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We have investigated multiphoton multiple ionization dynamics of argon and xenon atoms using a new x-ray free electron laser (XFEL) facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that highly charged…

We present a multichannel photoelectron interferometry technique based on trichromatic pulse shaping for unambiguous determination of quantum phases in multiphoton ionization (MPI) of potassium atoms. The colors of the laser field are…

原子物理 · 物理学 2022-05-25 K. Eickhoff , D. Köhnke , L. Feld , T. Bayer , M. Wollenhaupt

High-resolution photoelectron momentum distributions of Xe atoms ionized by 800-nm linearly polarized laser fields have been traced at intensities from 1.1*1013 to 3.5*1013W/cm2 using velocity-map imaging techniques. At certain laser…

原子物理 · 物理学 2015-12-09 Min Li , Peng Zhang , Siqiang Luo , Yueming Zhou , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We report the observation of multiple ionization of Argon through multi-XUV-photon absorption induced by an unprecedentedly powerful laser driven high-harmonic-generation source. Comparing the measured intensity dependence of the yield of…

Resonance-enhanced multiphoton ionization (REMPI) is a widely used technique for studying molecular photoionization and producing molecular cations for spectroscopy and dynamics studies. Here, we present a model for describing…

化学物理 · 物理学 2016-08-24 Matthias Germann , Stefan Willitsch

In this paper, we theoretically study x-ray multiphoton ionization dynamics of heavy atoms taking into account relativistic and resonance effects. When an atom is exposed to an intense x-ray pulse generated by an x-ray free-electron laser…

原子物理 · 物理学 2017-04-26 Koudai Toyota , Sang-Kil Son , Robin Santra

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

Resonance-enhanced multiphoton ionization (REMPI) in potassium atom is investigated within the strong coupling regime using photoelectron momentum imaging techniques. The kinetic energy distribution of the ionized electrons reveals the…

原子物理 · 物理学 2025-03-10 Wankai Li , Yixuan Wang , Xing Li , Tao Yang , Dongdong Zhang , Dajun Ding

Using Resonant Pulsed Rydberg Field-ionization (RPRFI) technique, we generate low-energy electron bunches at high repetition rates. By combining continuous-wave laser excitation with a pulsed electric field, this method selectively ionizes…

原子物理 · 物理学 2024-01-10 R. Hahn , D. Comparat

A simple model for sequential multiphoton ionization by ultra-intense x-rays is presented. The derived scaling of the ion yield with pulse energy quantitatively reproduces the experimental data, which shows that the ion yield increases…

原子物理 · 物理学 2021-09-29 Xiang Li , Rebecca Boll , Daniel Rolles , Artem Rudenko

We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are…

The production of high-quality electron bunches in Laser Wake Field Acceleration relies on the possibility to inject ultra-low emittance bunches in the plasma wave. In this paper we present a new bunch injection scheme in which electrons…

We theoretically study the process of photoelectron emission of the Helium atom by a high-intensity short-wavelength laser at a resonance condition of the residual singly charged ion. Photoionization followed by strong resonance coupling in…

原子物理 · 物理学 2014-01-14 Song Bin Zhang , Nina Rohringer

Recently a new injection scheme for Laser Wake Field Acceleration, employing a single 100-TW-class laser system, has been proposed. In the Resonant Multi-Pulse Ionization injection (ReMPI) a resonant train of pulses drives a large amplitude…

加速器物理 · 物理学 2018-12-26 P. Tomassini , S. De Nicola , L. Labate , P. Londrillo , R. Fedele , D. Terzani , F. Nguyen , G. Vantaggiato , L. A. Gizzi

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

We report on efficient rovibrational state-selective loading of single H$_2^+$ molecular ions into a cryogenic linear Paul trap using (2+1) resonance-enhanced multi-photon ionization (REMPI). The H$_2^+$ ions are created by resonant…

原子物理 · 物理学 2026-05-05 Ho June Kim , Fabian Schmid , David Holzapfel , Daniel Kienzler

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

原子物理 · 物理学 2015-05-27 C. Müller , A. B. Voitkiv

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light-matter interaction was, so far, not studied…

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

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