10-25 M. V. Klymenko , L. Z. Tan , S. P. Russo , J. H. Cole

We apply high-throughput DFT calculations and symbolic regression to hybrid inorganic/organic interfaces with the intent to extract physically meaningful correlations between the adsorption-induced work function modifications and the…

材料科学 · 物理学 2021-11-22 Johannes J. Cartus , Andreas Jeindl , Oliver T. Hofmann

The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of…

Transition metal dichalcogenides layered nano-crystals are emerging as promising candidates for next-generation optoelectronic and quantum devices. In such systems, the interaction between excitonic states and atomic vibrations is crucial…

介观与纳米尺度物理 · 物理学 2023-12-29 Jianbo Hu , Yang Xiang , Beatrice Matilde Ferrari , Emilio Scalise , Giovanni Maria Vanacore

MoS2 atomic layers have recently attracted much interest because of their two-dimensional structure as well as tunable optical, electrical, and mechanical properties for next generation electronic and electro-optical devices. Here we have…

We present a study by Scanning Tunneling Microscopy, supported by ab initio calculations, of the interaction between graphene and monolayer (semiconducting) PtSe$_2$ as a function of the twist angle ${\theta}$ between the two layers. We…

介观与纳米尺度物理 · 物理学 2023-12-22 P. Mallet , F. Ibrahim , K. Abdukayumov , A. Marty , C. Vergnaud , F. Bonell , M. Chshiev , M. Jamet , J-Y. Veuillen

In the past decade, photoemission orbital tomography (POT) has evolved into a powerful tool to investigate the electronic structure of organic molecules adsorbed on (metallic) surfaces. By measuring the angular distribution of…

Beyond-diffraction-limit optical absorption spectroscopy provides profound information on the graded band structures of composition-spread and stacked two-dimensional materials, in which direct/indirect bandgap, interlayer coupling,…

In this work electronic structures and optical properties of organic-inorganic exciton and polaritons in two-dimensional heterostructures combining both organic and semiconductor materials are studied. In those systems, Wannier-Frenkel…

介观与纳米尺度物理 · 物理学 2019-12-18 David W. Facemyer , Nguyen Que Huong

We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the…

介观与纳米尺度物理 · 物理学 2022-11-14 D. A. Baghdasaryan , E. S. Hakobyan , D. B. Hayrapetyan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

We present a mixed quantum-classical framework for the microscopic and non-Markovian modeling of exciton-phonon scattering in solid-state materials, and apply it to calculate the optical linewidths of monolayer MoS2. Within this framework,…

材料科学 · 物理学 2024-12-12 Alex Krotz , Roel Tempelaar

This paper deals with the study of the behaviour of the wave functions of a two-component Bose-Einstein condensate near the interface, in the case of strong segregation. This yields a system of two coupled ODE's for which we want to have…

偏微分方程分析 · 数学 2016-05-17 Amandine Aftalion , Christos Sourdis

Excitons in thin layers of semiconducting transition metal dichalcogenides are highly subject to the strongly modified Coulomb electron-hole interaction in these materials. Therefore, they do not follow the model system of a two-dimensional…

We investigate the molecular acceptors 3,4,9,10-perylene-tetracarboxylic acid dianhydride (PTCDA), 2,3,5,6-tetra uoro-7,7,8,8-tetracyanoquinodimethane (F4TCNQ), and 4,5,9,10-pyrenetetraone (PYTON) on Ag(111) using densityfunctional theory.…

材料科学 · 物理学 2015-06-17 Oliver T. Hofmann , Viktor Atalla , Nikolaj Moll , Patrick Rinke , Matthias Scheffler