相关论文: Frustrated tunneling dynamics in ultrashort laser …
By employing two-color counter-rotating circularly polarized laser fields, we investigate the dynamics of electron recapture into Rydberg states under strong, ultrashort laser pulses, probed via coherent extreme-ultraviolet free-induction…
We present both full quantum mechanical and semiclassical calculations of above threshold ionization (ATI) of a hydrogen atom in the tunneling regime by a few-cycle linearly polarized infrared laser pulse. As a quantum treatment, we applied…
Tunneling ionization followed by strong-field excitation leads to important ultrafast phenomena such as charge migration and lasing. Recent theoretical developments suggest that the population of the ionic excited state can be greatly…
Classically allowed transport is shown to compete with quantum tunneling during the ionization of atoms by ultrashort and intense laser pulses, despite Keldysh parameters smaller than unity. This is done by comparing exact probability…
By using a state of art tensor network state method, we study the ground-state phase diagram of an extended Bose-Hubbard model on the square lattice with frustrated next-nearest neighboring tunneling. In the hardcore limit, tunneling…
Tunneling ionization of an atom in ultrashort laser pulses is considered. When the driving laser pulse is switched-on and -off with a steep slope, the photoelectron momentum distribution (PMD) shows an edge-effect because of the…
Excited electronic states of molecules and solids play a fundamental role in fields such as catalysis and electronics. In electronic structure calculations, excited states typically correspond to saddle points on the surface described by…
Semiclassical methods are extremely important in the subjects of wave packet and coherent state dynamics. Unfortunately, these essentially saddle point approximations are considered nearly impossible to carry out in detail for systems with…
We formulate a three-dimensional semi-classical model to treat three-electron escape dynamics in a strongly-driven linear triatomic molecule, HeH$_{2}^{+}$. Our model includes the Coulomb singularities. Hence, to avoid unphysical…
We have investigated photoionization of Ne$^+$ in the combined field of a short infra-red laser pulse and a delayed ultra-short pulse of the infra-red laser's 23$^r$$^d$ harmonic. We observe an ionization yield compatible with a picture in…
We theoretically investigate tunneling through free-space or dielectric nanogaps between metallic nanocontacts driven by ultrashort ultrabroadband light pulses. For this purpose we develop a time-dependent quasiclassical theory being…
The yield of neutral excited atoms and low-energy photoelectrons generated by the electron dynamics in the combined Coulomb and laser field after tunneling is investigated. We present results of Monte-Carlo simulations built on the two-step…
The tunneling model of ionization applies only to longitudinal fields: quasistatic electric fields that do not propagate. Laser fields are transverse: plane wave fields that possess the ability to propagate. Although there is an approximate…
In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…
The present work explores quantitative limits to the Single-Active Electron (SAE) approximation, often used to deal with strong-field ionization and subsequent attosecond dynamics. Using a time-dependent multi\-configuration approach,…
We report on the measurement of electron emission after the interaction of strong laser pulses with atoms and molecules. These electrons originate from high-lying Rydberg states with quantum numbers up to $n \lesssim 120$ formed by…
Solving the time-dependent Schr\"odinger equation (TDSE) is pivotal for modeling non-adiabatic electron dynamics, a key process in ultrafast spectroscopy and laser-matter interactions. However, exact solutions to the TDSE remain…
Variational calculations of excited electronic states are carried out by finding saddle points on the surface that describes how the energy of the system varies as a function of the electronic degrees of freedom. This approach has several…
We theoretically study frustrated double ionization (FDI) of atoms subjected to intense circularly polarized laser pulses using a three-dimensional classical model. We find a novel "knee" structure of FDI probability as a function of…
Population dynamics in weakly-excited clouds of ultracold $^{87}$Rb Rydberg atoms were studied by means of trap loss, fluorescence detection, and state dependent stimulated emission. Rydberg atoms were excited to various nl Rydberg states…