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From the high vibrational dipolar strength offered by molecular liquids, we demonstrate that a molecular vibration can be ultra-strongly coupled to multiple IR cavity modes, with Rabi splittings reaching $24\%$ of the vibration frequencies.…

The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this…

Planar microcavity polaritons have recently emerged as a promising technology for improving several performance characteristics of organic light-emitting diodes, photodiodes and photovoltaics. To form polaritons and achieve enhanced…

Two-dimensional (2D) semiconducting microcavity, where exciton-polaritons can be formed, constitues a promising setup for exploring and manipulating various regimes of light-matter interaction. Here, the coupling between 2D excitons and…

材料科学 · 物理学 2021-09-08 Dino Novko , Vito Despoja

Vibrational polaritons form in a planar Fabry-Perot microcavity when a vibrational mode of a layer of molecules is near resonant with an infrared cavity mode. Herein, dispersion relations of vibrational polaritons are studied when the…

化学物理 · 物理学 2024-06-18 Tao E. Li

The strong coupling regime is observed in a system of two-dimensional electrons whose cyclotron motion is coupled to an electro-magnetic mode in a Fabry-Perot cavity resonator. The Rabi splitting of eigenfrequencies of coupled motion is…

介观与纳米尺度物理 · 物理学 2016-07-28 L. V. Abdurakhimov , R. Yamashiro , A. O. Badrutdinov , D. Konstantinov

Strong cavity coupling of gas-phase molecules will enable studies of benchmark chemical processes under strong light-matter interactions with a high level of experimental control and no solvent effects. We recently demonstrated the…

化学物理 · 物理学 2023-10-26 Adam D. Wright , Jane C. Nelson , Marissa L. Weichman

We report the experimental observation of collective multi-mode vacuum Rabi splitting in free space. In contrast to optical cavities, the atoms couple to a continuum of modes, and the optical thickness of the cloud provides a measure of…

We report on the strong coupling between the Bloch surface wave supported by an inorganic multilayer structure and $J$-aggregate excitons in an organic semiconductor. The dispersion curves of the resulting polariton modes are investigated…

We propose a cavity QED approach to describe light-matter interaction between an individual anharmonic molecular vibration and an infrared cavity field. Starting from a generic Morse oscillator with quantized nuclear motion, we derive a…

化学物理 · 物理学 2019-10-16 Federico Hernández , Felipe Herrera

A single nanotube synthesized from a transition metal dichalcogenide (TMDC) exhibits strong exciton resonances and, in addition, can support optical whispering gallery modes. This combination is promising for observing exciton-polaritons…

介观与纳米尺度物理 · 物理学 2024-01-17 A. I. Galimov , D. R. Kazanov , A. V. Poshakinskiy , M. V. Rakhlin , I. A. Eliseyev , A. A. Toropov , M. Remskar , T. V. Shubina

We demonstrate room-temperature strong-coupling between a mid-infrared ($\lambda$=9.9 $\mu$m) intersubband transition and the fundamental cavity mode of a metal-insulator-metal resonator. Patterning of the resonator surface enables…

We develop a microscopic theory for the multimode polariton dispersion in materials coupled to cavity radiation modes. Starting from a microscopic light-matter Hamiltonian, we devise a general strategy for obtaining simple matrix models of…

材料科学 · 物理学 2023-05-09 Arkajit Mandal , Ding Xu , Ankit Mahajan , Joonho Lee , Milan E. Delor , David R. Reichman

Strong coupling between cavity photons and molecular vibrations can lead to the formation of vibron-polaritons. In a recent experiment with PVAc molecules in a metal-metal microcavity [A.Shalabney et al., Ang.Chem.Int.Ed. 54 7971 (2015)],…

光学 · 物理学 2016-08-31 Artem Strashko , Jonathan Keeling

Polaritons are usually described within single-mode cavity QED models. However, nanophotonic environments typically involve several modes that spectrally overlap and interfere, giving rise to sharp dip features such as Fano profiles in the…

We have achieved a significant experimental Rabi-splitting (3.4 meV) for confined polaritons in a planar semiconductor $\lambda$ microcavity for only a single quantum well (SQW) of GaAs (10 nm) placed at the antinode. The Rabi-splitting…

介观与纳米尺度物理 · 物理学 2014-07-10 E. A. Cotta , P. M. S. Roma

We study the use of exciton-polaritons in semiconductor microcavities to generate radiation spanning the infrared to terahertz regions of the spectrum by exploiting transitions between upper and lower polariton branches. The process, which…

光学 · 物理学 2015-09-23 Fábio Barachati , Simone De Liberato , Stéphane Kéna-Cohen

We demonstrate Resonant Tunneling Diodes, embedded in double metal cavities, strongly coupled to the cavity field, while maintaining their electronic properties. We measure the polariton dispersion and find a relative vacuum Rabi splitting…

Two-dimensional transition metal dichalcogenides exhibit strong optical transitions with significant potential for optoelectronic devices. In particular they are suited for cavity quantum electrodynamics in which strong coupling leads to…

We investigate the demonstration and quantification of the strong coupling between excitons and guided photons in a GaN slab waveguide. The dispersions of waveguide polaritons are measured from T=6~K to 300~K through gratings. They are…

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