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Chiral molecules can selectively transport electrons of a particular spin orientation, yet the underlying mechanism remain poorly understood. Here, we present theoretical evidence that electrons propagating through chiral materials with…

材料科学 · 物理学 2024-03-01 Xiaoming Wang , Yeming Xian , Yanfa Yan

Chirality induced spin selectivity, discovered about two decades ago in helical molecules, is a non-equilibrium effect that emerges from the interplay between geometrical helicity and spin-orbit interactions. Several model Hamiltonians…

介观与纳米尺度物理 · 物理学 2019-11-13 J. Fransson

The elucidation of the mechanisms behind chiral-induced spin selectivity remains an outstanding scientific challenge. Here we consider the role of delocalised phonon modes in electron transport in chiral structures and demonstrate that spin…

介观与纳米尺度物理 · 物理学 2023-01-12 Clemens Vittmann , James Lim , Dario Tamascelli , Susana F. Huelga , Martin B. Plenio

Recent experiments have demonstrated the efficacy of chiral helically shaped molecules in polarizing the scattered electron spin, an effect termed as chiral-induced spin selectivity (CISS). Here we solve a simple tight-binding model for…

介观与纳米尺度物理 · 物理学 2016-02-03 Shlomi Matityahu , Yasuhiro Utsumi , Amnon Aharony , Ora Entin-Wohlman , Carlos A. Balseiro

We explicitly account for electron-electron interactions when modeling low-dimensional helical organic molecules. We show that competition between various hopping channels, together with interaction-induced double- and superexchange…

强关联电子 · 物理学 2026-05-29 Jacek Herbrych , Maria Daghofer

Chiral-induced spin selectivity (CISS) is a phenomenon in which electron spins are polarized as they are transported through chiral molecules, and the spin polarization depends on the handedness of the chiral molecule. In this study, we…

介观与纳米尺度物理 · 物理学 2023-02-09 Nguyen Thanh Phuc

The chirality-induced spin selectivity (CISS) effect gives rise to strongly spin-dependent transport through many organic molecules and structures. Its discovery raises fascinating fundamental questions as well as the prospect of possible…

介观与纳米尺度物理 · 物理学 2023-01-18 Dan Klein , Karen Michaeli

Chirality-induced spin selectivity is a spin-splitting phenomenon from a helical structure with a considerably effective spin-orbit coupling. This unexpectedly large spin-splitting phenomenon has been experimentally observed in chiral…

强关联电子 · 物理学 2024-05-08 Meng Xu , Yan Chen

This work investigates electron transport through chiral electrostatic potentials by modeling the system in three spatial dimensions and demonstrates that chirality-induced orbital selectivity (CIOS) produces pronounced enantiospecific…

介观与纳米尺度物理 · 物理学 2025-09-10 Namgee Cho , James Lim , Martin B. Plenio

The observation of spin-dependent transport through organic chiral structures has sparked numerous fundamental and applicative questions ranging from biology to spintronics. By now, there is a broad consensus that the effect results from…

介观与纳米尺度物理 · 物理学 2022-01-12 Lior Oppenheim , Karen Michaeli

Here we propose a mechanism by which spin polarization can be generated dynamically in chiral molecular systems undergoing photo-induced electron transfer. The proposed mechanism explains how spin polarization emerges in systems where…

介观与纳米尺度物理 · 物理学 2021-08-19 Thomas P. Fay , David T. Limmer

We present the first microscopic model for chirality-induced spin selectivity effect in electron-transfer, in which the internal degrees of freedom of the chiral bridge are explicitly included. By exactly solving this model on short chiral…

介观与纳米尺度物理 · 物理学 2024-10-08 A. Chiesa , E. Garlatti , M. Mezzadri , L. Celada , R. Sessoli , M. R. Wasielewski , R. Bittl , P. Santini , S. Carretta

A minimal model is exactly solved for electron spin transport on a helix. Electron transport is assumed to be supported by well oriented $p_z$ type orbitals on base molecules forming a staircase of definite chirality. In a tight binding…

介观与纳米尺度物理 · 物理学 2015-05-26 Ernesto Medina , Luis A. González-Arraga , Daniel Finkelstein-Shapiro , Bertrand Berche , Vladimiro Mujica

Chiral molecules are known to preferentially select electrons with a particular spin state, an effect termed chirality-induced spin selectivity (CISS). In this work, the transient CISS dynamics in a chiral molecule are investigated through…

介观与纳米尺度物理 · 物理学 2025-11-03 Riley Stuermer , Collin VanEssen , Jacob Byers , Keith Ferrer , Prasad Gudem , Diego Kienle , Jonas Fransson , Mani Vaidyanathan

The chiral-induced spin selectivity (CISS) effect, a phenomenon where the chirality of molecules imparts significant spin selectivity to electron transfer processes, has garnered increasing interest among the chemistry, biology, and physics…

化学物理 · 物理学 2025-09-05 Tian-Yi Zhang , Yue Mao , Ai-Min Guo , Qing-Feng Sun

Chirality-induced spin selectivity (CISS) has been extensively studied over the past two decades. While current-induced spin polarization in chiral molecules is widely recognized as the fundamental principle of the CISS, only a few studies…

材料科学 · 物理学 2023-08-25 Kouta Kondou , Shinji Miwa , Daigo Miyajima

Chiral induced spin selectivity is a phenomenon that has been attributed to chirality, spin-orbit interactions, and non-equilibrium conditions, while the role of electron exchange and correlations have been investigated only marginally…

介观与纳米尺度物理 · 物理学 2021-04-28 J. Fransson

Highly spin selective transport of electrons through a helically shaped electrostatic potential is demonstrated in the frame of a minimal model approach. The effect is significant even in the case of weak spin-orbit coupling. Two main…

介观与纳米尺度物理 · 物理学 2015-05-30 R. Gutierrez , E. Diaz , R. Naaman , G. Cuniberti

The observation of spin-dependent transmission of electrons through chiral molecules has led to the discovery of chiral-induced spin selectivity (CISS). The remarkably high efficiency of the spin polarizing effect has recently gained…

Chirality-induced spin selectivity (CISS) generates spin-polarized currents in nonmagnetic materials from structural chirality alone, yet its microscopic origin remains debated. Using a first-principles spatiotemporal density-matrix…

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