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Semiconducting single-walled carbon nanotubes show extraordinary electronic and optical properties, such as high charge carrier mobilities and diameter-dependent near-infrared photoluminescence. The introduction of sp3 defects in the carbon…

光学 · 物理学 2021-11-10 Jana Zaumseil

Near-infrared electroluminescence from carbon-based emitters, especially in the second biological window (NIR-II) or at telecommunication wavelengths, is difficult to achieve. Single-walled carbon nanotubes (SWCNTs) have been proposed as a…

The functionalization of semiconducting single-wall carbon nanotubes (SWCNTs) with luminescent sp$^{3}$ defects creates red-shifted emission features in the near-infrared and boosts their photoluminescence quantum yields (PLQYs). While…

The covalent functionalization of single-walled carbon nanotubes (SWNTs) with luminescent oxygen defects increases their brightness and enables their application as optical biosensors or fluorescent probes for in-vivo imaging in the…

Single-walled carbon nanotubes have advantages as a nanoscale light source compatible with silicon photonics because they show room-temperature luminescence at telecom-wavelengths and can be directly synthesized on silicon substrates. Here…

介观与纳米尺度物理 · 物理学 2013-04-24 S. Imamura , R. Watahiki , R. Miura , T. Shimada , Y. K. Kato

Diazonium reactions with carbon nanotubes form optical $sp^3$ defects that can be used in optical and electrical circuits. We investigate a direct on-device reaction supported by confined laser irradiation and present a technique where an…

介观与纳米尺度物理 · 物理学 2022-05-19 Georgy Gordeev , Thomas Rosenkranz , Frank Hennrich , Stephanie Reich , Ralph Krupke

Quantum light sources using single-walled carbon nanotubes show promise for quantum technologies but face challenges in achieving precise control over color center formation. Here we present a novel technique for deterministic creation of…

材料科学 · 物理学 2025-09-15 Daichi Kozawa , Yuto Shiota , Yuichiro K. Kato

Azide functionalization produced luminescent sp2-type defects on single-walled carbon nanotubes, by which defect photoluminescence appeared in near infrared regions (1116 nm). Changes in exciton properties were induced by localization…

Oxygen defects in semiconducting single-walled carbon nanotubes (SWCNTs) are localized disruptions in the carbon lattice caused by the formation of epoxy or ether groups, commonly through wet-chemical reactions. The associated modifications…

应用物理 · 物理学 2024-02-09 Sonja Wieland , Abdurrahman Ali El Yumin , Simon Settele , Jana Zaumseil

The covalent functionalization of single-walled carbon nanotubes (SWCNTs) with luminescent quantum defects enables their application as near-infrared single-photon sources, as optical sensors, and for in-vivo tissue imaging. Tuning the…

The functionalization of single-walled carbon nanotubes (SWCNTs) with luminescent sp$^{3}$ defects has greatly improved their performance in applications such as quantum light sources and bioimaging. Here, we report the covalent…

Carbon nanotubes are a good realization of one-dimensional crystals where basic science and potential nanodevice applications merge. Defects are known to modify the electrical resistance of carbon nanotubes. They can be present in as-grown…

The functionalization of semiconducting single-walled carbon nanotubes (SWNTs) with sp$^{3}$ defects that act as luminescent exciton traps is a powerful means to enhance their photoluminescence quantum yield (PLQY) and to add optical…

We identify a class of covalent functionalizations that preserves or controls the conductance of single-walled metallic carbon nanotubes. [2+1] cycloadditions can induce bond cleaving between adjacent sidewall carbons, recovering in the…

材料科学 · 物理学 2009-11-11 Young-Su Lee , Nicola Marzari

Photonic integrated circuits require robust room-temperature single-photon sources to enable scalable quantum technologies. Single-walled carbon nanotubes (CNTs), with their unique excitonic properties and chemical tunability, are…

The controlled introduction of covalent sp$^{3}$ defects into semiconducting single-walled carbon nanotubes (SWCNTs) gives rise to exciton localization and red-shifted near-infrared luminescence. The single-photon emission characteristics…

材料科学 · 物理学 2022-06-22 Wenhao Zheng , Nicolas F. Zorn , Mischa Bonn , Jana Zaumseil , Hai I. Wang

Inorganic pyrophosphate is a key molecule in many biological processes from DNA synthesis to cell metabolism. Here we introduce sp$^{3}$-functionalized (6,5) single-walled carbon nanotubes (SWNTs) with red-shifted defect emission as…

The extraordinary one-dimensional properties of carbon nanotubes have captivated scientists and engineers since their discovery in the early 1990s. In particular, semiconducting single-wall carbon nanotubes (SWCNTs) are highly promising for…

应用物理 · 物理学 2026-04-09 Ting-Wei Chang , Gustavo M. Rodriguez-Barrios , Andrey Baydin , Junichiro Kono

Single-Wall Carbon Nanotubes (SWNTs) are among the very few candidates for single-photon sources operating in the telecom bands since they exhibit large photon antibunching up to room temperature. However, coupling a nanotube to a photonic…

Semiconducting single-walled carbon-nanotubes (SWCNTs) are an interesting material for strong-light matter coupling due to their stable excitons, narrow emission in the near infrared and high charge carrier mobilities. Furthermore, they…

材料科学 · 物理学 2021-03-17 Jan M. Lüttgens , Felix J. Berger , Jana Zaumseil
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