相关论文: Ultrafast Fluorescence Depolarization in Conjugate…

We analyse various phonon-assisted mechanisms which contribute to the decoherence of excitonic qubits in quantum dot systems coupled by the F\"orster-type transfer process. We show the significant loss of coherence accompanied by…

Moir\'e superlattices of transition-metal dichalcogenides (TMDs) host strongly interacting Bose-Fermi mixtures in which bosonic excitons coexist with correlated electron lattices. Using ultrafast, time- and energy-resolved photoluminescence…

Conjugated polymers offer potential for many diverse applications but we still lack a fundamental microscopic understanding of their electronic structure. Elementary photoexcitations - excitons - span only a few nanometres of a molecule,…

The resolution of Brownian motion in simulations of micro-particle suspensions can be crucial to reproducing the correct dynamics of individual particles, as well as providing an accurate characterisation of suspension properties. Including…

The bilayer systems exhibit the Bose-Einstein condensation of excitons that emerge due to Coulomb pairing of electrons belonging to one layer with the holes belonging to the other layer. Here we present the microscopic derivation of the…

An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…

Understanding the ultrafast vibrational relaxation following photoexcitation of molecules in a condensed phase is essential to predict the outcome and improve the efficiency of photoinduced molecular processes. Here, the vibrational…

A system of several Wannier-Mott excitons interacting with phonons in a bulk material is considered. We show that strong exciton-phonon coupling causes the formation of a coherent two-exciton state -- the exciton pair. Unlike the…

The dynamics of pigment-pigment and pigment-protein interactions in light-harvesting complexes is studied with a novel approach which combines molecular dynamics (MD) simulations with quantum chemistry (QC) calculations. The MD simulations…

For finite-dimensional quantum systems, such as qubits, a well established strategy to protect such systems from decoherence is dynamical decoupling. However many promising quantum devices, such as oscillators, are infinite dimensional, for…

The interplay of dynamics and transport leads to intriguing spatiotemporal behaviors of nonequilibrium macroscopic quantum systems. By means of time-resolved spectroscopy, we here provide microscopic insights into the interplay of ballistic…

We study the time evolution of excitonic states after photo-excitation in the one-dimensional spin-less extended Falicov-Kimball model. Several numerical methods are employed and benchmarked against each other: time-dependent mean-field…

The UV photochemistry of small heteroaromatic molecules serves as a testbed for understanding fundamental photoinduced transformations in moderately complex compounds, including isomerization, ring-opening, and molecular dissociation. Here,…

We study dynamics of clustering in systems containing active particles that are immersed in an explicit solvent. For this purpose we have adopted a hybrid simulation method, consisting of molecular dynamics and multi-particle collision…

Using dissipative particle dynamics (DPD) simulation method, we study the phase separation dynamics in block copolymer (BCP) melt in $d=3$, subjected to external stimuli such as light. An initial homogeneous BCP melt is rapidly quenched to…

The photoluminescence dynamics of a microscopic gas of indirect excitons trapped in coupled quantum wells is probed at very low bath temperature (approximately 350 mK). Our experiments reveal the non linear energy relaxation characteristics…

We study the effect of decoherence on dynamical phase diffusion in the two-site Bose-Hubbard model. Starting with an odd parity excited coherent state, the initial loss of single particle coherence varies from small bound oscillations in…

Recently it was shown that by means of an STM it is experimentally possible to stimulate clock transitions between the singlet and the non-magnetic triplet state of a Heisenberg-coupled spin dimer (Bae et al., Science Advances 4, eaau4159).…

Molecular polaritons, hybrid light-matter states resulting from strong cavity coupling of optical transitions, may provide a new route to guide chemical reactions. However, demonstrations of cavity-modified reactivity in clean benchmark…

We have investigated the time-evolution of a free particle in interaction with a phonon thermal bath, using the tight-binding approach. A dissipative quantum walk can be defined and many important non-equilibrium decoherence properties can…