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Drying a droplet of colloidal dispersion can result in complex pattern formation due to both development and deformation of a skin at the drop surface. The present study focus on the drying process of droplets of colloidal dispersions in a…

软凝聚态物质 · 物理学 2012-11-08 François Boulogne , Frédérique Giorgiutti-Dauphiné , Ludovic Pauchard

We studied the dependence of solid deposit shape obtained by free drying of sessile drops on the particles concentration and Derjaguin-Landau-Verwey-Overbeek (DLVO) particle/substrate interaction. In contrast to previous contributions using…

软凝聚态物质 · 物理学 2020-11-25 N Bridonneau , M Zhao , N Battaglini , G Mattana , V Thévenet , V Noël , M Roché , S Zrig , F Carn

Understanding flow patterns and coupled transport phenomena during evaporation of droplets loaded with colloidal particles is central to design technical applications such as organizing proteins/DNA on a solid surface. We review recent…

软凝聚态物质 · 物理学 2019-04-16 Nagesh D. Patil , Rajneesh Bhardwaj

Explicit molecular dynamics simulations were applied to a pair of amorphous silica nanoparticles of diameter 3.2 nm immersed in a background electrolyte. Mean forces acting between the pair of silica nanoparticles were extracted at four…

化学物理 · 物理学 2007-09-11 S. Jenkins , S. R. Kirk , M. Persson , J. Carlen , Z. Abbas

We develop a dynamical density functional theory based model for the drying of colloidal films on planar surfaces. We consider mixtures of two different sizes of hard-sphere colloids. Depending on the solvent evaporation rate and the…

软凝聚态物质 · 物理学 2021-01-28 Boshen He , Ignacio Martin-Fabiani , Roland Roth , Gyula I. Tóth , Andrew J. Archer

In this work, we unravel the role of surface properties of colloidal particles on the formation of supraparticles (clusters of colloidal particles) in a colloidal Ouzo droplet. Self-lubricating colloidal Ouzo droplets are an efficient and…

We computed the self-organisation process of a monodisperse collection of spherical micrometric particles trapped in a two-dimensional (2D) thin liquid film isothermally dried on a chemically inert substrate. The substrate is either flat or…

软凝聚态物质 · 物理学 2009-11-11 F. Lallet , N. Olivi-Tran

Hypothesis: Colloidal molecules with anisotropic shapes and interactions are powerful model systems for deciphering the behavior of real molecules and building units for creating materials with designed properties. While many strategies for…

软凝聚态物质 · 物理学 2022-07-19 Yogesh Shelke , Susana Marín-Aguilar , Fabrizio Camerin , Marjolein Dijkstra , Daniela J. Kraft

We report an experimental study of the crack pattern formed during the drying of a colloidal suspension. A horizontal fiber, which provides a one dimensional, boundary-free substrate, is coated by a film of micronic thickness. The geometry…

软凝聚态物质 · 物理学 2014-09-30 François Boulogne , Ludovic Pauchard , Frédérique Giorgiutti-Dauphiné

We report small-angle x-ray scattering (SAXS) experiments on aqueous dispersions of colloidal silica with a broad monomodal size distribution (polydispersity 18%, size 8 nm). Over a range of volume fractions the silica particles segregate…

We review theoretical explanation of mechanisms of control of uniformity in growth of nanosize particles and colloids. The nanoparticles are synthesized as nanocrystals, by burst nucleation from solution. The colloids are self-assembled by…

统计力学 · 物理学 2010-09-22 Vladimir Privman

We consider the dynamic wetting and dewetting processes of films and droplets of complex liquids on planar surfaces, focusing on the case of colloidal suspensions, where the particle interactions can be sufficiently attractive to cause…

流体动力学 · 物理学 2024-11-20 J. Zhang , D. N. Sibley , D. Tseluiko , A. J. Archer

Aqueous colloidal dispersions of silica particles become anisotropic when they are dried through evaporation. This anisotropy is generated by a uniaxial strain of the liquid dispersions as they are compressed by the flow of water toward a…

We are presenting a new method of processing polystyrene-silica nanocomposites, which results in a very well-defined dispersion of small primary aggregates (assembly of 15 nanoparticles of 10 nm diameter) in the matrix. The process is based…

Recent experiments have shown that various structures may be formed during the evaporative dewetting of thin films of colloidal suspensions. Nano-particle deposits of strongly branched `flower-like', labyrinthine and network structures are…

软凝聚态物质 · 物理学 2011-10-03 M. J. Robbins , A. J. Archer , U. Thiele

We extend our previous work on monolayers of uniaxial particles [J. Chem. Phys. 140, 204906 (2014)] to study the effect of particle biaxiality on the phase behavior of liquid-crystal monolayers. Particles are modelled as board-like hard…

软凝聚态物质 · 物理学 2015-06-23 Miguel Gonzalez-Pinto , Yuri Martinez-Raton , Enrique Velasco , Szabolcs Varga

Building structures with hierarchical order through the self-assembly of smaller blocks is not only a prerogative of nature, but also a strategy to design artificial materials with tailored functions. We explore in simulation the…

软凝聚态物质 · 物理学 2020-02-17 Santi Prestipino , Domenico Gazzillo , Gianmarco Munaò , Dino Costa

We investigate deposit patterns and associated morphology formed after the evaporation of an aqueous droplet containing mono- and bi-dispersed colloidal particles. In particular, the combined effect of substrate heating and particle…

流体动力学 · 物理学 2018-07-11 Nagesh D. Patil , Rajneesh Bhardwaj , Atul Sharma

Colloidal particles are considered ideal building blocks to produce materials with enhanced physical properties. The state-of-the-art techniques for synthesizing these particles provide control over shape, size, and directionality of the…

软凝聚态物质 · 物理学 2016-12-21 N. A. M. Araújo , C. S. Dias , M. M. Telo da Gama

Targeting specific technological applications requires the control of nanoparticle properties, especially the crystalline polymorph. Freezing a nanodroplet deposited on a solid substrate leads to the formation of crystalline structures. We…

软凝聚态物质 · 物理学 2018-03-02 Julien Lam , James F. Lutsko