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The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

化学物理 · 物理学 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

Using a new technique to directly detect current induced on a nearby electrode, we measure plasma oscillations in ultracold plasmas, which are influenced by the inhomogeneous and time-varying density and changing neutrality. Electronic…

等离子体物理 · 物理学 2012-02-10 K. A. Twedt , S. L. Rolston

Understanding the interaction between metal ions and their aqueous environment is fundamental in many areas of chemistry, biology, and environmental science. In this study, we investigate the electronic structure of hydrated calcium ions,…

Conical intersections play a pivotal role in excited-state quantum dynamics. Capturing transient molecular structures near conical intersections remains challenging due to the rapid timescales and subtle structural changes involved. We…

How atoms and electrons in a molecule move during a chemical reaction and how rapidly energy is transferred to or from the surroundings can be studied with flashes of laser light. However, despite prolonged efforts to develop various…

化学物理 · 物理学 2022-01-05 JunWoo Kim , Jonggu Jeon , Tai Hyun Yoon , Minhaeng Cho

Ultrafast electron microscopy (UEM) has found widespread applications in physics, chemistry, and materials science, enabling real-space imaging of dynamics on ultrafast timescales. Recent advances have pushed the temporal resolution of UEM…

For atoms embedded in dense plasma, the plasma screening effects will greatly alter their structure and dynamics, and then determine the radiation transport properties of the plasma. In the present work, a new statistical model is proposed…

等离子体物理 · 物理学 2020-11-25 Fuyang Zhou , Yizhi Qu , Junwen Gao , Yulong Ma , Yong Wu , Jianguo Wang

Independent particle model in nuclear physics assumes that the nucleon in the nucleus moves in the average (mean field) potential generated by all other nucleons. This chapter gives a short overview of basic features of the independent…

核理论 · 物理学 2022-09-13 A. V. Afanasjev

Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…

化学物理 · 物理学 2017-12-19 Matz Liebel , Costanza Toninelli , Niek F. van Hulst

We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…

Solving the electronic Schr\"odinger equation for changing nuclear coordinates provides access to the Born-Oppenheimer potential energy surface. This surface is the key starting point for almost all theoretical studies of chemical processes…

化学物理 · 物理学 2022-01-14 Markus Reiher

We present a novel nuclear energy density functional method to calculate spectroscopic properties of atomic nuclei. Intrinsic nuclear quadrupole deformations and rotational frequencies are considered simultaneously as the degrees of freedom…

核理论 · 物理学 2016-02-10 J. Luis Egido , Marta Borrajo , Tomás R. Rodríguez

Techniques in time- and angle-resolved photoemission spectroscopy have facilitated a number of recent advances in the study of quantum materials. We review developments in this field related to the study of incoherent nonequilibrium…

强关联电子 · 物理学 2016-10-04 Christopher L. Smallwood , Robert A. Kaindl , Alessandra Lanzara

Due to the electron correlation, a fast removal of an electron from a molecule may create a coherent superposition of cationic states and in this way initiate pure electronic dynamics in which the hole-charge left by ionization migrates…

化学物理 · 物理学 2023-04-03 J. Vester , V. Despré , A. I. Kuleff

The properties of nuclei embedded in an electron gas are studied within the relativistic mean-field approach. These studies are relevant for nuclear properties in astrophysical environments such as neutron-star crusts and supernova…

核理论 · 物理学 2008-11-26 Thomas J. Buervenich , Igor N. Mishustin , Walter Greiner

Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

量子物理 · 物理学 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

Double-beta processes play a key role in the exploration of neutrino and weak interaction properties, and in the searches for effects beyond the Standard Model. During the last half century many attempts were undertaken to search for…

高能物理 - 唯象学 · 物理学 2020-12-18 K. Blaum , S. Eliseev , F. A. Danevich , V. I. Tretyak , Sergey Kovalenko , M. I. Krivoruchenko , Yu. N. Novikov , J. Suhonen

The most important law of radioactivity is that of the exponential decay. In the realm of quantum mechanics, however, this decay law is neither rigorous nor fundamental. The deviations from the exponential decay have been observed…

核理论 · 物理学 2023-06-26 S. M. Wang , W. Nazarewicz , A. Volya , Y. G. Ma

The rotating nuclei represent one of most interesting subjects for theoretical and experimental studies. They open a new dimension of nuclear landscape, namely, spin direction. Contrary to the majority of nuclear systems, their properties…

核理论 · 物理学 2016-04-27 A. V. Afanasjev

Double-resonant photoexcitation of nitric oxide in a molecular beam creates a dense ensemble of $50f(2)$ Rydberg states, which evolves to form a plasma of free electrons trapped in the potential well of an NO$^+$ spacecharge. The plasma…

化学物理 · 物理学 2015-05-27 N. Saquet , J. P. Morrison , M. Schulz-Weiling , H. Sadeghi , J. Yiu , C. J. Rennick , E. R. Grant