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相关论文: Efficient electrochemical reduction of CO2 to CO b…

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To pursuit high electrochemical performance of supercapacitors based on Faradaic charge-transfer with redox reaction or absorption/desorption effect, the intercalation efficiency of electrolyte ions into electrode materials is a crucial…

材料科学 · 物理学 2017-06-27 Shuang Zhou , Huimin Gao , Cheng Zhang , Jie Yang , Shaolong Tang , Qingyu Xu , Shuai Dong

Capture and conversion of CO2 are of great importance for environment-friendly and sustainable development of human society. Poly(ionic liquid)s (PILs) combine some unique properties of ILs with that of polymers and are versatile materials…

化学物理 · 物理学 2019-01-16 Xianjing Zhou , Jens Weber , Jiayin Yuan

Enhancing the transport of oxygen anions in the cathode while maintaining surface stability is essential for improving the performance of intermediate-temperature solid oxide fuel cells (IT-SOFCs). This study investigates a novel cathode…

材料科学 · 物理学 2025-03-04 Jyotsana Kalaa , Vicky Dhongde , Suddhasatwa Basu , Brajesh Kumar Mani , M. Ali Haider

We have studied electron-induced ion-pair dissociation dynamics of CO using the state-of-art velocity map imaging technique in combination with a time-of-flight-based two-field mass spectrometer. Extracting the characteristics for O$^-$/CO…

原子物理 · 物理学 2022-08-31 Narayan Kundu , Vikrant Kumar , Dhananjay Nandi

The formation of well-defined three-dimensional (3D) redox-active molecular nanostructures at the electrode surfaces may open additional routes to achieve higher conductance in molecular junctions (MJs). We report here experimental and…

The electro-Fenton (EF) process using a boron-doped diamond (BDD) anode and a carbon cloth air-diffusion cathode was optimized for efficient fipronil degradation. The system achieved high H2O2 electrogeneration with close to 80% current…

The photochemical CO2 reduction reaction represents a zero-carbon pathway for converting CO2 into value-added chemicals, yet its industrial implementation has been constrained by low selectivity and product diversity. Dirac nodal arc…

材料科学 · 物理学 2026-02-23 Kangwang Wang , Jie Zhan , Jun Liu , Zaichen Xiang , Wanyi Zhang , Lingyong Zeng , Kai Yan , Yan Sun , Huixia Luo

The conductivity of ionic solutions is arguably their most important trait, being widely used in electrochemical, biochemical, and environmental applications. The Debye-H\"uckel-Onsager theory successfully predicts the conductivity at very…

软凝聚态物质 · 物理学 2023-01-03 Yael Avni , Ram M. Adar , David Andelman , Henri Orland

Lithium titanium oxide Li$_4$Ti$_5$O$_{12}$ (LTO) is an intriguing anode material promising particularly long lived batteries, due to its remarkable phase stability during (dis)charging of the cell. However, its usage is limited by its low…

Herein, NiO nanosheets supported with Ag single atoms are synthesized for photothermal CO2 hydrogenation to achieve 1065 mmol g$^{-1}$ h$^{-1}$ of CO production rate under 1 sun irradiation, revealing the unparalleled weak sunlight driven…

This article is withdrawn since it is published in a journal We report on the first reduction methodology, compatible with flexible, temperature sensitive substrates, for the production of reduced spin coated graphene oxide (GO) electrodes.…

Excessive CO2 emission from fossil fuel usage has resulted in global warming and environmental crises. To solve this problem, the photocatalytic conversion of CO2 to CO or useful components is a new strategy that has received significant…

材料科学 · 物理学 2023-01-27 Saeid Akrami , Tatsumi Ishihara , Masayoshi Fuji , Kaveh Edalati

The development of novel task-specific ionic liquids (ILs) represents an essential challenge in modern organic and physical chemistries. Recently we reported surface-active ILs contained the two well-known organic cations…

软凝聚态物质 · 物理学 2022-01-04 Vitaly V. Chaban

The requirements for beneficial materials restructuring into a higher performance OER electrocatalyst are still a largely open question. Here we use Erythrite (Co$_3$(AsO$_4$)$_2\cdot$8H$_2$O) as a Co-based OER electrocatalyst to evaluate…

The use of proton exchange membrane (PEM) electrolyzers is the method of choice for the conversion of solar energy when frequently occurring changes of the current load are an issue. However, this technique requires electrolytes with low…

Electrochemically mediated selective adsorption is an emerging electrosorption technique that utilizes Faradaically enhanced redox active electrodes, which can adsorb ions not only electrostatically, but also electrochemically. The superb…

化学物理 · 物理学 2021-01-05 Fan He , Martin Z. Bazant , T. Alan Hatton

Nowadays, electrochemical reduction of CO$_2$ has been considered as an effective method to solve the problem of global warming. The primary challenge in studying the mechanism is to determine the adsorption states of CO$_2$, since…

化学物理 · 物理学 2020-07-03 Shuai Guo , Yao Li , Lei Liu , Xiangping Zhang , Suojiang Zhang

Cobalt-porphyrin catalyzed reductive decomposition of CO2 to CO is investigated based on Koper's water facilitated CO2 reduction mechanism using a simple but accurate protocol based on thermodynamics. In our protocol, accurate predictions…

介观与纳米尺度物理 · 物理学 2019-05-06 Kaito Miyamoto , Ryoji Asahi

Covalent-organic frameworks (COFs) are intriguing platforms for designing functional molecular materials. Here, we present a computational study based on van der Waals dispersion-corrected hybrid density functional theory (DFT-D) to design…

材料科学 · 物理学 2017-09-07 Srimanta Pakhira , Kevin P. Lucht , Jose L. Mendoza-Cortes

An attractive class of materials for photo(electro)chemical reactions are hybrids based on semiconducting metal oxides and nanocarbons (e.g. carbon nanotubes (CNT), graphene), where the nanocarbon acts as a highly-stable conductive scaffold…