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Correlated oxides, such as BiMnO$_3$ and LaMnO$_3$, show complex interplay of electronic correlations and crystal structure exhibiting multiple first order phase transitions, some without a clear order parameter. The quantitative…

强关联电子 · 物理学 2022-12-12 Gheorghe Lucian Pascut , Kristjan Haule

The kagome metals AV$_{3}$Sb$_{5}$ (A = K, Rb, Cs) provide a unique platform to investigate the physics of interacting electrons, a central challenge in condensed matter physics. A key obstacle in unraveling their correlated behavior is to…

The electronic structure of a LaNiO$_3$ bilayer grown along the [111] direction and confined between insulating layers of LaAlO$_3$ is theoretically investigated using a combination of first principle calculations and effective…

强关联电子 · 物理学 2012-06-28 Andreas Rüegg , Chandrima Mitra , Alexander A. Demkov , Gregory A. Fiete

The interface electronic structure of correlated LaTiO$_3$/SrTiO$_3$ superlattices is investigated by means of the charge self-consistent combination of the local density approximation (LDA) to density functional theory (DFT) with dynamical…

强关联电子 · 物理学 2013-06-07 Frank Lechermann , Lewin Boehnke , Daniel Grieger

Emergent magnetic states at oxide interfaces arise from the interplay of charge transfer, orbital reconstruction, and dimensional confinement, offering a route to engineered correlated-electron behavior in nanoscale spintronic materials.…

First-principles density functional theory calculations have been performed to understand the electronic structure and orbital polarization of LaNiO$_3$ with a reduced coordination and under strain. From the slab calculation to simulate…

材料科学 · 物理学 2011-10-03 Myung Joon Han , Michel van Veenendaal

The experimental observation that vanadate superlattices (LaVO$_3$)$_m$/SrVO$_3$ show ferromagnetism up to room temperature [U.\ L\"uders {\it et al.}, Phys.\ Rev.\ B {\bf 80}, 241102R (2009)] is investigated by means of density functional…

强关联电子 · 物理学 2016-12-13 Cosima Schuster , Ulrike Lueders , Udo Schwingenschloegl , Raymond Fresard

Through powder x-ray diffraction we have investigated the structural behavior of SmVO3, in which orbital and magnetic degrees of freedom are believed to be closely coupled to the crystal lattice. We have found, contrary to previous reports,…

We investigate the mechanism of the resonant X-ray scattering on the Ti $K$ edge region of YTiO$_3$ using the band structure calculation combined with the local density approximation. A large intensity is obtained for the orbital…

强关联电子 · 物理学 2007-05-23 Manabu Takahashi , Jun-ichi Igarashi

In complex oxide materials, changes in electronic properties are often associated with changes in crystal structure, raising the question of the relative roles of the electronic and lattice effects in driving the metal-insulator transition.…

强关联电子 · 物理学 2019-07-23 Alexandru B. Georgescu , Oleg E. Peil , Ankit Disa , Antoine Georges , Andrew J. Millis

Several puzzling aspects of interplay of the experimental lattice distortion and the the magnetic properties of four narrow $t_{2g}$-band perovskite oxides (YTiO$_3$, LaTiO$_3$, YVO$_3$, and LaVO$_3$) are clarified using results of…

强关联电子 · 物理学 2007-05-23 I. V. Solovyev

Using density functional theory we investigate the lattice instability and electronic structure of recently discovered ferroelectric metal LiOsO$_3$. We show that the ferroelectric-like lattice instability is related to the Li-O distortion…

材料科学 · 物理学 2015-03-19 Gianluca Giovannetti , Massimo Capone

The temperature dependence of the local structure of V_2O_3 in the vicinity of the metal to insulator transition (MIT) has been investigated using hard X-ray absorption spectroscopy. It is shown that the vanadium pair distance along the…

强关联电子 · 物理学 2009-11-11 P. Pfalzer , G. Obermeier , M. Klemm , S. Horn , M. L. denBoer

Oxygen packaging in transition metal oxides determines the metal-oxygen hybridization and electronic occupation at metal orbitals. Strontium vanadate (SrVO$_3$), having a single electron in a $3d$ orbital, is thought to be the simplest…

At interfaces between oxide materials, lattice and electronic reconstructions always play important roles in exotic phenomena. In this study, the density functional theory and maximally localized Wannier functions are employed to…

材料科学 · 物理学 2017-04-17 Yakui Weng , Jun-Jie Zhang , Bin Gao , Shuai Dong

In pursuit of rational control of orbital polarization, we present a combined experimental and theoretical study of single unit cell superlattices of the correlated metal LaNiO$_3$ and the band insulator LaAlO$_3$. Polarized x-ray…

强关联电子 · 物理学 2012-01-23 J. W. Freeland , Jian Liu , M. Kareev , B. Gray , J. W. Kim , P. Ryan , R. Pentcheva , J. Chakhalian

The diverse functionality emerging at oxide interfaces calls for a fundamental understanding of the mechanisms and control parameters of electronic reconstructions. Here, we explore the evolution of electronic phases in…

强关联电子 · 物理学 2015-01-19 David Doennig , Rossitza Pentcheva

Heterostructures of transition metal oxides (TMO) perovskites represent an ideal platform to explore exotic phenomena involving the complex interplay between the spin, charge, orbital and lattice degrees of freedom available in these…

The occupation of d-orbitals controls the magnitude and anisotropy of the inter-atomic electron transfer in transition metal oxides and hence exerts a key influence on their chemical bonding and physical properties. Atomic-scale modulations…

The application of modern layer-by-layer growth techniques to transition-metal oxide materials raises the possibility of creating new classes of materials with rationally designed correlated electron properties. An important step toward…

材料科学 · 物理学 2010-10-07 Myung Joon Han , Chris A. Marianetti , Andrew J. Millis
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