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Van der Waals heterostructures have recently emerged as an exciting platform for investigating the effects of strong electronic correlations, including various forms of magnetic or electrical orders. Here, we perform an unbiased exact…

强关联电子 · 物理学 2024-07-15 Ahmed Abouelkomsan , Emil J. Bergholtz , Shubhayu Chatterjee

Converting solar energy into chemical energy by splitting water is a promising means to generate a sustainable and renewable solution without detrimental environmental impact. The two-dimensional semiconductors serve as potential catalysts…

介观与纳米尺度物理 · 物理学 2019-09-18 Srilatha Arra , Rohit Babar , Mukul Kabir

Two-dimensional Transition-Metal Dichalcogenides (TMDs) are of great interest for second harmonic (SH) generation due to their large second-order susceptibility, atomically thin structure, and relaxed phase-matching conditions. TMDs are…

Transition metal dichalcogenides (TMDs) are regarded as a possible materials platform for quantum information science and related device applications. In TMD monolayers, the dephasing time and inhomogeneity are crucial parameters for any…

Two-dimensional transition-metal dichalcogenides (TMDs) are gaining increasing attention as alternative to graphene for their very high potential in optoelectronics applications. Here we consider two prototypical metallic 2D TMDs, NbSe$_2$…

材料科学 · 物理学 2015-06-18 Pierluigi Cudazzo , Matteo Gatti , Angel Rubio

Atomic-scale control of light-matter interactions represent the ultimate frontier for many applications in photonics and quantum technology. Two-dimensional semiconductors, including transition metal dichalcogenides, are a promising…

介观与纳米尺度物理 · 物理学 2024-08-22 John M. Woods , Saroj B. Chand , Enrique Mejia , Takashi Taniguchi , Kenji Watanabe , Johannes Flick , Gabriele Grosso

The science and applications of electronics and optoelectronics have been driven for decades by progress in growth of semiconducting heterostructures. Many applications in the infrared and terahertz frequency range exploit transitions…

Atomically thin two-dimensional (2D) semiconductors are extensively investigated for opto-electronic applications that require strong light-matter interactions. In view of such applications, it is essential to understand how…

材料科学 · 物理学 2022-11-16 Pieter Schiettecatte , Zeger Hens , Pieter Geiregat

Layered transition metal dichalcogenide (TMD) materials, i.e. 1T-TiSe$_2$ and 2H-NbSe$_2$, harbor a second order charge density wave (CDW) transition where phonons play a key role for the periodic modulations of conduction electron…

强关联电子 · 物理学 2017-10-11 Ang J. Li , Xiaochen Zhu , Daniel Rhodes , Christopher C. Samouce , Luis Balicas , Arthur F. Hebard

van der Waals (vdW) heterojunctions formed by two-dimensional (2D) materials have attracted tremendous attention due to their excellent electrical/optical properties and device applications. However, current 2D heterojunctions are largely…

Tuning dimensionality in van der Waals materials with finite interlayer coupling has introduced various electronic phase transitions by conventional mechanical exfoliation. Particularly when the electronic order is tied to the modulation of…

强关联电子 · 物理学 2023-01-12 Hyoung Kug Kim , So Young Kim , C. J. Won , Sang-Wook Cheong , Jonghwan Kim , Jun Sung Kim , Tae-Hwan Kim

At the few-atom-thick limit, transition metal dichalcogenides (TMDs) exhibit a host of attractive electronic optical, and structural properties. The possibility to pattern these properties has a great impact on applied and fundamental…

The optical response of two-dimensional (2D) materials has been customarily calculated ab initio using plane waves and without separating the most important orbitals contributions. In the family of transition metal dichalcogenides (TMDC)…

介观与纳米尺度物理 · 物理学 2025-12-30 Angiolo Huamán

Heterostructures of transition metal dichalcogenides (TMDs) offer unique opportunities in optoelectronics due to their strong light-matter interaction and the formation of dipolar interlayer excitons. Introducing a twist angle or lattice…

光学 · 物理学 2025-09-16 Giuseppe Meneghini , Samuel Brem , Ermin Malic

Integration of two-dimensional (2D) van der Waals (vdWs) materials with non-2D materials to realize mixed-dimensional heterostructures has potential for creating functional devices beyond the reach of existing materials and has long been a…

材料科学 · 物理学 2022-12-06 Ya-Ning Ren , Mo-Han Zhang , Qi Zheng , Lin He

Bilayer two-dimensional (2D) van der Waals (vdW) materials are attracting increasing attention due to their predicted high quality electronic and optical properties. Here we demonstrate dense, selective growth of WSe2 bilayer flakes by…

Two-dimensional materials and their van der Waals heterostructures enable a large range of applications, including label-free biosensing. Lattice mismatch and work function difference in the heterostructure material result in strain and…

介观与纳米尺度物理 · 物理学 2021-11-19 Tetyana Ignatova , Sajedeh Pourianejad , Xinyi Li , Kirby Schmidt , Frederick Aryeetey , Shyam Aravamudhan , Slava V. Rotkin

The optical and electronic properties of 2D semiconductors are intrinsically linked via the strong interactions between optically excited bound species and free carriers. Here we use near-field scanning microwave microscopy (SMM) to image…

Quantifying anisotropy in the chemical reactions of mesoscopic crystals has mostly resorted on the combination of electron microscopy and diffraction. In this work, we established crystal-facet-resolved kinetic measurements of oxidation…

化学物理 · 物理学 2021-07-19 Myeongin Song , Haneul Kang , Dan Rhodes , Bumho Kim , James Hone , Sunmin Ryu

2D intercorrelated ferroelectrics, exhibiting a coupled in-plane and out-of-plane ferroelectricity, is a fundamental phenomenon in the field of condensed-mater physics. The current research is based on the paradigm of bi-directional…

材料科学 · 物理学 2020-11-24 Yan Liang , Shiying Shen , Baibiao Haung , Ying Dai , Yandong Ma