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Static dipole polarizabilities are calculated in the ground and metastable states of Sr$^+$, Ba$^+$ and Ra$^+$ using the relativistic coupled-cluster method. Trends of the electron correlation effects are investigated in these atomic ions.…

原子物理 · 物理学 2015-05-14 B. K. Sahoo , R. G. E. Timmermans , B. P. Das , D. Mukherjee

Relativistic many-body perturbation theory is applied to study properties of ions of the francium isoelectronic sequence. Specifically, energies of the 7s, 7p, 6d, and 5f states of Fr-like ions with nuclear charges Z = 87 - 100 are…

原子物理 · 物理学 2009-11-13 U. I. Safronova , W. R. Johnson , M. S. Safronova

We present the formulation and implementation of triples correction scheme to the relativistic equation-of-motion coupled-cluster method for ionization potential. Both full and partial triples correction schemes are implemented using the…

化学物理 · 物理学 2026-03-31 Mrinal Thapa , Achinyta Kumar Dutta

The successive ionization potentials (IPs) and electron affinities (EAs) for superheavy elements with $111 \leq Z \leq 114$, namely, Rg, Cn, Nh, and Fl are reexamined using the relativistic Fock-space coupled-cluster method with…

A Cholesky decomposition (CD)-based implementation of relativistic two-component coupled-cluster (CC) and equation-of-motion CC (EOM-CC) methods using an exact two-component Hamiltonian augmented with atomic-mean-field spin-orbit integrals…

化学物理 · 物理学 2023-09-19 Chaoqun Zhang , Filippo Lipparini , Stella Stopkowicz , Jürgen Gauss , Lan Cheng

We compute the ground-state electric dipole polarizability of group-IIIA ions using the perturbed relativistic coupled-cluster (PRCC) theory. To account for the relativistic effects and QED corrections, we use the Dirac-Coulomb-Breit…

原子物理 · 物理学 2020-01-15 Ravi Kumar , S. Chattopadhyay , B. K. Mani , D. Angom

High-accuracy calculations of electric dipole polarizabilities and quadrupole moments ($\Theta$) of the clock states of the singly charged calcium (Ca$^+$), strontium (Sr$^+$) and barium (Ba$^+$) alkaline-earth ions are estimated by…

原子物理 · 物理学 2026-01-28 A. Chakraborty , Vaibhav Katyal , B. K. Sahoo

The perturbed relativistic coupled-cluster (PRCC) theory is applied to calculate the electric dipole polarizabilities of alkaline Earth metal atoms. The Dirac-Coulomb-Breit atomic Hamiltonian is used and we include the triple excitations in…

原子物理 · 物理学 2014-02-10 S. Chattopadhyay , B. K. Mani , D. Angom

Mercury (Hg) and superheavy element copernicium (Cn) are investigated using equation-of-motion relativistic coupled-cluster (EOM-RCC) and configuration interaction plus many-body perturbation theory (CI+MBPT) methods. Key atomic properties…

原子物理 · 物理学 2025-07-25 Hongxu Liu , Jize Han , Yanmei Yu , Yanfeng Ge , Yong Liu , Zhiguo Huang

The low-lying n(=3,4,5)d $^2D_{5/2}$ states alkaline earth ions are of vital importance in a number of different physical applications. The hyperfine structure constants of these states are characterized by unusually strong electron…

原子物理 · 物理学 2015-06-26 B. K. Sahoo , C. Sur , T. Beier , B. P. Das , R. K. Chaudhuri , D. Mukherjee

We report an implementation of the core-valence separation approach to the 4-component relativistic Hamiltonian based equation-of-motion coupled-cluster with singles and doubles theory (CVS-EOM-CCSD), for the calculation of relativistic…

Alkaline-earth-like transition-metal atoms such as Zn and Cd are promising candidates for precision measurements and quantum many-body physics experiments. Here, we theoretically investigate the properties of diatomic molecules containing…

原子物理 · 物理学 2021-11-02 Klaudia Zaremba-Kopczyk , Michał Tomza

We employ four-component spinor relativistic equation-of-motion coupled-cluster (EOMCC) method within the single- and double- excitation approximation to calculate the single ionization potentials (IPs) and double ionization potentials…

原子物理 · 物理学 2015-06-11 Himadri Pathak , B. K. Sahoo , Turbasu Sengupta , B. P. Das , Nayana Vaval , Sourav Pal

The article considers the successful implementation of relativistic equation-of-motion coupled cluster method for the electron attachment problem (EA-EOMCC) at the level of single- and double- excitation approximation. The implemented…

原子物理 · 物理学 2016-01-06 Himadri Pathak , Sudip Sasmal , Malaya K. Nayak , Nayana Vaval , Sourav Pal

Atomic properties of the 24 low-lying ns, np, nd, nf, and ng states in Th IV ion are calculated using the high-precision relativistic all-order method where all single, double, and partial triple excitations of the Dirac-Fock wave functions…

原子物理 · 物理学 2015-06-15 M. S. Safronova , U. I. Safronova

The effect of 50\% Cu doping at the Au site in the topological Dirac semimetal CaAuAs is investigated through electronic band structure calculations, electrical resistivity, and magnetotransport measurements. Electronic structure…

强关联电子 · 物理学 2022-08-15 Sudip Malick , Arup Ghosh , Chanchal K. Barman , Aftab Alam , Z. Hossain , Prabhat Mandal , J. Nayak

It was shown that the divalent rare earth ions (La, Ce, Gd, Tb, Lu, and Y) in cubic sites in alkaline earth fluorides are unstable with respect to electron autodetachment since its d1(eg) ground state is located in the conduction band which…

材料科学 · 物理学 2016-01-20 A. V. Egranov , T. Yu. Sizova , R. Yu. Shendrik , N. A. Smirnova

Several new aspects of the subtle interplay between electronic correlations and disorder are reviewed. First, the dynamical mean-field theory (DMFT)together with the geometrically averaged ("typical") local density of states is employed to…

强关联电子 · 物理学 2015-05-18 K. Byczuk , W. Hofstetter , U. Yu , D. Vollhardt

The charge, bonding, and optical properties of the calcium-doped boron cluster B$_7$Ca$_2$ have been systematically investigated using density functional theory calculations. Extensive global basin-hopping searches identify a single-ring…

材料科学 · 物理学 2026-03-04 Peter Ludwig Rodríguez-Kessler

We report the implementation of equation-of-motion coupled-cluster (EOMCC) method in the four-component relativistic framework with the spherical atomic potential to generate the excited states from a closed-shell atomic configuration. This…

原子物理 · 物理学 2015-06-19 D. K. Nandy , Yashpal Singh , B. K. Sahoo