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We perform numerical simulations to study self-assembly of nanoparticles mediated by an elastic planar surface. We show how the nontrivial elastic response to deformations of these surfaces leads to anisotropic interactions between the…

软凝聚态物质 · 物理学 2012-01-04 Andela Šarić , Angelo Cacciuto

Surface diffusion has an impact on the lateral resolution of nanostructures in bottom-up atom nanofabrication. In this paper we study the effects of the gallium atoms self-assembled on silicon surfaces (100) patterned with trenches at…

材料科学 · 物理学 2009-11-10 B. Fazio , O. M. Marago' , E. Arimondo , C. Spinella , C. Bongiorno , G. D'Arrigo

In the field of freezing colloidal suspensions, it is important to understand the particle-scale behavior of particle packing. Here, we reveal the dynamics of particle packing by identifying the behavior of each single particle in situ. The…

材料科学 · 物理学 2017-03-08 Jiaxue You , Jincheng Wang , Lilin Wang , Ziren Wang , Zhijun Wang , Junjie Li , Xin Lin

Silica nanoparticles trapped at air-water interface form a 2D solid state with amorphous order. We propose a theoretical model to describe how this solid-like state deforms under a shear strain ramp up to and beyond a yielding point which…

软凝聚态物质 · 物理学 2017-10-30 Armando Maestro , Alessio Zaccone

We investigate the 3D structure and drying dynamics of complex mixtures of emulsion droplets and colloidal particles, using confocal microscopy. Air invades and rapidly collapses large emulsion droplets, forcing their contents into the…

Patterns generated by a colloidal suspension of nanospheres drying on a frictional substrate are studied by experiments and computer simulations. The obtained two-dimensional self-assembled structures are commonly used for nanosphere…

软凝聚态物质 · 物理学 2009-11-11 F. Jarai-Szabo , S. Astilean , Z. Neda

Conventional drying of colloidal materials and gels (including cement) can lead to detrimental effects due to the buildup of internal stresses as water evaporates from the nano/microscopic pores. However, the underlying nanoscopic…

材料科学 · 物理学 2018-03-29 Kengran Yang , V. Ongun Özçelik , Nishant Garg , Kai Gong , Claire E. White

The ordering of a multilayer consisting of DSPC bilayers on a silica sol substrate is studied within the model-independent approach to the reconstruction of profiles of the electron density from X-ray reflectometry data. It is found that…

The drying of a colloidal dispersion can result in a gel phase defined as a porous matrix saturated in solvent. During the drying process, high mechanical stresses are generated. When these stresses exceed the strength of the material, they…

软凝聚态物质 · 物理学 2013-02-15 François Boulogne , Frédérique Giorgiutti-Dauphiné , Ludovic Pauchard

Since the 1920s, packing arguments have been used to rationalize crystal structures in systems ranging from atomic mixtures to colloidal crystals. Packing arguments have recently been applied to complex nanoparticle structures, where they…

软凝聚态物质 · 物理学 2018-05-09 Rose Cersonsky , Greg van Anders , Paul M. Dodd , Sharon C. Glotzer

Structural rearrangement of polystyrene colloidal crystals under dry sintering conditions has been revealed by in situ grazing incidence X-ray scattering. Measured diffraction patterns were analysed using distorted wave Born approximation…

This short review is devoted to the simple process of drying a multi-component droplet consisting of a complex fluid containing a salt. These processes provide a fascinating subject for study. The explanation of the rich variety of patterns…

软凝聚态物质 · 物理学 2016-11-04 Yuri Yu. Tarasevich , Sujata Tarafdar , Tapati Dutta

We use molecular dynamics computer simulations to study the equilibrium properties of the surface of amorphous silica. Two types of geometries are investigated: i) clusters with different diameters (13.5\AA, 19\AA, and 26.5\AA) and ii) a…

统计力学 · 物理学 2009-10-31 Alexandra Roder , Walter Kob , Kurt Binder

We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically…

We studied the morphology of linear particle deposits obtained by inkjet-printing of silica nanoparticle suspension in drying condition where contact line depinning occurs. We show that this evaporation mode can be obtained by adjusting the…

软凝聚态物质 · 物理学 2020-12-09 N. Bridonneau , G. Mattana , V. Noël , S. Zrig , F. Carn

Using a phase field crystal model we study the structure and dynamics of a drop of colloidal suspension during evaporation of the solvent. We model an experimental system where contact line pinning of the drop on the substrate is…

软凝聚态物质 · 物理学 2012-09-06 Nirmalendu Ganai , Arnab Saha , Surajit Sengupta

Understanding the relationship between colloidal building block shape and self-assembled material structure is important for the development of novel materials by self-assembly. In this regard, colloidal superballs are unique building…

软凝聚态物质 · 物理学 2021-12-16 Sarah N. Schyck , Janne-Mieke Meijer , Lucia Baldauf , Peter Schall , Andrei V. Petukhov , Laura Rossi

We present an experimental investigation of drying suspensions of both hard and soft nanolatex spheres. The crack formation is examined as a function of the proportion of hard and soft deformable particles, leading to tunable elastic…

软凝聚态物质 · 物理学 2010-10-26 L. Pauchard , B. Abou , K. Sekimoto

The structure of the transient layer at the interface between air and the aqueous solution of silica nanoparticles with the size distribution of particles that has been determined from small-angle scattering has been studied by the X-ray…

The ordering of particles in the drying process of a colloidal suspension is crucial in determining the properties of the resulting film. For example, microscopic inhomogeneities can lead to the formation of cracks and defects that can…

软凝聚态物质 · 物理学 2021-10-04 Maarten Wouters , Othmane Aouane , Marcello Sega , Jens Harting