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Interatomic Coulombic decay (ICD) plays a crucial role in weakly bound complexes exposed to intense or high-energy radiation. So far, neutral or ionic atoms or molecules have been prepared in singly excited electron or hole states which can…

An ultrafast mechanism belonging to the family of interatomic Coulombic decay (ICD) phenomena is proposed. When two excited species are present, an ultrafast energy transfer can take place bringing one of them to its ground state and…

When weakly-bound complexes are multiply excited by intense electromagnetic radiation, energy can be exchanged between neighboring atoms through a type of resonant interatomic Coulombic decay (ICD). This decay mechanism due to multiple…

The electron removal and excitation channels in argon dimer target and helium ion projectile collision systems that facilitate interatomic Coulombic decay (ICD) are investigated. We implement an independent-atom and independent-electron…

原子与分子团簇 · 物理学 2026-03-25 Darij Starko , Tom Kirchner

We examine the possible control of the celebrated Purcell effect in cavity quantum electrodynamics. We demonstrate that the presence of an unexcited atom can significantly alter the Purcell decay depending on the strength of coupling of the…

量子物理 · 物理学 2024-04-03 G. S. Agarwal

As opposed to purely molecular systems where electron dynamics proceed only through intramolecular processes, weakly bound complexes such as He droplets offer an environment where local excitations can interact with neighbouring embedded…

原子与分子团簇 · 物理学 2021-04-15 A. C. LaForge , M. Shcherbinin , F. Stienkemeier , R. Richter , R. Moshammer , T. Pfeifer , M. Mudrich

During the last 15 years a novel decay mechanism of excited atoms has been discovered and investigated. This so called ''Interatomic Coulombic Decay'' (ICD) involves the chemical environment of the electronically excited atom: the…

To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic…

原子与分子团簇 · 物理学 2012-01-04 Philipp V. Demekhin , Spas D. Stoychev , Alexander I. Kuleff , Lorenz S. Cederbaum

When a vacancy is created in an inner-valence orbital of a dimer of atoms or molecules, the resulting species can undergo interatomic/intermolecular Coulombic decay (ICD): the hole is filled through a relaxation process that leads to a…

化学物理 · 物理学 2023-05-18 Valentina Parravicini , Thomas-C. Jagau

The increased decay rate of a two-level system weakly coupled to an optical cavity, known as the Purcell effect, is a cornerstone of cavity QED. However, the effect of cavity coupling is not well understood if the two-level system is…

量子物理 · 物理学 2023-06-19 Charlie Nation , Valentina Notararigo , Alexandra Olaya-Castro

Using neon and its dimer as a specific example, it is shown that excited Auger decay channels that are electronically stable in the isolated monomer can relax in a cluster by electron emission. The decay mechanism, leading to the formation…

原子与分子团簇 · 物理学 2009-11-10 Robin Santra , Lorenz S. Cederbaum

Excited atoms and molecules can utilize their excess energy to ionize a neighboring system by a process named interatomic and intermolecular Coulombic decay (ICD). ICD is ultrafast, in the femtosecond regime, and has many modes of…

化学物理 · 物理学 2026-03-10 Alan G. Falkowski , Alexander I. Kuleff , Lorenz S. Cederbaum

Interatomic coulombic decay (ICD) is a relaxation process induced by electronic correlation. In this work we study the ICD process in a two coupled Quantum wells (QWs) nano-structure. We study a simple one-dimensional effective potential…

介观与纳米尺度物理 · 物理学 2015-06-11 Tamar Goldzak , Liron Gantz , Ido Gilary , Gad Bahir , Nimrod Moiseyev

Two-atom systems in small traps are of fundamental interest, first of all for understanding the role of interactions in degenerate cold gases and for the creation of quantum gates in quantum information processing with single-atom traps.…

The recent availability of intense and ultrashort extreme ultraviolet sources opens the possibility to investigate ultrafast electronic relaxation processes in matter in an unprecedented regime. In this work we report on the observation of…

Within the framework of master equation, we study decay dynamics of an atom-molecule system strongly coupled by two photoassociation lasers. Summing over the infinite number of electromagnetic vacuum modes that are coupled to the…

原子物理 · 物理学 2014-05-23 Arpita Rakshit , Saikat Ghosh , Bimalendu Deb

Strong Coulomb interactions in two-dimensional systems, together with quantum confinement, make many-body processes particularly effective for carrier dynamics, which plays a crucial role in determining carrier lifetime, photoconductivity,…

介观与纳米尺度物理 · 物理学 2022-02-01 Di Li , Wenjie Zhang , Peng Suo , Jiaming Chen , Kaiwen Sun , Yuqin Zou , Hong Ma , Xian Lin , Xiaona Yan , Saifeng Zhang , Bo Li , Guohong Ma

Standard cavity cooling of atoms or dielectric particles is based on the action of dispersive optical forces in high-finesse cavities. We investigate here a complementary regime characterized by large cavity losses, resembling the standard…

量子物理 · 物理学 2024-08-21 Julian Lyne , Nico S. Bassler , Seong eun Park , Guido Pupillo , Claudiu Genes

We investigate theoretically the collective radiance characteristics of an atomic ensemble with the simultaneous decay of two atoms. We show that the two-atom decay can significantly suppress the steady-state collective radiance of the…

量子物理 · 物理学 2022-12-21 Qian Bin , Xin-You Lü

Interatomic Coulombic decay (ICD) is a mechanism which allows microscopic objects to rapidly exchange energy. When the two objects are distant, the energy transfer between the donor and acceptor species takes place via the exchange of a…

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