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相关论文: Mn ions' site and valence in PbTiO$_{3}$ based on …

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Mn is used as a dopant to improve the electromechanical properties of perovskite oxides. We elucidate the role of Mn defects and associated vacancies on the electronic, atomic and ferroelectric properties of BaTiO$_3$. Using density…

材料科学 · 物理学 2014-12-24 J. F. Nossa , Ivan I. Naumov , R. E. Cohen

Doping Bi$_2$Se$_3$ by magnetic ions represents an interesting problem since it may break the time reversal symmetry needed to maintain the topological insulator character. Mn dopants in Bi$_2$Se$_3$ represent one of the most studied…

材料科学 · 物理学 2020-02-26 K. Carva , P. Baláž , J. Šebesta , I. Turek , J. Kudrnovský , F. Máca , V. Drchal , J. Chico , V. Sechovský , J. Honolka

We present a computational study of PbCoO$_3$ at ambient and elevated pressure. We employ the static and dynamic treatment of local correlation in form of density functional theory + $U$ (DFT+$U$) and + dynamical mean-field theory…

强关联电子 · 物理学 2021-12-03 Atsushi Hariki , Kyo-Hoon Ahn , Jan Kuneš

We study Mn substitution for Ti in BaTiO3 with and without compensating oxygen vacancies using density functional theory (DFT) in combination with dynamical mean field theory (DMFT). We find strong charge and spin fluctuations. Without…

材料科学 · 物理学 2018-09-12 Subhasish Mandal , R. E. Cohen , K. Haule

Structure, transport and magnetic properties have been investigated for layered NaCo1-xMnxO2 materials. With the increase of Mn-doping amount, measurements of x-ray diffraction indicate that the in-plane lattice parameter a decreases…

强关联电子 · 物理学 2007-05-23 W. Y. Zhang , H. C. Yu , Y. G. Zhao , X. P. Zhang , Y. G. Shi , Z. H. Cheng , J. Q. Li

The magnetic lattice of mixed-valence Mn ions in La$_{0.7}$Sr$_{0.3}$MnO$_3$ is selectively diluted by partial substitution of Mn by Al or Ti. The ferromagnetic transition temperature and the saturation moment decreases with substitution in…

材料科学 · 物理学 2009-11-11 D. N. H. Nam , L. V. Bau , N. V. Khiem , N. V. Dai , L. V. Hong , N. X. Phuc , R. S. Newrock , P. Nordblad

Transition metals (TMs) implanted in oxides with rock-salt crystal structures (for example MgO and BaO) are assumed to substitute cations (Mg in case of MgO) from the lattice sites. We show that not all implanted TMs substitute cations but…

材料科学 · 物理学 2019-03-14 Debolina Misra , Satyesh K. Yadav

We have carried out \textit{ab-initio} calculations of local structure of Mn and Ni in Mn$_{2}$Ni$_{1.5}$In$_{0.5}$ alloy with different site occupancies in order to understand the similarities in martensitic and magnetic properties of…

材料科学 · 物理学 2017-01-31 D. N. Lobo , K. R. Priolkar , A. Koide , S. Emura

The magnetic lattice of mixed-valence Mn ions in La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ is selectively diluted by partial substitution of Al or Ti for Mn. The ferromagnetic transition temperature $T_\mathrm{c}$ and the saturation magnetization…

材料科学 · 物理学 2015-05-13 D. N. H. Nam , N. V. Dai , L. V. Hong , N. X. Phuc , L. V. Bau , P. Nordblad , R. S. Newrock

We present a first-principles study of the electronic, magnetic, and transport properties of the topological insulator Bi$_{2}$Te$_{3}$ doped with Mn atoms in substitutional (Mn$_{\rm Bi}$) and interstitial van der Waals gap positions…

材料科学 · 物理学 2016-06-15 K. Carva , J. Kudrnovský , F. Máca , V. Drchal , I. Turek , P. Baláž , V. Tkáč , V. Holý , V. Sechovský , J. Honolka

The local environment and oxidation state of Mn impurity in strontium titanate doped with 3% Mn were studied by X-ray absorption fine structure spectroscopy. The influence of the preparation conditions on the incorporation of the impurity…

材料科学 · 物理学 2015-07-28 I. A. Sluchinskaya , A. I. Lebedev , A. Erko

P mono-doped and (P, N) co-doped ZnO are investigated by the first-principles calculations. It is found that substitutive P defect forms a deep acceptor level at O site (PO) and it behaves as a donor at Zn site (PZn), while interstitial P…

材料科学 · 物理学 2015-05-13 Ren-Yu Tian , Yu-Jun Zhao

ZnO is co-doped with Na+ and Si4+ in the ratio 2:1. The ratio was intentionally chosen so that net valence state of dopant theoretically matches that of host. This is to avoid dependence in the amount of oxygen vacancies/interstitials…

Combining experiments with first principles calculations, we show that site-specific doping of Mn into SrTiO3 has a decisive influence on the dielectric properties of these doped systems. We find that phonon contributions to the dielectric…

We report a detailed first-principles study of doping in Li$_2$MnO$_3$, in both the dilute doping limit and heavy doping, using hybrid density-functional calculations. We find that Al, Fe, Mo, and Ru impurities are energetically most…

材料科学 · 物理学 2017-12-07 Khang Hoang

To understand the interaction between nitrogen dopants and native point defects in graphene, we have studied the energetic stability of N-doped graphene with vacancies and Stone-Wales (SW) defect by performing the density functional theory…

介观与纳米尺度物理 · 物理学 2012-05-03 Zhufeng Hou , Xianlong Wang , Takashi Ikeda , Kiyoyuki Terakura , Masaharu Oshima , Masa-aki Kakimoto , Seizo Miyata

Dopability in semiconductors plays a crucial role in device performance. Using the first-principles density-functional theory calculations, we investigate systematically the doping properties of layered MX2 (M= Mo, W; X=S, Te) by replacing…

材料科学 · 物理学 2018-04-27 Dan Guo , Kaike Yang , Tao Shen , Jin Xiao , Li-Ming Tang , Zhongming Wei , Guanghui Zhou , Hui-Xiong Deng

Mn site is substituted with closed shell ions (Al, Ga. Ti, Zr and a certain combination of Zr and Al) and also with Fe and Ru ions carrying the magnetic moment (S=5/2 and 2 respectively) at a fixed concentration of 5 at. %. Substitution did…

强关联电子 · 物理学 2007-05-23 L. Seetha Lakshmi , V. Sridharan , D. V. Natarajan , V. Sankara Sastry , T. S. Radhakrishnan

La1-xCaxMnO3+delta and La1-xNaxMnO3+delta samples with well defined cation molecularity and oxygen contents are analyzed with XRPD, electrical conductivity, electron paramagnetic resonance and static magnetization measurements. Point…

The development of ferromagnetism in Mn-doped Bi2Te3 is characterized through measurements on a series of single crystals with different Mn content. Scanning tunneling microscopy analysis shows that the Mn substitutes on the Bi sites,…

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