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Double ionization of an atom by single-photon absorption in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly to the other atom,…

原子物理 · 物理学 2020-02-19 A. Eckey , A. B. Voitkiv , C. Müller

We propose a new scheme to control the shape of the Autler-Townes (AT) doublet in the photoelectron spectrum from atomic resonance-enhanced multiphoton ionization (REMPI). The scheme is based on the interference of two AT doublets created…

原子物理 · 物理学 2025-07-01 T. Bayer , K. Eickhoff , D. Köhnke , M. Wollenhaupt

Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…

原子物理 · 物理学 2009-10-30 D. Bauer

We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of…

The spectrum of electronic states at 30000--33000 cm$^{-1}$ in hafnium fluoride has been studied using (1+1) resonance-enhanced multi-photon ionization (REMPI) and (1+1$'$) REMPI. Six $\Omega' = 3/2$ and ten $\Pi_{1/2}$ vibronic bands have…

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

Multiphoton ionization provides a clear window into the nature of electron correlations in the helium atom. In the present study, the final state energy range extends up to the region near the $N=2$ and $N=3$ ionization thresholds, where…

原子物理 · 物理学 2021-03-10 Yimeng Wang , Chris H. Greene

Relativistic and resonance effects in the photoionization of Mg-like Fe~XV are investigated using the Breit-Pauli R-matrix Method (BPRM) at near-threshold and intermediate energies, complemented by the Relativistic Random Phase…

天体物理学 · 物理学 2009-10-31 Nasreen Haque , Anil K. Pradhan

We present a joint experimental and theoretical study on strong-field photo-ionization of sodium atoms using chirped femtosecond laser pulses. By tuning the chirp parameter, selectivity among the population in the highly excited states 5p,…

原子物理 · 物理学 2015-05-28 M Krug , T Bayer , M Wollenhaupt , C Sarpe-Tudoran , T Baumert , S S Ivanov , N V Vitanov

Photoionization of an atom via interatomic correlations to N neighboring atoms may be strongly enhanced due to constructive interference of quantum pathways. The ionization proceeds via resonant photoexcitation of a neighbor atom and…

原子物理 · 物理学 2015-05-30 Carsten Müller , Mihai A. Macovei , Alexander B. Voitkiv

Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller…

原子物理 · 物理学 2015-06-04 B. Najjari , C. Müller , A. B. Voitkiv

We present an experimental study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral argon atoms. Using 9.3 eV photons produced via high harmonic generation and a 3-D momentum imaging…

原子物理 · 物理学 2020-08-28 Kirk A. Larsen , Daniel S. Slaughter , Thorsten Weber

Resonances leave prominent signatures in atomic and molecular ionization triggered by the absorption of single or multiple photons. These signatures reveal various aspects of the ionization process, characterizing both the initial and final…

原子物理 · 物理学 2026-03-03 Anatoli S. Kheifets

We consider the process of double photoionization (DPI) in a rare gas atom as a two-step process, namely (i) photoionization in an inner shell followed by (ii) the emission of an Auger electron from an outer shell. An angular correlation…

原子物理 · 物理学 2009-11-07 Dipankar Chattarji , Chiranjib Sur

A method is suggested to produce, with the help of colliding laser photons with bunches of relativistic ions having two energy levels, both intense beams of monochromatic polarized X-ray fluorescence photons and significant number of X-ray…

高能物理 - 实验 · 物理学 2010-04-05 K. A. Ispirian , M. K. Ispiryan

Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…

原子物理 · 物理学 2022-02-24 A. Plunkett , M. A. Alarcon , J. K. Wood , C. H. Greene , A. Sandhu

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

原子物理 · 物理学 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

Fano resonances are ubiquitous phenomena appearing in many fields of physics, e.g. atomic or molecular photoionization, or electron transport in quantum dots. Recently, attosecond interferometric techniques have been used to measure the…

The ability to prepare molecular ions in selected quantum states enables studies in areas such as chemistry, metrology, spectroscopy, quantum information, and precision measurements. Here, we demonstrate $(2+1)$ resonance-enhanced…